English

Room-temperature exciton-polaritons with two-dimensional WS2

Mesoscale and Nanoscale Physics 2016-08-31 v2 Materials Science Optics

Abstract

Two-dimensional transition metal dichalcogenides exhibit strong optical transitions with significant potential for optoelectronic devices. In particular they are suited for cavity quantum electrodynamics in which strong coupling leads to polariton formation as a root to realisation of inversionless lasing, polariton condensationand superfluidity. Demonstrations of such strongly correlated phenomena to date have often relied on cryogenic temperatures, high excitation densities and were frequently impaired by strong material disorder. At room-temperature, experiments approaching the strong coupling regime with transition metal dichalcogenides have been reported, but well resolved exciton-polaritons have yet to be achieved. Here we report a study of monolayer WS2_2 coupled to an open Fabry-Perot cavity at room-temperature, in which polariton eigenstates are unambiguously displayed. In-situ tunability of the cavity length results in a maximal Rabi splitting of ΩRabi=70\hbar \Omega_{\rm{Rabi}} = 70 meV, exceeding the exciton linewidth. Our data are well described by a transfer matrix model appropriate for the large linewidth regime. This work provides a platform towards observing strongly correlated polariton phenomena in compact photonic devices for ambient temperature applications.

Keywords

Cite

@article{arxiv.1605.04743,
  title  = {Room-temperature exciton-polaritons with two-dimensional WS2},
  author = {Lucas C. Flatten and Zhengyu He and David M. Coles and Aurelien A. P. Trichet and Alex W. Powell and Robert A. Taylor and Jamie H. Warner and Jason M. Smith},
  journal= {arXiv preprint arXiv:1605.04743},
  year   = {2016}
}

Comments

12 pages, 6 figures

R2 v1 2026-06-22T14:01:36.678Z