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The properties of excitons in semiconducting single-walled carbon nanotubes (SWCNTs), isolated in vacuum or a medium, and their contributions to the optical spectra of nanotubes are studied within the elementary potential model, in which an…

Materials Science · Physics 2010-12-15 Oleksii A. Smyrnov

The spectrum of large radius exciton in an individual semiconducting single-walled carbon nanotube (SWCNT) is described within the framework of elementary potential model, in which exciton is modeled as bound state of two oppositely charged…

Other Condensed Matter · Physics 2010-11-18 Vadym M. Adamyan , Oleksii A. Smyrnov

The functionalization of single-walled carbon nanotubes (SWCNTs) with luminescent sp$^{3}$ defects has greatly improved their performance in applications such as quantum light sources and bioimaging. Here, we report the covalent…

Theory predicts peculiar features for excited-state dynamics in one dimension (1D) that are difficult to be observed experimentally. Single-walled carbon nanotubes (SWNTs) are an excellent approximation to 1D quantum confinement, due to…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Giancarlo Soavi , Francesco Scotognella , Daniele Viola , Timo Hefner , Tobias Hertel , Giulio Cerullo , Guglielmo Lanzani

Quantum confinement significantly influences the excited states of sub-10 nm single-walled carbon nanotubes (SWCNTs), crucial for advancements in transistor technology and the development of novel opto-electronic materials such as…

Mesoscale and Nanoscale Physics · Physics 2024-10-30 Benjamin Eller , Charles W. Clark , YuHuang Wang

We present evidence of all optical trion generation and emission in undoped single walled carbon nanotubes (SWCNTs). Luminescence spectra, recorded on individual SWCNTs over a large CW excitation intensity range, show trion emission peaks…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Silvia Santos , Bertrand Yuma , Stéphane Berciaud , Jonah Shaver , Mathieu Gallart , Pierre Gilliot , Laurent Cognet , Brahim Lounis

The ground-state exciton binding energy for single-walled carbon nanotubes (SWCNTs) in vacuum calculated ignoring the screening of Coulomb interaction appears to be much greater than the corresponding band gap. The most essential…

Other Condensed Matter · Physics 2010-11-18 Vadym M. Adamyan , Oleksii A. Smyrnov , Sergey V. Tishchenko

Doping substantially influences the electronic and photophysical properties of semiconducting single-wall carbon nanotubes (s-SWNTs). Although prior studies have noted that surplus charge carriers modify optical spectra and accelerate…

Materials Science · Physics 2023-07-19 Klaus H. Eckstein , Pascal Kunkel , Markus Voelckel , Friedrich Schöppler , Tobias Hertel

We studied the nonlinear time-resolved luminescence signals due to multiexciton recombination processes in single-walled carbon nanotubes (SWNTs) using femtosecond excitation correlation (FEC) spectroscopy. From theoretical analysis of the…

Materials Science · Physics 2015-05-13 Yuhei Miyauchi , Kazunari Matsuda , Yoshihiko Kanemitsu

We predict properties of triplet excited states in single-walled carbon nanotubes (CNTs) using a time-dependent density-functional theory (TD-DFT). We show that the lowest triplet state energy in CNTs to be about 0.2-0.3 eV lower than the…

Materials Science · Physics 2015-06-25 Sergei Tretiak

We have investigated excitons in highly-aligned single-walled carbon nanotubes (SWCNTs) through optical spectroscopy at low temperature (1.5 K) and high magnetic fields ($\textbf{\textit{B}}$) up to 55 T. SWCNT/polyacrylic acid films were…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Shaver , S. A. Crooker , J. A. Fagan , E. K. Hobbie , N. Ubrig , O. Portugall , V. Perebeinos , Ph. Avouris , J. Kono

We show that the energy differences between the lowest optical singlet exciton and the lowest triplet exciton in semiconducting single-walled carbon nanotubes with diameter $\sim 1$ nm and graphene nanoribbons with widths $\sim 2$ nm are an…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 K. Aryanpour , Sumit Mazumdar , Hongbo Zhao

We investigate the lowest many-body excited states in carbon nanotubes by means of ab initio calculations. On the basis of these calculations and an additional theoretical analysis of the excitons, we demonstrate that the splitting between…

Materials Science · Physics 2007-05-23 Eric Chang , Deborah Prezzi , Alice Ruini , Elisa Molinari

We study quantum optical properties of the single-walled carbon nanotube (SWCNT) by introducing the effective interaction between the quantized electromagnetic field and the confined electrons in the SWCNT. Our purpose is to explore the…

Mesoscale and Nanoscale Physics · Physics 2009-04-30 Z. L. Guo , Z. R. Gong , C. P. Sun

An artifcial two-atomic molecule, also called a double quantum dot (DQD), is an ideal system for exploring few electron physics. Spin-entanglement between just two electrons can be explored in such systems where singlet and triplet states…

Mesoscale and Nanoscale Physics · Physics 2008-12-22 H. Ingerslev Jørgensen , K. Grove-Rasmussen , K. -Y. Wang , A. M. Blackburn , K. Flensberg , P. E. Lindelof , D. A. Williams

Optical properties of single-wall carbon nanotubes (SWCNTs) for light polarized parallel to the nanotube axis have been extensively studied, whereas their response to light polarized perpendicular to the nanotube axis has not been well…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Fumiya Katsutani , Weilu Gao , Xinwei Li , Yota Ichinose , Yohei Yomogida , Kazuhiro Yanagi , Junichiro Kono

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

Materials Science · Physics 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

It is strong Coulomb effects in carbon nanotubes that lead to formation of the so-called "bright" and "dark" (forbidden one-photon optical transition) exciton states, and dramatically decrease the efficiency of one-photon light emission via…

Quantum Physics · Physics 2009-02-09 Nikolai G. Kalugin , Yuri V. Rostovtsev

Single-walled carbon nanotubes (SWCNTs) are promising absorbers and emitters to enable novel photonic and optoelectronic applications but are also known to severely suffer from low optical quantum yields. Here we demonstrate SWCNTs excitons…

Mesoscale and Nanoscale Physics · Physics 2017-12-20 Yue Luo , Ehsaneh D. Ahmadi , Kamran Shayan , Yichen Ma , Kevin S. Mistry , Changjian Zhang , James Hone , Jeffrey L. Blackburn , Stefan Strauf

We report the direct observation of the spin-singlet dark excitonic state in individual single-walled carbon nanotubes through low-temperature micro-photoluminescence spectroscopy in magnetic fields. A magnetic field up to 5 T, applied…

Mesoscale and Nanoscale Physics · Physics 2008-08-22 A. Srivastava , H. Htoon , V. I. Klimov , J. Kono
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