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Related papers: Establishing non-thermal regimes in pump-probe ele…

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The interaction of light with a material's electronic system creates an out-of-equilibrium (non-thermal) distribution of optically excited electrons. Non-equilibrium dynamics relaxes this distribution on an ultrafast timescale to a hot…

Strongly Correlated Electrons · Physics 2014-03-05 Søren Ulstrup , Jens Christian Johannsen , Marco Grioni , Philip Hofmann

In complex materials various interactions play important roles in determining the material properties. Angle Resolved Photoelectron Spectroscopy (ARPES) has been used to study these processes by resolving the complex single particle self…

Time- and angle-resolved photoemission spectroscopy (tr-ARPES) constitutes a powerful tool to inspect the dynamics and thermalization of hot carriers. The identification of the processes that drive the dynamics, however, is challenging even…

Materials Science · Physics 2020-01-22 Fabio Caruso , Dino Novko , Claudia Draxl

The electron dynamics in the unoccupied states of the Weyl semimetal PtBi$_2$ is studied by time- and angle-resolved photoemission spectroscopy (TR-ARPES). The measurement's result is the photoemission intensity $I$ as a function of at…

Angle-resolved photoemission spectroscopy (ARPES) -- with its exceptional sensitivity to both the binding energy and momentum of valence electrons in solids -- provides unparalleled insights into the electronic structure of quantum…

Strongly Correlated Electrons · Physics 2024-09-06 Fabio Boschini , Marta Zonno , Andrea Damascelli

We study how time- and angle-resolved photoemission (tr-ARPES) reveals the dynamics of BCS-type, s-wave superconducting systems with time-varying order parameters. Approximate methods are discussed, based on previous approaches to either…

Superconductivity · Physics 2019-01-10 Tianrui Xu , Takahiro Morimoto , Alessandra Lanzara , Joel E. Moore

In pump-probe time and angle-resolved photoemission spectroscopy (TR-ARPES) experiments the presence of the pump pulse adds a new level of complexity to the photoemission process in comparison to conventional ARPES. This is evidenced by…

Time- and angle-resolved photoemission spectroscopy (trARPES) is a powerful spectroscopic method to measure the ultrafast electron dynamics directly in momentum-space. However, band gap materials with exceptional strong Coulomb interaction…

Mesoscale and Nanoscale Physics · Physics 2019-12-09 Dominik Christiansen , Malte Selig , Ermin Malic , Ralph Ernstorfer , Andreas Knorr

Nonequilibrium pump-probe time domain spectroscopies can become an important tool to disentangle degrees of freedom whose coupling leads to broad structures in the frequency domain. Here, using the time-resolved solution of a model…

Real-time probing of electrons can uncover intricate relaxation mechanisms and many-body interactions hidden in strongly correlated materials. While experimenters have used ultrafast optical pump-probe methods in bulk materials, laser…

Mesoscale and Nanoscale Physics · Physics 2024-01-23 H. M. Yoo , M. Korkusinski , D. Miravet , K. W. Baldwin , K. West , L. Pfeiffer , P. Hawrylak , R. C. Ashoori

In the past decade, the advent of time-resolved spectroscopic tools has provided a new ground to explore fundamental interactions in solids and to disentangle degrees of freedom whose coupling leads to broad structures in the frequency…

The simulation of non-equilibrium electron distributions is essential for capturing light-metal interactions and therefore the study of photoabsorption, photocatalysis, laser ablation, and many other phenomena. Current methodologies, such…

Materials Science · Physics 2025-03-13 M. Uehlein , H. T. Snowden , C. Seibel , T. Held , S. T. Weber , R. J. Maurer , B. Rethfeld

The pursuit of a comprehensive understanding of the dynamical nature of intertwined orders in quantum matter has fueled the development of several new experimental techniques, including time- and angle-resolved photoemission spectroscopy…

Superconductivity · Physics 2021-07-21 Marta Zonno , Fabio Boschini , Andrea Damascelli

Angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental technique for directly probing electron dynamics in solids. The energy vs. momentum dispersion relations and the associated spectral broadenings measured by ARPES…

Materials Science · Physics 2010-01-19 Cheol-Hwan Park , Feliciano Giustino , Catalin D. Spataru , Marvin L. Cohen , Steven G. Louie

The present paper is a review of the phenomena related to non-equilibrium electron relaxation in bulk and nano-scale metallic samples. The workable Two-Temperature Model (TTM) based on Boltzmann-Bloch-Peierls (BBP) kinetic equation has been…

Statistical Mechanics · Physics 2009-03-23 Navinder Singh

Relaxation of electrons in a Hubbard model coupled to a dissipative bosonic bath is studied to simulate the pump-probe photoemission measurement. From this insight, we propose an experimental method of eliciting unoccupied part of the…

Strongly Correlated Electrons · Physics 2016-08-15 Youhei Yamaji , Masatoshi Imada

Ultrafast spectroscopies have become an important tool for elucidating the microscopic description and dynamical properties of quantum materials. In particular, by tracking the dynamics of non-thermal electrons, a material's dominant…

Motivated by recent development in time-resolved angle-resolved photoemission spectroscopy (trARPES) for d-wave superconductors, we analyze the non-equilibrium relaxation dynamics of the laser pulse excited sample within the scenario of…

Superconductivity · Physics 2014-03-26 Yong Wang , Fu-Chun Zhang

Angle-resolved photoemission spectroscopy (ARPES) is one of the most direct methods of studying the electronic structure of solids. By measuring the kinetic energy and angular distribution of the electrons photoemitted from a sample…

Strongly Correlated Electrons · Physics 2013-03-07 Riccardo Comin , Andrea Damascelli

Optical pumping of solids creates a non-equilibrium electronic structure where electrons and photons combine to form quasiparticles of dressed electronic states. The resulting shift of electronic levels is known as the optical Stark effect,…

Materials Science · Physics 2016-12-02 Umberto De Giovannini , Hannes Hübener , Angel Rubio
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