Related papers: Table-top Nonlinear Extreme Ultraviolet Spectrosco…
High-harmonic generation (HHG) provides the only source of attosecond pulses -- currently the shortest accessible time intervals, and it is employed as the only table-top source of light in extreme UV and soft X-ray spectral regions. Chiral…
Understanding the mechanisms and spatial correlations of crystallographic symmetry breaking in ferroelectric materials is essential to tuning their functional properties. While optical second harmonic generation (SHG) has long been utilized…
Since the first observation of second harmonic generation (SHG), there have been extensive studies on this nonlinear phenomenon not only to clarify its physical origin but also to realize unconventional functionalities. Nonetheless, a…
High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…
Relativistic electrons are prodigious sources of photons. Beyond classical accelerators, ultra-intense laser interactions are of particular interest as they allow the coherent motion of relativistic electrons to be controlled and exploited…
Achieving compact and efficient visible laser sources is crucial for a wide range of applications. However traditional semiconductor laser technology faces difficulties in producing high-brightness green light, leaving a green gap in…
Experimental insight into the elementary processes underlying charge transfer across interfaces has blossomed with the wide-spread availability of ultra-high vacuum set-ups that allow the preparation and characterization of solid surfaces…
The goal to control short-wavelength radiation for the investigation and manipulation of ultrafast dynamics in quantum systems coevolves with the growing availability of extreme-ultraviolet (XUV) and x-ray sources from high-harmonic…
High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…
We present spatial coherence measurements of extreme-ultraviolet light generated using the process of high-harmonic upconversion of a femtosecond laser. Using a phase-matched hollow-fiber geometry, the generated beam is found to exhibit…
Free-electron lasers (FEL) in the extreme ultraviolet (XUV) and X-ray regime opened up the possibility for experiments at high power densities, in particular allowing for fluence-dependent absorption and scattering experiments to reveal…
Full coherent soft X-ray attosecond pulses are now available through high-order harmonic generation (HHG); however, its insufficient output energy hinders various applications, such as attosecond-scale soft X-ray nonlinear experiments, the…
We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…
Extreme ultraviolet (EUV) coherent sources below 120nm are of paramount significance for promoting next-generation nano-scale lithography,precision spectroscopy, and exploring the emerging physical phenomena in quantum materials. Nonlinear…
Together with one of its variants, the recently proposed phase-merging enhanced harmonic generation (PEHG) free-electron lasers (FELs) have been systematically studied in this paper. Different form the standard-HGHG, a transverse gradient…
Measurements of the phase of two-photon matrix elements are presented for resonant and antiresonant two-color ionization of helium. A tunable, narrow-bandwidth, near-infrared (NIR) laser source is used for extreme ultra-violet (XUV)…
A setup of a unique x-ray source is put forward employing a relativistic electron beam interacting with two counter-propagating laser pulses in the nonlinear few-photon regime. In contrast to Compton scattering sources, the envisaged x-ray…
We introduce a machine-learning-based approach to enhance the sensitivity of optical-extreme ultraviolet (XUV) transient absorption spectroscopy. A reference spectrum is used as input to a three-layer feed-forward neural network, allowing…
Raman spectroscopy and Second Harmonic Generation (SHG) are complementary, non-destructive techniques that provide rich and distinct insights into the structural and electronic properties of materials. Raman spectroscopy offers detailed…
High-repetition-rate, fully coherent extreme-ultraviolet (EUV) and X-ray free-electron lasers (FELs) are essential for advanced time-resolved ultrafast spectroscopies. While external seeding serves as the standard technique to achieve…