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Localized surface plasmon resonances have recently attracted considerable attention due to their ability to dramatically enhance near-field optical intensities and boost nanoscale light-matter interactions. Here we demonstrate unambiguously…

Optics · Physics 2013-01-30 Neda Ghofraniha , Pascal Andrè , Andrea Di falco , Claudio Conti

Vibrational polaritons, hybrid light-matter states formed between molecular vibrations and infrared (IR) cavity modes, provide a novel approach for modifying chemical reaction pathways and energy transfer processes. For vibrational…

Chemical Physics · Physics 2025-05-16 Xinwei Ji , Tao E. Li

Fabry-Perot microcavities can strongly enhance interactions between light and molecules, leading to the formation of hybrid light-matter states known as polaritons. Polaritons possess much smaller effective masses and much larger group…

Chemical Physics · Physics 2023-10-18 Zeyu Zhou , Hsing-Ta Chen , Maxim Sukharev , Joseph E. Subotnik , Abraham Nitzan

Realizing strong light-matter interactions between individual 2-level systems and resonating cavities in atomic and solid state systems opens up possibilities to study optical nonlinearities on a single photon level, which can be useful for…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Gülis Zengin , Martin Wersäll , Sara Nilsson , Tomasz J. Antosiewicz , Mikael Käll , Timur Shegai

Interaction between light and molecular vibrations leads to hybrid light-matter states called vibrational polaritons. Even though many intriguing phenomena have been predicted for single-molecule vibrational strong coupling (VSC), several…

Resonant photoelastic coupling in semiconductor nanostructures opens new perspectives for strongly enhanced light-sound interaction in optomechanical resonators. One potential problem, however, is the reduction of the cavity Q-factor…

Mesoscale and Nanoscale Physics · Physics 2014-11-19 G. Rozas , A. E. Bruchhausen , A. Fainstein , B. Jusserand , A. Lemaître

Gold nanoparticle assemblies show a strong plasmonic response due to the combined effects of the individual nanoparticles' plasmon modes. Increasing the number of nanoparticles in structured assemblies leads to significant shifts in the…

Optics · Physics 2022-07-13 Aditya K. Sahu , Satyabrata Raj

Optical circuits and light sources, such as lasers, undergo continuous miniaturization. In its extreme, nanolasers might be comprised of only a few molecules confined in plasmonic nanoresonators. Few-emitter lasers promise low energy…

Quantum Physics · Physics 2026-05-08 Kai Müller , Kimmo Luoma , Christian Schäfer

Strong coupling between light and matter generates hybrid polariton modes. We present a continuum formalism that expresses the polariton modes in terms of light and matter densities of states (DOS). We derive exact expressions for the light…

Materials Science · Physics 2024-12-03 Suman Gunasekaran , Ryan F. Pinard , Andrew J. Musser

Resonant coupling of a vibration to a cavity mode has been reported to dramatically modify spontaneous Raman scattering, but subsequent studies have produced conflicting results. In this Letter, we develop a microscopic quantum framework…

Mesoscale and Nanoscale Physics · Physics 2025-11-04 Maxime Dherbécourt , Joël Bellessa , Clémentine Symonds , Guillaume Weick , David Hagenmüller

Realizing nonlinear coupling across space can enable new scientific and technological advances, including ultrafast operation and propagation of information in IR photonic circuitry, remote triggering or catalyzing of chemical reactions,…

Optics · Physics 2019-12-13 Jiaxi Wang , Bo Xiang , Wei Xiong

Recent advances in polaritonic chemistry suggest that chemical reactions can be controlled via collective vibrational strong coupling (VSC) in a cavity. In this fully analytical work, we demonstrate that the collective vibrations of a…

Quantum Physics · Physics 2025-04-15 Vasil Rokaj , Ilia Tutunnikov , H. R. Sadeghpour

Manipulating strong light-matter interaction in semiconductor microcavities is crucial for developing high-performance exciton polariton devices with great potentials in next-generation all-solid state quantum technologies. In this work, we…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 Qiuyu Shang , Shuai Zhang , Jie Chen , Pengfei Yang , Wei Li , Yanfeng Zhang , Qihua Xiong , Xinfeng Liu , Qing Zhang

Strong light-matter coupling has garnered significant attention for its potential to optimize optoelectronic responses. In this study, we designed open cavities featuring non-local metasurfaces composed of aluminum nanoparticle arrays. The…

We theoretically designed and experimentally demonstrated a mechanism to protect a spatially segregated mixed light-matter state, known as intercavity exciton-polariton in strongly coupled optical cavities. This excitation, shared across…

Strong coupling between light and molecular matter is currently attracting interest both in chemistry and physics, in the fast-growing field of molecular polaritonics. The large near-field enhancement of the electric field of plasmonic…

Mesoscale and Nanoscale Physics · Physics 2024-10-03 Álvaro Buendía , Jose A. Sánchez-Gil , Vincenzo Giannini , William L. Barnes , Marie S. Rider

Coupled and shape-tailored metallic nanoparticles are known to exhibit hybridized plasmon resonances. This Letter discuss the optical properties of a complementary system formed by overlapped nanovoid dimers buried in gold and filled with…

Materials Science · Physics 2009-11-13 I. Romero , T. V. Teperik , F. J. Garcia de Abajo

Plasmonic coupling of metallic nanoparticles and adjacent pigments can dramatically increase the brightness of the pigments due to the enhanced local electric field. Here, we demonstrate that the fluorescence brightness of a single plant…

Recent experiments in polariton chemistry have demonstrated that reaction rates can be modified by vibrational strong coupling to an optical cavity mode. Importantly, this modification only occurs when the frequency of the cavity mode is…

Chemical Physics · Physics 2023-05-15 Marit R. Fiechter , Johan E. Runeson , Joseph E. Lawrence , Jeremy O. Richardson

Exciton transport can be enhanced in the strong coupling regime where excitons hybridise with confined light modes to form polaritons. Because polaritons have group velocity, their propagation should be ballistic and long-ranged. However,…

Chemical Physics · Physics 2024-03-20 Ilia Sokolovskii , Ruth H. Tichauer , Dmitry Morozov , Johannes Feist , Gerrit Groenhof