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Control is exerted over the exciton-polariton physics in metal - Poly(9,9-dioctyl fluorene) - metal microcavities via conformational changes to the polymer backbone. Using thin-film samples containing increasing fractions of $\beta$-phase…

Soft Condensed Matter · Physics 2018-11-21 F. Le Roux , D. D. C. Bradley

The strong-coupling regime between an electronic transition and the photonic mode of a optical resonator manifests itself in the lifting of the degeneracy between the two modes and the creation of two polariton states with mixed optical and…

Mesoscale and Nanoscale Physics · Physics 2016-11-26 Markus Geiser , Giacomo Scalari , Fabrizio Castellano , Mattias Beck , Jérôme Faist

Two-dimensional transition metal dichalcogenides exhibit strong optical transitions with significant potential for optoelectronic devices. In particular they are suited for cavity quantum electrodynamics in which strong coupling leads to…

We have developed a non-Markovian theory of the polariton luminescence taking the molecular vibrations into account. The calculations were made in the polariton basis. We have shown that the frequency shift and the polariton spectral lines…

Mesoscale and Nanoscale Physics · Physics 2022-04-19 B. D. Fainberg , V. Al. Osipov

Organic semiconductors are a promising platform for ambient polaritonics. Several applications, such as polariton routers, and many-body condensed matter phenomena are currently hindered due to the ultra-short polariton lifetimes in…

We present a comprehensive investigation of the light-matter interaction dynamics in two-dimensional materials coupled with a spectrally isolated cavity mode in the strong coupling regime. The interaction between light and matter breaks the…

Mesoscale and Nanoscale Physics · Physics 2023-12-18 Maria Vittoria Gurrieri , Emil V. Denning , Kristian Seegert , Philip T. Kristensen , Jesper Mørk

Halide perovskites, such as methylammonium lead bromide (MAPbBr$_3$), host tightly bound three-dimensional excitons which are robust at room temperature. Excellent optical properties of MAPbBr$_3$ allow for designing of optical single-mode…

We study the elastic response of a stationarily driven system of a cavity field strongly coupled with molecular excitons, taking into account the main dissipation channels due to the finite cavity linewidth and molecular vibrations. We show…

Quantum Physics · Physics 2021-02-24 Kalle S. U. Kansanen , J. Jussi Toppari , Tero T. Heikkilä

Optical nonlinearities are crucial for advanced photonic technologies since they allow photons to be managed by photons. Exciton-polaritons resulting from strong light-matter coupling are hybrid in nature: they combine small mass and high…

In this work, we develop an optomechanical formalism for macroscopic quantum states in exciton-polariton systems with strong exciton-phonon interactions. We show that polariton optomechanical interactions induce dynamical backaction,…

Quantum Gases · Physics 2024-10-31 Vladislav Yu. Shishkov , Evgeny S. Andrianov , Anton V. Zasedatelev

Optical resonators have shown outstanding abilities to tailor chemical landscapes through enhanced light-matter interaction between confined optical modes and molecule vibrations. We propose a theoretical model to study cooperative…

Optics · Physics 2024-12-11 Mingxuan Xiao , Wei Wang , Wenjing Liu , Zheng Li , Shui-Jing Tang , Yun-Feng Xiao

We revisit the exciton mechanism of superconductivity in the framework of microcavity physics, replacing virtual excitons as a binding agent of Cooper pairs by excitations of an exciton-polariton Bose-Einstein condensate. We consider a…

Superconductivity · Physics 2010-04-13 Fabrice P. Laussy , Alexey Kavokin , Ivan Shelykh

We measured the dynamics of polariton parametric stimulated scattering in semiconductor microcavities, by time-resolving the amplified signal with 250 fs resolution. Our experiments demonstrate that the stimulation process is considerably…

Condensed Matter · Physics 2007-05-23 S. Kundermann , M. Saba , C. Ciuti , T. Guillet , JL. Staehli , B. Deveaud

Vibrational polaritons are formed by strong coupling of molecular vibrations and photon modes in an optical cavity. Experiments have demonstrated that vibrational strong coupling can change molecular properties and even affect chemical…

Quantum Physics · Physics 2025-01-14 Thomas Schnappinger , Cyril Falvo , Markus Kowalewski

Following experimental realizations of room temperature polariton lasing with organic molecules, we present a microscopic model that allows us to explore the crossover from weak to strong matter-light coupling. We consider a non-equilibrium…

Quantum Gases · Physics 2018-11-14 Artem Strashko , Peter Kirton , Jonathan Keeling

We explore the dynamics of energy transfer between two nanocrystal quantum dots placed within an optical microcavity. By adjusting the coupling strength between the cavity photon mode and the quantum dots, we have the capacity to fine-tune…

Mesoscale and Nanoscale Physics · Physics 2024-10-02 Kaiyue Peng , Eran Rabani

Ultrafast spectroscopy is an emerging technique with great promise in the study of quantum materials, as it makes it possible to track similarities and correlations that are not evident near equilibrium. Thus far, however, the way in which…

Through a non-perturbative quantum theory, we investigate how the quasi-electron excitations of a two-dimensional electron gas are modified by strong coupling to the vacuum field of a microcavity. We show that the electronic dressed states…

Quantum Physics · Physics 2009-11-13 Simone De Liberato , Cristiano Ciuti

Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub{\aa}ngstrom and femtosecond spatiotemporal resolution. We present a theory predicting that…

Ultrafast nonlinear photonics enables a host of applications in advanced on-chip spectroscopy and information processing. These rely on a strong intensity dependent (nonlinear) refractive index capable of modulating optical pulses on…