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We report a study of high-resolution microwave spectroscopy of nitrogen-vacancy centers in diamond crystals at and around zero magnetic field. We observe characteristic splitting and transition imbalance of the hyperfine transitions, which…

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

The ability to perform nanoscale electric field imaging of elementary charges at ambient temperatures will have diverse interdisciplinary applications. While the nitrogen-vacancy (NV) center in diamond is capable of high-sensitivity…

Mesoscale and Nanoscale Physics · Physics 2021-04-28 M. S. J Barson , L. M. Oberg , L. P. McGuinness , A. Denisenko , N. B. Manson , J. Wrachtrup , M. W. Doherty

We demonstrate preferential orientation of nitrogen-vacancy (NV) color centers along two of four possible crystallographic axes in diamonds grown by chemical vapor deposition on the {100} face. We identify the relevant growth regime and…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 L. M. Pham , N. Bar-Gill , D. Le Sage , A. Stacey , M. Markham , D. J. Twitchen , M. D. Lukin , R. L. Walsworth

We investigate spin and optical properties of individual nitrogen-vacancy centers located within 1-10 nm from the diamond surface. We observe stable defects with a characteristic optically detected magnetic resonance spectrum down to lowest…

Mesoscale and Nanoscale Physics · Physics 2012-08-27 B. K. Ofori-Okai , S. Pezzagna , K. Chang , M. Loretz , R. Schirhagl , Y. Tao , B. A. Moores , K. Groot-Berning , J. Meijer , C. L. Degen

Dynamical polarization of nuclear spin ensembles is of central importance for magnetic resonance studies, precision sensing and for applications in quantum information theory. Here we propose a scheme to generate long-lived singlet pairs in…

Quantum Physics · Physics 2017-04-06 Johannes N. Greiner , D. D. Bhaktavatsala Rao , Jörg Wrachtrup

The Nitrogen-Vacancy (NV) center in diamond has attractive properties for a number of quantum technologies that rely on the spin angular momentum of the electron and the nuclei adjacent to the center. The nucleus with the strongest…

Quantum Physics · Physics 2016-10-17 K. Rama Koteswara Rao , Dieter Suter

We give instructions for the construction and operation of a simple apparatus for performing optically detected magnetic resonance measurements on diamond samples containing high concentrations of nitrogen-vacancy (NV) centers. Each NV…

Mesoscale and Nanoscale Physics · Physics 2018-03-14 Haimei Zhang , Carina Belvin , Wanyi Li , Jennifer Wang , Julia Wainwright , Robbie Berg , Joshua Bridger

Dynamic Nuclear Polarization (DNP) presently stands as the preferred strategy to enhance the sensitivity of nuclear magnetic resonance measurements, but its application relies on the use of high-frequency microwave to manipulate electron…

Mesoscale and Nanoscale Physics · Physics 2022-02-02 Carlos A. Meriles , Pablo R. Zangara

Knowledge of the nitrogen-vacancy center formation kinetics in diamond is critical to engineering sensors and quantum information devices based on this defect. Here we utilize the longitudinal tracking of single NV centers to elucidate NV…

We determine and analyze the charge and spin density distributions of nitrogen-vacancy (N-V) center in diamond for both the ground and excited states by \emph{ab initio} supercell calculations. We show that the hyperfine tensor of $^{15}$N…

Materials Science · Physics 2009-05-11 Adam Gali

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

Sensing single nuclear spins is a central challenge in magnetic resonance based imaging techniques. Although different methods and especially diamond defect based sensing and imaging techniques in principle have shown sufficient…

We demonstrate vector magnetometry with an ensemble of nitrogen-vacancy (NV) centers in diamond without the need for an external bias field. The anisotropy of the electric dipole moments of the NV center reduces the ambiguity of the…

Mesoscale and Nanoscale Physics · Physics 2017-01-05 Franz Münzhuber , Johannes Kleinlein , Tobias Kiessling , Laurens W. Molenkamp

The nitrogen-vacancy (NV) center in diamond is a heavily studied defect due to its potential applications to quantum metrology and computation, particularly in ambient conditions. The key mechanism to using the NV in any application lies in…

Quantum Physics · Physics 2023-05-03 Liam Hanlon , Michael Olney-Fraser , Lukas Razinkovas , Marcus W. Dohert

The negatively charged nitrogen-vacancy (NV$^-$) center in diamond is a model quantum system for university teaching labs due to its room-temperature compatibility and cost-effective operation. Based on the low-cost experimental setup that…

Nuclear spins in solids exhibit long coherence times due to the small nuclear gyromagnetic ratio. This weak environmental coupling comes at the expense of slow quantum gate operations, which should be as fast as possible for many…

Quantum Physics · Physics 2022-11-11 R. M. Goldblatt , A. M. Martin , A. A. Wood

Bulk 13C polarization can be strongly enhanced in diamond at room-temperature based on the optical pumping of nitrogen-vacancy color centers. This effect was confirmed by irradiating suitably aligned single-crystals at a ~50 mT field…

By applying a new technique for dynamic nuclear polarization involving simultaneous excitation of electronic and nuclear transitions, we have enhanced the nuclear polarization of the nitrogen nuclei in 15N@C60 by a factor of 1000 at a fixed…

Generation of local magnetic field at the nanoscale is desired for many applications such as spin-qubit-based quantum memories. However, this is a challenge due to the slow decay of static magnetic fields. Here, we demonstrate photonic spin…

Quantum Physics · Physics 2022-07-13 Farid Kalhor , Noah F. Opondo , Shoaib Mahmud , Leif Bauer , Li-Ping Yang , Sunil A. Bhave , Zubin Jacob
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