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Bright ultrashort X-ray pulses allow scientists to observe ultrafast motion of atoms and molecules. Coherent light sources, such as the X-ray free electron laser (XFEL), enable remarkable discoveries in cell biology, protein…

A new regime in the interaction of a two-colour ($\omega$,$2\omega$) laser with a nanometre-scale foil is identified, resulting in the emission of extremely intense, isolated attosecond pulses - even in the case of multi-cycle lasers. For…

Plasma Physics · Physics 2020-04-22 Y. X. Zhang , S. Rykovanov , Mingyuan Shi , C. L. Zhong , X. T. He , B. Qiao , M. Zepf

Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…

We demonstrate an all-optical approach for precise characterization of attosecond extreme ultraviolet pulses. Isolated attosecond pulse is produced from high order harmonics using intense driving pulse with proper gating technique. When a…

Isotropic gases irradiated by long pulses of intense IR light can generate very high harmonics of the incident field. It is generally accepted that, due to the symmetry of the generating medium, be it an atomic or an isotropic molecular…

Atomic Physics · Physics 2016-09-28 R. E. F. Silva , P. Rivière , F. Morales , O. Smirnova , M. Ivanov , F. Martín

The landscape of ultrafast structured light pulses has recently evolved driven by the capability of high-order harmonic generation (HHG) to up-convert orbital angular momentum (OAM) from the infrared to the extreme-ultraviolet (EUV)…

High-harmonic generation (HHG) provides the only source of attosecond pulses -- currently the shortest accessible time intervals, and it is employed as the only table-top source of light in extreme UV and soft X-ray spectral regions. Chiral…

With the high-order harmonic generation (HHG) from plasma sur- faces it is possible to turn a laser pulse into a train of attosecond or even zeptosecond pulses in the backward radiation. These attosecond pulses may have amplitude several…

Plasma Physics · Physics 2016-11-03 Mykyta Cherednychek , Alexander Pukhov

We have produced a soft x-ray supercontinuum with a pulse energy of 0.24-$\mu$J using high-order harmonics from a multiterawatt, 10-Hz, stable, three-channel waveform synthesizer [Sci. Adv. eaay2802 (2020)]. We report here an attosecond…

Optics · Physics 2022-03-24 Bing Xue , Katsumi Midorikawa , Eiji J. Takahashi

Attosecond angular streaking measurements have revealed deep insights into the timing of tunnel ionization processes of atoms in intense laser fields. So far experiments of this type have been performed only with a cold-target recoil-ion…

Atomic Physics · Physics 2013-10-21 Matthias Weger , Jochen Maurer , André Ludwig , Lukas Gallmann , Ursula Keller

Advancing table-top attosecond sources in brightness and pulse duration is of immense interest and importance for an expanding sphere of applications. Recent theoretical studies [New J. Phys., 22 093030 (2020)] have found that high-order…

Optics · Physics 2022-08-31 V. A. Birulia , M. A. Khokhlova , V. V. Strelkov

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

We present a method of performing high-speed rotational anisotropy nonlinear optical harmonic generation experiments at rotational frequencies of several hertz by projecting the harmonic light reflected at different angles from a sample…

Materials Science · Physics 2015-10-15 J. W. Harter , L. Niu , A. J. Woss , D. Hsieh

Attosecond science is based on steering of electrons with the electric field of well-controlled femtosecond laser pulses. It has led to, for example, the generation of XUV light pulses with a duration in the sub-100-attosecond regime, to…

Quantum Physics · Physics 2011-07-11 Michael Krüger , Markus Schenk , Peter Hommelhoff

On the basis of real-time ab initio calculations, we study the non-perturbative interaction of two-color laser pulses with MgO crystal in the strong field regime to generate isolated attosecond pulse from high-harmonic emissions from MgO…

Attosecond pulses from free-electron lasers have opened the doors to atomic site-specific pumping and probing of quantum systems. Key to their success has been electron beam shaping techniques enabling the generation of sub-femtosecond…

We have used optically excited ultrashort electrical pulses to measure the magnetoplasmon resonance of a two-dimensional electron gas formed in an AlGaAs/GaAs heterostructure at frequencies up to 200 gigahertz. This is accomplished by…

Materials Science · Physics 2009-11-07 E. A. Shaner , S. A. Lyon

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

The ionization of atoms with sequences of attosecond pulses gives rise to excited ionic states that are entangled with the emitted photoelectron. Still, the ionic ensemble preserves some coherence that can be controlled through the laser…

Atomic Physics · Physics 2023-03-15 Saad Mehmood , Eva Lindroth , Luca Argenti

We report on continuous high-harmonic generation at 1 kHz repetition rate from a liquid-sheet plasma mirror driven by relativistic-intensity near-single-cycle light transients. Through precise control of both the surface plasma density…