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Exciton spectroscopy serves as a sensitive probe of electronic states in two-dimensional semiconductors. A prominent feature in optical spectra is the trion peak arising from the binding of a charge carrier to an exciton. The splitting…

Mesoscale and Nanoscale Physics · Physics 2025-07-23 Arthur Christianen , Atac Imamoglu

Hyperspectral imaging at cryogenic temperatures is used to investigate exciton and trion propagation in MoSe$_2$ monolayers encapsulated with hexagonal boron nitride (hBN). Under a tightly focused, continuous-wave laser excitation, the…

Two-dimensional electron-hole gases in colloidal semiconductors have a wide variety of applications. Therefore, a proper physical understanding of these materials is of great importance. In this paper we present a detailed theoretical…

Mesoscale and Nanoscale Physics · Physics 2019-12-18 F. García Flórez , Aditya Kulkarni , Laurens D. A. Siebbeles , H. T. C. Stoof

Excitonic effects due to the correlation of electrons and holes in excited states of matter dominate the optical spectra of many interesting materials. They are usually studied in the long-wavelength limit. Here we investigate excitons at…

Materials Science · Physics 2023-04-18 Vitaly Gorelov , Lucia Reining , Matteo Gatti

Tightly bound excitons in monolayer semiconductors represent a versatile platform to study two-dimensional propagation of neutral quasiparticles. Their intrinsic properties, however, can be severely obscured by spatial energy fluctuations…

Interactions among a collection of particles generate many-body effects in solids resulting in striking modifications of material properties. The heavy carrier mass that yields strong interactions and gate control of carrier density over a…

Metal monochalcogenide GaSe is a classic layered semiconductor that has received increasing research interest due to its highly tunable electronic and optical properties for ultrathin electronics applications. Despite intense research…

Materials Science · Physics 2024-05-14 Fanhao Jia , Zhao Tang , Greis J. Cruz , Weiwei Gao , Shaowen Xu , Wei Ren , Peihong Zhang

Semiconducting transition metal dichalcogenides (TMDs), such as MoSe$_2$ and WSe$_2$, exhibit unique optical and electronic properties. Vertical stacking of layers of one or more TMDs, to create heterostructures, has expanded the fields of…

Two-dimensional excitons formed in quantum materials such as monolayer transition-metal dichalcogenides and their strong light-matter interaction have attracted unrivalled attention by the research community due to their extraordinarily…

Mesoscale and Nanoscale Physics · Physics 2018-12-31 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

We analyze the lineshape of the quasiparticle photoluminescence of monolayer and bilayer molybdenum ditelluride in temperature- and excitation intensity-dependent experiments. We confirm the existence of a negatively charged trion in the…

Excitonic band structure is critical for investigating exciton dynamics. Theoretically, quantum effects from exchange scattering between electron-hole pairs significantly modulate exciton dispersion. Here, we report the direct observation…

Strongly Correlated Electrons · Physics 2026-03-25 Zhibin Su , Junjian Mi , Shaohua Yan , Jiade Li , Siwei Xue , Zhiyu Tao , Enling Wang , Xiongfei Shi , Hechang Lei , Zhuan Xu , Jiandong Guo , Xuetao Zhu

Control of the band-edge offsets at heterojunctions between organic semiconductors allows efficient operation of either photovoltaic or light-emitting diodes. We investigate systems where the exciton is marginally stable against charge…

Soft Condensed Matter · Physics 2013-09-27 Arne C. Morteani , Paiboon Sreearunothai , Laura M. Herz , Richard H. Friend , Carlos Silva

Strong Coulomb interactions in low-dimensional quantum materials give rise to emergent bound states such as excitons and trions, which play a central role in correlated electronic phases. In quasi-one-dimensional systems, equilibrium…

Significant excitonic effects were observed in graphene by measuring its optical conductivity in a broad spectral range including the two-dimensional {\pi}-band saddle-point singularities in the electronic structure. The strong…

Materials Science · Physics 2015-05-20 Kin Fai Mak , Jie Shan , Tony F. Heinz

The interplay of optics, dynamics and transport is crucial for the design of novel optoelectronic devices, such as photodetectors and solar cells. In this context, transition metal dichalcogenides (TMDs) have received much attention. Here,…

Mesoscale and Nanoscale Physics · Physics 2019-11-04 Raul Perea-Causin , Samuel Brem , Roberto Rosati , Roland Jago , Marvin Kulig , Jonas D. Ziegler , Jonas Zipfel , Alexey Chernikov , Ermin Malic

We describe exciton-polariton modes formed by the interaction between excitons in a 2D layer of a transition metal dichalcogenide embedded in a cylindrical microcavity and the microcavity photons. For this, an expression for the excitonic…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 José Nuno S. Gomes , Carlos Trallero-Giner , Nuno M. R. Peres , Mikhail I. Vasilevskiy

Two-dimensional (2D) transition metal dichalcogenides (TMDC) and their moir\'e interfaces have been demonstrated for correlated electron states, including Mott insulators and electron/hole crystals commensurate with moir\'e superlattices.…

Mesoscale and Nanoscale Physics · Physics 2024-01-08 Yusong Bai , Yiliu Li , Song Liu , Yinjie Guo , Jordan Pack , Jue Wang , Cory R. Dean , James Hone , X. -Y. Zhu

In low-dimensional systems with strong electronic correlations, the application of an ultrashort laser pulse often yields novel phases that are otherwise inaccessible. The central challenge in understanding such phenomena is to determine…

We report on the charge dynamics of Ta$_2$Pd$_3$Te$_5$ using temperature-dependent optical spectroscopy with polarized light. We observe a metal-insulator transition characterized by the collapse of Drude response and the emergence of sharp…

The transition metal chalcogenide Ta$_2$NiSe$_5$ undergoes a second-order phase transition at $T_c=328$ K involving a small lattice distortion. Below $T_c$, a band gap at the center of its Brillouin zone increases up to about 0.35 eV. In…

Strongly Correlated Electrons · Physics 2020-08-07 C. Monney , M. Herzog , A. Pulkkinen , Y. Huang , J. Pelliciari , P. Olalde-Velasco , N. Katayama , M. Nohara , H. Takagi , T. Schmitt , T. Mizokawa