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We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby $^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 A. Dréau , J. -R. Maze , M. Lesik , J. -F. Roch , V. Jacques

Nuclear magnetic resonance (NMR) imaging with shallow nitrogen-vacancy (NV) centers in diamond offers an exciting route toward sensitive and localized chemical characterization at the nanoscale. Remarkable progress has been made to combat…

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

Chemical Physics · Physics 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

Photonic spin density (PSD) in the near-field gives rise to exotic phenomena such as photonic skyrmions, optical spin-momentum locking and unidirectional topological edge waves. Experimental investigation of these phenomena requires a…

Quantum Physics · Physics 2021-10-04 Farid Kalhor , Li-Ping Yang , Leif Bauer , Zubin Jacob

Nuclear spins in the proximity of electronic spin defects in solids are promising platforms for quantum information processing due to their ability to preserve quantum states for a remarkably long time. Here we report a comprehensive study…

Quantum Physics · Physics 2023-10-03 Mykyta Onizhuk , Giulia Galli

We investigate spin-dependent decay and intersystem crossing in the optical cycle of single negatively-charged nitrogen-vacancy (NV) centres in diamond. We use spin control and pulsed optical excitation to extract both the spin-resolved…

Quantum Physics · Physics 2011-02-25 Lucio Robledo , Hannes Bernien , Toeno van der Sar , Ronald Hanson

Nitrogen vacancy (NV) color centers in diamond are a leading modality for both superresolution optical imaging and nanoscale magnetic field sensing. In this work, we solve the remaining key challenge of performing optical magnetic imaging…

We present a new magnetometry method integrating an ensemble of nitrogen-vacancy (NV) centers in a single-crystal diamond with an extended dynamic range for monitoring the fast changing magnetic-field. The NV-center spin resonance frequency…

Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…

Dephasing and relaxation of the nuclear spins coupled to the nitrogen-vacancy (NV) center during optical initialization and readout is an important issue for various applications of this hybrid quantum register. Here we present both an…

Quantum Physics · Physics 2016-07-15 Ping Wang , Wen Yang

Nitrogen-vacancy centers possessing nuclear spins are promising candidates for a novel nuclear spin gyroscope. Preparation of a nuclear spin state is a crucial step to implement a sensor that utilizes a nuclear spin. In a low magnetic…

Symmetry considerations are used in presenting a model of the electronic structure and the associated dynamics of the nitrogen-vacancy center in diamond. The model accounts for the occurrence of optically induced spin polarization, for the…

Materials Science · Physics 2013-05-29 N. B. Manson , J. P. Harrison , M. J. Sellars

The nitrogen-vacancy center in diamond attracts a lot of attention in sensing applications, mainly for temperature, magnetic field, and rotation measurements. Nuclear spins of carbon-13 surrounding the nitrogen-vacancy center can be used as…

We report measurements of optically detected magnetic resonance spectra of ensembles of negatively charged nitrogen-vacancy (NV) centers in diamonds in the presence of strain and DC external electric fields. The Stark shift of the spectral…

Atomic Physics · Physics 2018-02-27 Sarvagya Sharma , Chris Hovde , Douglas H. Beck , Fahad Alghannam

Hyper-polarization of nuclear spins is crucial for advancing nuclear magnetic resonance (NMR) and quantum information technologies, as nuclear spins typically exhibit extremely low polarization at room temperature due to their small…

Quantum Physics · Physics 2025-05-20 Haiyang Li , Hao Liao , Ping Wang

Chemical sensors with high sensitivity that can be used in extreme conditions and can be miniaturized are of high interest in science and industry. The Nitrogen-vacancy (NV) center in diamond is an ideal candidate as a nanosensor due to the…

Quantum Physics · Physics 2021-02-16 Hossein T. Dinani , Enrique Muñoz , Jeronimo R. Maze

In this work we investigated the time behavior of the polarization of bulk 13C nuclei in diamond above the thermal equilibrium. This nonthermal nuclear hyperpolarization is achieved by cross relaxation between two nitrogen related…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 Ralf Wunderlich , Jonas Kohlrautz , Bernd Abel , Jürgen Haase , Jan Meijer

The electronic spins of the nitrogen-vacancy centers (NV centers) in Chemical-Vapor-Deposition (CVD) grown diamonds form ideal probes of magnetic fields and temperature, as well as promising qu-bits for quantum information processing.…

Quantum Physics · Physics 2021-03-31 C. Pellet-Mary , P. Huillery , M. Perdriat , A. Tallaire , G. Hétet

The nitrogen-vacancy (NV) center in diamond is of high importance in quantum information processing applications which relies on the efficient optical polarization of its electron spin. However, the full optical spinpolarization process, in…

Quantum Physics · Physics 2018-09-12 Gergő Thiering , Adam Gali

Using pulsed photoionization the coherent spin manipulation and echo formation of ensembles of NV- centers in diamond are detected electrically realizing contrasts of up to 17 %. The underlying spin-dependent ionization dynamics are…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Florian M. Hrubesch , Georg Braunbeck , Martin Stutzmann , Friedemann Reinhard , Martin S. Brandt
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