Related papers: Resonant collisional shielding of reactive molecul…
Proposals for quantum computing using rotational states of polar molecules as qubits have previously considered only diatomic molecules. For these the Stark effect is second-order, so a sizable external electric field is required to produce…
Combining the measured binding energies of four of the most weakly bound rovibrational levels of the $^{87}$Rb$_2$ molecule with the results of two other recent high-precision rubidium experiments, we obtain exceptionally strong constraints…
The Rb-NH interaction is investigated as a prototype for interactions between alkali metal atoms and stable molecules. For spin-aligned Rb and NH that interact on a quartet surface ($^4A''$), the interaction is relatively weak, with a well…
We propose to use a new platform - ultracold polar molecules - for quantum computing with switchable interactions. The on/off switch is accomplished by selective excitation of one of the "0" or "1" qubits - long-lived molecular states - to…
Resonant electric dipole-dipole interactions between cold Rydberg atoms were observed using microwave spectroscopy. Laser-cooled Rb atoms in a magneto-optical trap were optically excited to 45d Rydberg states using a pulsed laser. A…
The interaction between free electrons and laser-induced near-fields provides a platform to study ultrafast processes and quantum phenomena while enabling precise manipulation of electron wavefunctions through linear and orbital momentum…
We study collisions of ultracold CaF molecules in strong static electric fields. These fields allow the creation of long-range barriers in the interaction potential, effectively preventing the molecules from reaching the short-range region…
Quantum computation (QC) and simulation rely on long-lived qubits with controllable interactions. Early work in quantum computing made use of molecules because of their readily available intramolecular nuclear spin coupling and chemical…
We have measured a p-wave Feshbach resonance in a single-component, ultracold Fermi gas of potassium atoms. We have used this resonance to enhance the normally suppressed p-wave collision cross-section to values larger than the background…
Quantum gases of ultracold polar molecules have novel properties because of the strong dipolar forces between molecules. Current experiments shield the molecules from destructive collisions by engineering long-range repulsive interactions…
The presence of electric or microwave fields can modify the long-range forces between ultracold dipolar molecules in such a way as to engineer weakly-bound states of molecule pairs. These so-called field-linked states [Avdeenkov et al.,…
We study polar molecule scattering in quasi-one-dimensional geometries. Elastic and reactive collision rates are computed as a function of collision energy and electric dipole moment for different confinement strengths. The numerical…
A novel atom-molecule conversion technique has been investigated. Ultracold 85Rb atoms sitting in a DC magnetic field near the 155G Feshbach resonance are associated by applying a small sinusoidal oscillation to the magnetic field. There is…
We explore the quantum dynamics of heteronuclear atomic collisions in waveguides and demonstrate the existence of a novel mechanism for the resonant formation of polar molecules. The molecular formation probabilities can be tuned by…
Ultracold dipolar molecules hold great promise for the creation of novel quantum states of matter, but the realization of long-lived molecular bulk samples with strong dipole-dipole interactions has remained elusive. Here, we realize a…
Tunable scattering resonances are crucial for controlling atomic and molecular systems. However, their use has so far been limited to ultracold temperatures. These conditions remain hard to achieve for most hybrid trapped ion-atom systems…
A general variational approach for computing the rovibrational dynamics of polyatomic molecules in the presence of external electric fields is presented. Highly accurate, full-dimensional variational calculations provide a basis of…
We theoretically explore the effect of a transverse electric field on the frictional response of a bi-layer of packed zwitterionic molecules. The dipole-moment reorientation promoted by the electric field can lead to either stick-slip or…
Compared to purely atomic collisions, ultracold collisions involving molecules have the potential to support a much larger number of Fano-Feshbach resonances due to the huge amount of ro-vibrational states available. In order to handle such…
Ultracold ground state dipolar 40K-87Rb molecules have recently been produced in a loose harmonic trap by employing a magnetic field sweep across a Feshbach resonance followed by stimulated Raman adiabatic passage [K.-K. Ni et al., Science…