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Related papers: Enhancing vibrational light-matter coupling streng…

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Molecular strong coupling offers exciting prospects in physics, chemistry and materials science. Whilst attention has been focused on developing realistic models for the molecular systems, the important role played by the entire photonic…

The plasmon-mechanical resonators are frequently used in the development of sensors. Active frameworks impose mechanical motion into the lasing dynamics through the use of an optical gain and achieve better sensitivity. Here…

Optics · Physics 2023-07-10 Giuseppina Simone

One of the most popular subjects now being researched in molecular science is strong light-matter coupling. The introduction of vibrational strong coupling and the formation vibro-polaritonic states tend to modify chemical reactivity,…

Chemical Physics · Physics 2023-08-10 Akhila Kadyan , Monu P. Suresh , Ben Johns , Jino George

Developing theoretical frameworks for vibrational strong coupling (VSC) beyond the single-mode approximation is crucial for a comprehensive understanding of experiments with planar Fabry-P\'erot cavities. Herein, a generalized cavity…

Chemical Physics · Physics 2024-06-18 Tao E. Li

Ultrastrong light-matter coupling has traditionally been studied in optical cavities, where it occurs when the light-matter coupling strength reaches a significant fraction of the transition frequency. This regime fundamentally alters the…

Optics · Physics 2025-05-13 Niclas S. Mueller , Eduardo B. Barros , Stephanie Reich

The coupling of mechanical oscillators with light has seen a recent surge of interest, as recent reviews report.[1, 2] This coupling is enhanced when confining light in an optical cavity where the mechanical oscillator is integrated as…

The fluorescence of organic fluorophore molecules is enhanced when they are placed in contact with certain metals (Al, Ag, Cu, Au, etc.) whose surface plasmon waves couple into the radiative modes of the molecules and increase the radiative…

Mesoscale and Nanoscale Physics · Physics 2015-04-21 S. Sarkar , B. Kanchibotla , J. D. Nelson , J. D. Edwards , J. Anderson , G. C. Tepper , S. Bandyopadhyay

The strong coupling of an IR-active molecular transition with an optical mode of the cavity results in vibrational polaritons, which opens a new way to control chemical reactivity via confined electromagnetic fields of the cavity. In this…

Recent years have seen significant developments in the study of strong light-matter coupling including the control of chemical reactions by altering the vibrational normal modes of molecules. In the vibrational strong coupling regime the…

Quantum Physics · Physics 2021-08-27 John Bonini , Johannes Flick

Several years ago, it was shown that strong coupling between an electronic transition in organic molecules and a resonant photonic structure can modify the electronic landscape of the molecules and affect their chemical behavior. Since…

Ultrastrong coupling between optical and material excitations is a distinct regime of electromagnetic interaction that enables a variety of intriguing physical phenomena. Traditional ways to ultrastrong light-matter coupling involve the use…

We demonstrate that the fluorescent emitters can increase light emission from the plasmonic nanostructures in turn. With the help of atomic force microscopy, a hybrid system consisting of a fluorescent nanodiamond and a gold nanoparticle…

Strong light-matter coupling gives rise to polaritons - hybrid excitations whose mixed photonic and matter character enables control over optical, electronic and chemical properties. This Feature Article surveys the main architectures…

Physical and chemical properties of materials can be modified by a resonant optical mode. Such recent demonstrations have mostly relied on a planar cavity geometry, others have relied on a plasmonic resonator. However, the combination of…

We present a microscopic semi-analytical theory for the description of organic molecules interacting strongly with a cavity mode. Exciton-vibration coupling within the molecule and exciton-cavity interaction are treated on an equal footing…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 Ning Wu , Johannes Feist , Francisco J. Garcia-Vidal

Macroscopic spontaneous coherence of exciton-polariton in semiconductor cavity is one important research field in condensed matter physics. All-inorganic micro/nanowire Fabry-P\'erot cavity with excellent optical performance makes it…

Mesoscale and Nanoscale Physics · Physics 2017-11-16 Wenna Du , Shuai Zhang , Jia Shi , Jie Chen , Zhiyong Wu , Yang Mi , Zhixiong Liu , Yuanzheng Li , Xinyu Sui , Tom Wu , Yunfeng Xiao , Qing Zhang , Xinfeng Liu

Recent experiments have demonstrated that molecular polaritons, hybrid states of light and matter formed by the strong coupling between molecular electronic or vibrational excitations and an optical cavity, can substantially modify the…

Chemical Physics · Physics 2021-07-08 Nguyen Thanh Phuc

Strong coupling of molecules to vacuum fields has been widely reported to lead to modified chemical properties such as reaction rates. However, some recent attempts to reproduce infrared strong coupling results have not been successful,…

Mesoscale and Nanoscale Physics · Physics 2024-01-03 Philip A. Thomas , Wai Jue Tan , Vasyl G. Kravets , Alexander N. Grigorenko , William L. Barnes

There is growing interest in using strongly coupled organic microcavities to tune molecular dynamics, including the electronic and vibrational properties of molecules. However, very little attention has been paid to the utility of cavity…

Materials Science · Physics 2024-06-12 Bin Liu , Vinod M. Menon , Matthew Y. Sfeir

We show that strong electron-electron interactions in cavity-coupled quantum materials can enable collectively enhanced light-matter interactions with ultrastrong effective coupling strengths. As a paradigmatic example we consider a…

Strongly Correlated Electrons · Physics 2019-09-04 Martin Kiffner , Jonathan Coulthard , Frank Schlawin , Arzhang Ardavan , Dieter Jaksch