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Plasmonic excitations decay within femtoseconds, leaving non-thermal (often referred to as "hot") charge carriers behind that can be injected into molecular structures to trigger chemical reactions that are otherwise out of reach -- a…

Materials Science · Physics 2025-01-28 Jakub Fojt , Paul Erhart , Christian Schäfer

We solve the Maxwell and heat equations self-consistently for metal nanoparticles under intense continuous wave (CW) illumination. Unlike previous studies, we rely on {\em experimentally}-measured data for the metal permittivity for…

Optics · Physics 2016-07-13 Yonatan Sivan , Shi-Wei Chu

Surface plasmon enhanced processes and hot-carrier dynamics in plasmonic nanostructures are of great fundamental interest to reveal light-matter interactions at the nanoscale. Using plasmonic tunnel junctions as a platform supporting both…

The pulsed photothermal phenomenon due to optically absorbed energy, result from non-radiative decay mechanisms, which in nature, these imply the temporal change in the local free energy and thus a temporary change in the local temperature.…

Mesoscale and Nanoscale Physics · Physics 2019-04-04 M. Rodríguez-Matus , C. Garcia-Segundo , Jean-Parick Connerade

Two preceding parts of a paper (cond-mat/0508457, cond-mat/0508460) considered the heuristic values of recent experiments pointing to the nearly universal occurrence of photovoltages across solid surfaces under short-circuit conditions.…

Materials Science · Physics 2007-06-27 O. Ivanov , Eugene Leyarovski , V. Lovchinov , Chr. Popov , M. Kamenova , M. Georgiev

We study the natural excitation of molecular systems, applicable to, for example, photosynthetic light-harvesting complexes, by natural incoherent light. In contrast with the conventional classical models, we show that the light need not…

Chemical Physics · Physics 2022-01-11 Aurélia Chenu , Paul Brumer

The damping of surface plasmons generates hot carriers, which holds promise for photoelectric conversion and photocatalysis. Recent studies have revealed the nonequilibrium characters of the plasmonic hot carriers and their nonadiabatic…

Materials Science · Physics 2025-07-10 Yu Chen , Shengxiang Wu , Shiwu Gao

We theoretically investigate equilibrium behaviors and photothermal effects of a flexible plasmonic metamaterial composed of aramid nanofibers and gold nanoparticles. The fiber matrix is considered as an external field to reconfigure a…

Mesoscale and Nanoscale Physics · Physics 2020-11-12 Anh D. Phan , Vu D. Lam , Katsunori Wakabayashi

We analyze the mathematical model that describes the heat generated by electromagnetic nanoparticles. We use the known optical properties of the nanoparticles to control the support and amount of the heat needed around a nanoparticle.…

Analysis of PDEs · Mathematics 2022-06-10 Arpan Mukherjee , Mourad Sini

Noble-metal nanoparticles for photocatalysis have become a major research object in recent years due to their plasmon-enhanced strong light-matter interaction. The dynamics of the hot electrons in the noble metal are crucial for the…

The optical response of materials based on gold nanoparticle assemblies depends on many parameters regarding both material morphology and light excitation characteristics. In this paper, the interplay between the optical and thermal…

Strong coupling between plasmons and excitons gives rise to new hybrid polariton states with various fields of potential applications. Despite a plethora of research on plasmon--exciton systems, their transient behaviour is not yet fully…

Optics · Physics 2023-06-13 Felix Stete , Matias Bargheer , Wouter Koopman

This paper is devoted to the modelization of the photoacoustic effect generated by the electromagnetic heating of metallic nanoparticles embedded in a biological tissue. We first derive an asymptotic models for the plasmonic resonances and…

Mathematical Physics · Physics 2017-01-24 Faouzi Triki , Margaux Vauthrin

While direct hot-carrier transfer can increase photo-catalytic activity, it is difficult to discern experimentally and competes with several other mechanisms. To shed light on these aspects, here, we model from first principles hot-carrier…

Mesoscale and Nanoscale Physics · Physics 2023-11-20 Jakub Fojt , Tuomas P Rossi , Paul Erhart

Nanoscale electronics and photonics are among the most promising research areas providing functional nano-components for data transfer and signal processing. By adopting metal-based optical antennas as a disruptive technological vehicle, we…

The study of metallic nanoparticles has a long tradition in linear and nonlinear optics [1], with current emphasis on the ultrafast dynamics, size, shape and collective effects in their optical response [2-6]. Nanoparticles also represent…

We show that the scattering interaction between a high energy electron and a photon can be strongly enhanced by different types of localized plasmons in a non-trivial way. The scattering interaction is predicted by an eigen-response theory,…

Optics · Physics 2014-01-21 Kin Hung Fung , Anil Kumar , Nicholas X. Fang

In the article an ultracold electron-ion plasma created by photoionization of cooled atoms is investigated. We obtained analitical expressions for non-ideality parameters which establish due to correlation heating. In the work the nearest…

Plasma Physics · Physics 2011-08-01 Anatoli Gavrilyuk

Molecular aggregates on plasmonic nanoparticles have emerged as attractive systems for the studies of cavity quantum electrodynamics. They are highly tunable, scalable, easy to synthesize and offer sub-wavelength confinement, all while…

A physically transparent unified theory of optically and plasmon induced hot carrier generation in metals is developed with all the relevant mechanisms included. Analytical expressions that estimate the carrier generation rates, their…

Optics · Physics 2019-06-19 Jacob B Khurgin