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In order to explore the consequences of spin-orbit coupling on spin-phonon interactions in a set of chemically-similar mixed metal oxides, we measured the infrared vibrational properties of Co$_4B_2$O$_9$ ($B$ = Nb, Ta) as a function of…

Materials Science · Physics 2023-05-26 K. Park , J. Kim , S. Choi , S. Fan , C. Kim , D. G. Oh , N. Lee , S. -W. Cheong , V. Kiryukhin , Y. J. Choi , D. Vanderbilt , J. H. Lee , J. L. Musfeldt

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

For quasi-one dimensional quantum spin systems theory predicts the occurrence of a confinement of spinon excitation due to interchain couplings. Here we investigate the system SrCo2V2O8, a realization of the weakly-coupled Ising-like XXZ…

Strongly Correlated Electrons · Physics 2015-04-10 Zhe Wang , M. Schmidt , A. K. Bera , A. T. M. N. Islam , B. Lake , A. Loidl , J. Deisenhofer

We have investigated the magnetic and magnetocaloric properties of antiferromagnetic Ising spin chain CoV$_{2}$O$_{6}$ by magnetization and heat capacity measurements. Both monoclinic $\alpha$-CoV$_{2}$O$_{6}$ and triclinic…

Strongly Correlated Electrons · Physics 2016-05-04 M. Nandi , P. Mandal

Among the 3d transition metal ions doped polar Ni3TeO6, Mn-doped Ni3TeO6 has stimulated great interest due to its high magnetic ordering temperature and complex magnetic phases, but the mechanism of magnetoelectric (ME) coupling is far from…

The magnetic properties of the molecular cluster Mn12Ac are due to the four Mn3+ ions which have spins S=3/2 and the eight Mn4+ ions with spins S=2. These spins are coupled by superexchange mechanism. We determine the four exchange…

Strongly Correlated Electrons · Physics 2009-11-07 N. Regnault , Th. Jolicoeur , R. Sessoli , D. Gatteschi , M. Verdaguer

The magnetoelectric effect and skyrmions are two fundamental phenomena in the field of condensed-matter physics. Here, using first-principles calculations and Monte-Carlo simulations, we propose that strong magnetoelectric coupling can be…

Materials Science · Physics 2022-06-01 Kaiying Dou , Wenhui Du , Ying Dai , Baibiao Huang , Yandong Ma

The results of ac and dc magnetization and heat capacity measurements as a function of temperature (T = 1.8 to 300 K) are reported for a quasi-one-dimensional compound, Ca$_3$CuMnO$_6$, crystallizing in a triclinically distorted…

Strongly Correlated Electrons · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , K. K. Iyer , E. V. Sampathkumaran

Magnetoelectric coupling permits a magnetic order parameter to be addressed electrically or vice versa, and could find use in data storage, field sensors and actuators. Coupling constants for single phase materials such as chromium dioxide,…

Materials Science · Physics 2007-05-23 W. Eerenstein , M. Wiora , J. L. Prieto , J. F. Scott , N. D. Mathur

Dielectric and magnetic phenomena in spin and charge frustrated system RFe2O4 (R is a rare-earth metal ion) are studied. An electronic model for charge, spin and orbital degrees in a pair of triangular-lattice planes is derived. We analyze…

Strongly Correlated Electrons · Physics 2009-11-13 Makoto Naka , Aya Nagano , Sumio Ishihara

The intermetallic compound Nd$_2$Co$_{0.85}$Si$_{2.88}$ having a triangular lattice could be synthesized in single-phase only with defect crystal structure. Investigation through different experimental techniques indicate the presence of…

The magnetoelectric coupling effect serves as a crucial bridge between electrical and magnetic order parameters in condensed matter physics, forming the physical basis for the development of next-generation low-power information storage and…

Materials Science · Physics 2025-12-16 Yalong Yu , Hengwei Zhang , Xiaoyan Liu , Tao Chu

A spin-ice compound dysprosium titanate, Dy2Ti2O7, is studied by specific heat measurements in magnetic fields applied along the [110] direction of the cubic unit cell. Above a magnetic field of 0.4 T a relatively sharp peak at T = 1.1 K in…

Materials Science · Physics 2009-11-10 Zenji Hiroi , Kazuyuki Matsuhira , Masao Ogata

We report on the longitudinal magnetoresistance (MR) in thin metal films on an Ising-type antiferromagnetic insulator, Na5Co15.5Te6O36 (NCTO). Steep changes in the MR spectra with hysteresis were observed at spin-flip transitions driven by…

Strongly Correlated Electrons · Physics 2026-05-04 Hirotsugu Tagami , Takuya Kawada , Yuki Shiomi

Good quality and fine grain Bi6Fe2Ti3O18 magnetic ferroelectric films with single-phase layered perovskite structure have been successfully prepared via metal organic decomposition (MOD) method. Results of low-temperature magnetocapacitance…

Materials Science · Physics 2007-05-23 J. Lu , L. J. Qiao , X. Q. Ma , W. Y. Chu

We report detailed Raman spectroscopic and magnetic susceptibility studies on the spin-driven ferroelectric compounds Mn4Nb2O9 (MNO) and Mn4Ta2O9 (MTO). Both systems exhibit strong spin-phonon coupling below the short-range magnetic…

Materials Science · Physics 2026-02-09 Rajesh Jana , Alka Garg , Rekha Rao , Thomas Meier

We investigate magnetic properties of the $s$ = 1/2 compound K$_{2}$Cu$_{3}$(MoO$_{4}$)$_{4}$ by combining magnetic susceptibility, magnetization, specific heat, and electron spin resonance (ESR) with density functional calculations. Its…

The microscopic spin-spin correlations in the 2D layered spin-1 honeycomb lattice compound Na2Ni2TeO6 have been investigated by neutron diffraction and inelastic neutron scattering. The honeycomb lattice of spin-1 Ni2+ ions, within the…

Strongly Correlated Electrons · Physics 2022-02-17 A. K. Bera , S. M. Yusuf , L. Keller , F. Yokaichiya , J. R. Stewart

We report magneto-dielectric properties of partially B-site ordered monoclinic Tb2CoMnO6 double perovskite thin film epitaxially grown by metalorganic aerosol deposition technique. Transmission electron microscopy and electron energy loss…

Strongly Correlated Electrons · Physics 2020-03-25 R. Mandal , M. Chandra , V. Roddatis , M. Tripathi , R. Rawat , R. J. Choudhary , V. Moshnyaga

We present a joint experimental and theoretical characterization of the magnetic properties of coordination clusters with an antiferromagnetic core of four magnetic ions. Two different compounds are analyzed, with Co and Mn ions in the…

Chemical Physics · Physics 2021-09-16 Simona Achilli , Claire Besson , Xu He , Pablo Ordejòn , Carola Meyer , Zeila Zanolli