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A high power factor and low lattice thermal conductivity are two essential ingredients of highly efficient thermoelectric materials. Although monolayers of transition metal dichalcogenides possess high power factors, high lattice thermal…

Materials Science · Physics 2018-10-02 S. Shahab Naghavi , Jiangang He , Yi Xia , C. Wolverton

When two planar atomic membranes are placed within the van der Waals distance, the charge and heat transport across the interface are coupled by the rules of momentum conservation and structural commensurability, leading to outstanding…

Mesoscale and Nanoscale Physics · Physics 2018-01-08 Phanibhusan S. Mahapatra , Kingshuk Sarkar , H. R. Krishnamurthy , Subroto Mukerjee , Arindam Ghosh

Tin chalcogenides (SnS, SnSe, and SnTe) are found to have improved thermoelectric properties upon the reduction of their dimensionality. Here we found the tilted AA + s stacked two-dimensional (2D) SnTe bilayer as the most stable phase…

Materials Science · Physics 2021-03-10 Abhiyan Pandit , Raad Haleoot , Bothina Hamad

Building two-dimensional (2D) van der Waals (vdW) heterostructures and enhancing their properties through strain engineering unlocks new applications for their constituent materials. In this study, we present a comprehensive…

Materials Science · Physics 2024-10-23 Sarga P K , Karthik H J , Swastibrata Bhattacharyya

Twisted bilayer graphene provides a new two-dimensional platform for studying electron interaction phenomena and flat band properties such as correlated insulator transition, superconductivity and ferromagnetism at certain magic angles.…

Mesoscale and Nanoscale Physics · Physics 2019-07-10 Liheng An , Xiangbin Cai , Meizhen Huang , Zefei Wu , Jiangxiazi Lin , Zhehan Ying , Ziqing Ye , Xuemeng Feng , Ning Wang

We present thermoelectric properties of Be$_2$C monolayer based on density functional theory and semi-classical Boltzmann transport theory. Electronic structure calculations predict this material as a semiconductor with a direct bandgap of…

Materials Science · Physics 2022-01-27 Gautam Sharma , K. C. Bhamu

The electronic and phonon transport properties of graphene-like boron phosphide (BP), boron arsenide (BAs), and boron antimonide (BSb) monolayers are investigated using first-principles calculations and Boltzmann theory. By considering both…

Materials Science · Physics 2019-07-24 Z. Z. Zhou , H. J. Liu , D. D. Fan , G. H. Cao

Besides its predicted promising high electron mobilities at room temperature, PtSe2 bandgap sensitively depends on the number of monolayers combined by van der Waals interaction according to our calculations. We understand this by using…

Materials Science · Physics 2019-05-28 Zhishuo Huang , Wenxu Zhang , Wanli Zhang

In their article, Zhang et al. [Phys. Rev. B 86, 024516 (2012)] present a remarkable result for A$_x$(S)$_y$TiNCl compounds ($\alpha$-phase TiNCl partially intercalated with alkali A and optionally co-intercalated molecular species S),…

Superconductivity · Physics 2015-06-23 Dale R. Harshman , Anthony T. Fiory

Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying a multitude of different quantum ground states. In particular, d$^3$ TMDCs are paradigmatic materials hosting a variety of symmetry broken…

Mesoscale and Nanoscale Physics · Physics 2022-03-10 Somesh Chandra Ganguli , Viliam Vaňo , Shawulienu Kezilebieke , Jose L. Lado , Peter Liljeroth

We predict a new family of robust two-dimensional (2D) topological insulators in van der Waals heterostructures comprising graphene and chalcogenides BiTeX (X=Cl, Br and I). The layered structures of both constituent materials produce a…

Materials Science · Physics 2014-12-25 Liangzhi Kou , Shu-Chun Wu , Claudia Felser , Thomas Frauenheim , Changfeng Chen , Binghai Yan

Low-dimensional layered materials have attracted tremendous attentions due to their wide range of physical and chemical properties and potential applications in electronic devices. Using first-principles method taking into account the…

Materials Science · Physics 2018-08-16 Z. Z. Zhou , H. J. Liu , D. D. Fan , C. Y. Sheng , G. H. Cao

High thermoelectric properties are associated with the phonon-glass electron-crystal paradigm. Conventional wisdom suggests that the optimal bandgap of semiconductor to achieve the largest power factor should be between 6 and 10 kbT. To…

Materials Science · Physics 2024-09-10 Xiaoying Wang , Mengyang Li , Minxuan Feng , Xuejie Li , Yuzhou Hao , Wen Shi , Jiangang He , Xiangdong Ding , Zhibin Gao

We have discovered superconductivity in the two-layer semiconducting monochalcogenide heterostrutures PbTe/PbS, PbTe/PbSe and PbTe/YbS. By comparing data from two-layer samples with data from single monochalcogenide films we conclude that…

Superconductivity at the interface of a heterostructure confined to nanometer-sized scale offers unique opportunities to study the exotic physics of two-dimensional superconductivity. The realization of superconductivity at the interface…

Group-IV monochalcogenides have recently shown great potential for their thermoelectric, ferroelectric, and other intriguing properties. The electrical properties of group-IV monochalcogenides exhibit a strong dependence on the chalcogen…

Using first-principles calculations and Boltzmann theory, we explore the feasibility to maximize the thermoelectric figure of merit (ZT) of topological insulator Bi2Te3 films in the few-quintuple layer regime. We discover that the delicate…

Mesoscale and Nanoscale Physics · Physics 2016-06-09 Jinghua Liang , Long Cheng , Jie Zhang , Huijun Liu , Zhenyu Zhang

One novel family of two-dimensional IV-V compounds have been proposed, whose dynamical stabilities and electronic properties have been systematically investigated using the density functional theory. Extending from our previous work, two…

Materials Science · Physics 2020-10-21 Wanxing Lin , Shi-Dong Liang , Jiesen Li , Dao-Xin Yao

Two-dimensional thermoelectric materials with a figure of merit $ZT$, which is greater than 2.0 at room temperature, would be highly desirable in energy conversion since the efficiency is competitive to conventional energy conversion…

Materials Science · Physics 2019-07-24 Shenghui Zhang , Xiaobin Niu , Yiqun Xie , Kui Gong , Hezhu Shao , Yibin Hu , Yin Wang

Half-Heusler compounds usually exhibit relatively higher lattice thermal conductivity that is undesirable for thermoelectric applications. Here we demonstrate by first-principles calculations and Boltzmann transport theory that the BiBaK…

Materials Science · Physics 2020-08-26 S. H. Han , Z. Z. Zhou , C. Y. Sheng , J. H. Liu , L. Wang , H. M. Yuan , H. J. Liu