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The dielectric behavior of the single crystals of the spin-chain system Ca3Co2O6, undergoing geometrically frustrated antiferromagnetic ordering below 25 K, has been investigated as a function of temperature and magnetic field (H) and…

Materials Science · Physics 2016-03-17 Tathamay Basu , Kartik K. Iyer , P. L. Paulose , E. V. Sampathkumaran

Dielectric constant measurement under magnetic field is an efficient technique to study the coupling between charges and spins in insulating materials. For magnetic oxides, the geometric frustration is known to be a key ingredient to…

Materials Science · Physics 2009-11-13 Natalia Bellido , Charles Simon , Antoine Maignan

A large spin-orbit coupling is a way to control strong magnetodielectric (MD) coupling in a higher d-orbital materials. However reports are rare on such compounds due to often leaky conductive behavior. Here, we demonstrate MD coupling in a…

Materials Science · Physics 2018-07-25 Tathamay Basu , Alain Pautrat , Vincent Hardy , Alois Loidl , Stephan Krohns

The magnetoelectric (ME) effects are investigated in a cubic compound SrCuTe2O6, in which uniform Cu2+ (S=1/2) spin chains with considerable spin frustration exhibit a concomitant antiferromagnetic transition and dielectric constant peak at…

Materials Science · Physics 2016-03-16 B. Koteswararao , Kyongjun Yoo , F. C. Chou , Kee Hoon Kim

We study the magnetocapacitance (MC) effect and magnetoelectric (ME) coupling in spin-flop driven antiferromagnet Co4Ta2O9. The magnetocapacitance data at high magnetic fields are analyzed by phenomenological Ginzburg-landau theory of…

Materials Science · Physics 2017-07-12 S. Chaudhary , P. Srivastava , S. Patnaik

We report that the spin-chain compound Dy2BaNiO5 recently proven to exhibit magnetoelectric coupling below its Neel temperature (T_N) of 58 K, exhibits strong frequency-dependent behavior in ac magnetic susceptibility and complex dielectric…

Strongly Correlated Electrons · Physics 2014-03-18 Tathamay Basu , P. L. Paulose , Kartik K Iyer , Kiran Singh , N. Mohapatra , S. Chowki , Babu Gonde , E. V. Sampathkumaran

We have studied magnetodielectric and spin-lattice coupling in CoNb$_{2}$O$_{6}$ single crystals. Magnetostriction and magnetodielectric experiments are performed at temperatures in and above antifferomagnetic phase of quasi 1D Ising spin…

Strongly Correlated Electrons · Physics 2016-09-08 M. Nandi , D. Prabhakaran , P. Mandal

We present polarised-neutron diffraction measurements of the Ising-like spin-chain compound Ca3Co2O6 above and below the magnetic ordering temperature TN. Below TN, a clear evolution from a single-phase spin-density wave (SDW) structure to…

We report magnetization measurements and magnetic resonance data for SrTiO3 doped by manganese. We show that the recently reported coexistent spin and dipole glass (multiglass) behaviours are strongly affected by the distribution of Mn ions…

We report the results of various measurements, namely magnetization, complex dielectric permittivity and electric polarization (P) on Dy2BaNiO5 as a function of temperature (T) and magnetic-field (H), apart from heat-capacity (C), with the…

Materials Science · Physics 2015-06-15 Kiran Singh , Tathamay Basu , S. Chowki , N. Mahapotra , K. Iyer , P. L. Paulose , E. V. Sampathkumaran

We report a neutron diffraction study of the multiferroic mechanism in (ND4)2FeCl5D2O, a molecular compound that exhibits magnetically induced ferroelectricity. This material exhibits two successive magnetic transitions on cooling: a…

We have investigated the magnetic, dielectric and magnetodielectric (MDE) behavior of a geometrically frustrated spin-chain system, Ca3Co1.4Rh0.6O6, in the single crystalline form for different orientations. The results bring out that the…

Strongly Correlated Electrons · Physics 2015-06-22 Tathamay Basu , Kartik K. Iyer , Kiran Singh , K. Mukherjee , P. L. Paulose , E. V. Sampathkumaran

We report the magnetic, heat-capacity, dielectric and magnetodielectric (MDE) behaviour of a Haldane spin-chain compound containing light rare-earth ion, Nd2BaNiO5, in detail, as a function of temperature (T) and magnetic field (H) down to…

Materials Science · Physics 2015-03-12 Tathamay Basu , Niharika Mohapatra , Kiran Singh , E. V. Sampathkumaran

By combining single crystal x-ray and neutron diffraction, and the magnetodielectric measurements on single crystal Fe4Nb2O9, we present the magnetic structure and the symmetry-allowed magnetoelectric coupling in Fe4Nb2O9. It undergoes an…

Strongly Correlated Electrons · Physics 2020-08-12 Lei Ding , Yan Wu , Minseong Lee , Eun Sang Choi , Ryan Sinclair , Haidong Zhou , Bryan C. Chakoumakos , Huibo Cao

The intrinsic noncollinear spin patterns in rare-earth pyrochlore are physically interesting, hosting many emergent properties, e.g. spin ice and monopole-type excitation. Recently, the magnetic monopole excitation of spin ice systems was…

Materials Science · Physics 2015-12-18 Lin Lin , Y. L. Xie , J. -J. Wen , Shuai Dong , Z. B. Yan , J. -M. Liu

We have investigated the magnetoelectric properties of (Ca$_{1-x}$Sr$_{x}$)$_2$CoSi$_2$O$_7$ ($0\leq x\leq 1$) crystals with a quasi-two-dimensional structure. In Ca$_2$CoSi$_2$O$_7$ ($x=0$), a canted antiferromagnetic transition occurs at…

Strongly Correlated Electrons · Physics 2015-05-14 M. Akaki , J. Tozawa , M. Hitomi , D. Akahoshi , H. Kuwahara

The compound, Fe2TiO5 (FTO)is a well-known uniaxial anisotropic spin-glass insulator with two successive glassy freezing temperatures i.e. transverse (TTF= 9K) and longitudinal (TLF= 55 K). In this article, we present the results of…

Materials Science · Physics 2014-10-28 Shivani Sharma , Tathamay Basu , Aga Shahee , K. Singh , N. P. Lalla , E. V. Sampathkumaran

The origin of both the Ising chain magnetism and ferroelectricity in Ca$_3$CoMnO$_6$ is studied by $ab$ $initio$ electronic structure calculations and x-ray absorption spectroscopy. We find that Ca$_3$CoMnO$_6$ has the alternate trigonal…

Materials Science · Physics 2009-01-15 Hua Wu , T. Burnus , Z. Hu , C. Martin , A. Maignan , J. C. Cezar , A. Tanaka , N. B. Brookes , D. I. Khomskii , L. H. Tjeng

We investigate magnetic, thermal, and dielectric properties of SrCuTe2O6, which is isostructural to PbCuTe2O6, a recently found, Cu-based 3D frustrated magnet with a corner sharing triangular spin network having dominant first and second…

Strongly Correlated Electrons · Physics 2016-03-16 B. Koteswararao , S. K. Panda , R. Kumar , Kyongjun Yoo , A. V. Mahajan , I. Dasgupta , B. H. Chen , Kee Hoon Kim , F. C. Chou

The crystal structure of hexagonal-Sr0.6Ba0.4MnO3 allows various competing superexchange interactions, leading to intriguing magnetic properties. Local structural changes modify overlapping between Mn and oxygen ions with temperature.…

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