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The insulating ferrimagnet Cu2OSeO3 shows a rich variety of phases such as skyrmion lattice and helical magnetism controlled by interplay of different exchange interactions which can be tuned by external pressure. In this work we have…

The formation and characteristics of magnetic skyrmions are strongly governed by the symmetry of the underlying crystal structure. In this study, we report the discovery of a new trigonal polymorph of Cu2OSeO3, observed exclusively in…

Materials Science · Physics 2025-09-18 Alla Arakcheeva , Priya Ranjan Baral , Wen Hua Bi , Christian Jandl , Oleg Janson , Arnaud Magrez

We report the observation of the skyrmion lattice in the chiral multiferroic insulator Cu2OSeO3 using Cu L3-edge resonant soft x-ray diffraction. We observe the unexpected existence of two distinct skyrmion sublattices that arise from…

Strongly Correlated Electrons · Physics 2015-06-18 M. C. Langner , S. Roy , S. K. Mishra , J. C. T. Lee , X. W. Shi , M. A. Hossain , Y. -D. Chuang , S. Seki , Y. Tokura , S. D. Kevan , R. W. Schoenlein

Magnetic materials can host skyrmions, which are topologically non-trivial spin textures. In chiral magnets with cubic lattice symmetry, all previously-observed skyrmion phases require thermal fluctuations to become thermodynamically stable…

Strongly Correlated Electrons · Physics 2021-04-06 A. Chacon , L. Heinen , M. Halder , A. Bauer , W. Simeth , S. Mühlbauer , H. Berger , M. Garst , A. Rosch , C. Pfleiderer

The effects of high pressure on the crystal structure of orthorhombic (Pnma) perovskite type cerium scandate have been studied in situ under high pressure by means of synchrotron x-ray powder diffraction, using a diamond anvil cell. We have…

Insulating helimagnetic Cu2OSeO3 shows sizeable magnetoelectric effects in its skyrmion phase. Using magnetization measurements, magneto-current analysis and dielectric spectroscopy, we provide a thorough investigation of magnetoelectric…

Strongly Correlated Electrons · Physics 2015-11-05 E. Ruff , P. Lunkenheimer , A. Loidl , H. Berger , S. Krohns

We report the single-crystal X-ray analysis and magnetic properties of a new double-layered perovskite antiferromagnet, Cs$_3$Cu$_2$Cl$_4$Br$_3$. This structure is composed of Cu$_2$Cl$_4$Br$_3$ double layers with elongated CuCl$_4$Br$_2$…

Strongly Correlated Electrons · Physics 2015-06-25 F. Yamada , T. Ono , H. Tanaka , J. Yamaura

Topological spin textures such as skyrmions hold high potential for use as magnetically active elements in diverse near-future applications. While skyrmions in metallic multilayers attract great attention in this context, unleashing the…

The lack of inversion symmetry in the crystal lattice of magnetic materials gives rise to complex non-collinear spin orders through interactions of relativistic nature, resulting in interesting physical phenomena, such as emergent…

In this work we explore the overall structural behaviour of the [(CH3)2NH2][Mn(HCOO)3] multiferroic compound across the temperature range where its ferroelectric transition takes place by means of calorimetry, thermal expansion measurements…

A skyrmion state in a non-centrosymmetric helimagnet displays topologically protected spin textures with profound technological implications for high density information storage, ultrafast spintronics, and effective microwave devices.…

The high pressure structural properties of bismuth oxide Bi2SiO5 have been investigated up to 28 GPa using in situ powder synchrotron X-ray diffraction and up to 50 GPa with DFT calculations. The monoclinic structure is found to persist up…

Small angle neutron scattering experiments were performed on a bulk single crystal of chiral-lattice multiferroic insulator Cu$_2$OSeO$_3$. In the absence of an external magnetic field, helical spin order with magnetic modulation vector $q…

Strongly Correlated Electrons · Physics 2012-06-25 S. Seki , J. -H. Kim , D. S. Inosov , R. Georgii , B. Keimer , S. Ishiwata , Y. Tokura

Spin density waves, based on modulated local moments, are usually associated with metallic materials, but have recently been reported in insulators which display coupled magnetic and structural order parameters. We discuss one such example,…

Materials Science · Physics 2020-07-30 N. Giles-Donovan , N. Qureshi , R. D. Johnson , L. Y. Zhang , S. -W. Cheong , S. Cochran , C. Stock

The bulk helimagnet Cu2OSeO3 represents a unique example in the family of B20 cubic helimagnets exhibiting a tilted spiral and skyrmion phase at low temperatures when the magnetic field is applied along the easy <001> crystallographic…

Materials Science · Physics 2023-07-20 M. Crisanti , A. O. Leonov , R. Cubitt , A. Labh , H. Wilhelm , Marcus P. Schmidt , C. Pappas

BaFe2Se3 (Pnma, CsAg2I3-type structure), recently assumed to show superconductivity at ~ 11 K, exhibits a pressure-dependent structural transition to the CsCu2Cl3-type structure (Cmcm space group) around 60 kbar, as evidenced from…

The structural transformation of multiferroic EuTiO$_3$ has been intensively investigated by synchrotron x-ray diffraction at pressures up to 50.3 GPa and temperatures from 50 to 500 K. An antiferrodistortive phase transition from cubic…

Materials Science · Physics 2015-08-12 P. Parisiades , E. Liarokapis , J. Köhler , A. Bussmann-Holder , M. Mezouar

The strongly correlated cuprate Cu$_2$OSeO$_3$ has recently been identified as the first insulating system exhibiting a skyrmion lattice phase. Using a microscopic multi-boson theory for its magnetic ground state and excitations, we…

Strongly Correlated Electrons · Physics 2014-11-05 Judit Romhányi , Jeroen van den Brink , Ioannis Rousochatzakis

We present a detailed study of the phase diagram surrounding the skyrmion lattice (SkL) phase of Cu2OSe2O3 using high-precision magnetic ac susceptibility measurements. An extensive investigation of transition dynamics around the SkL phase…

Strongly Correlated Electrons · Physics 2015-06-23 I. Levatić , V. Šurija , H. Berger , I. Živković

This article reports the experimentally clarified crystal structure of a recently discovered sulfur hydride in high temperature superconducting phase which has the highest critical temperature Tc over 200 K which has been ever reported. For…

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