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Electronic structure and magnetic properties for iron deficient TlFe$_{2-x}$Se$_2$ compounds are studied by first-principles calculations. We find that for the case of $x=0.5$ with a Fe-vacancy ordered orthorhombic superstructure, the…

Superconductivity · Physics 2011-05-23 Chao Cao , Jianhui Dai

In bulk samples and few layer flakes, the transition metal dichalcogenides NbS$_2$ and NbSe$_2$ assume the H polytype structure with trigonal prismatic coordination of the Nb atom. Recently, however, single and few layers of 1T-NbSe$_2$…

Strongly Correlated Electrons · Physics 2019-05-27 Cesare Tresca , Matteo Calandra

Tuning the electronic properties of a matter is of fundamental interest in scientific research as well as in applications. Recently, the Mott insulator-metal transition has been reported in a pristine layered transition metal…

Strongly Correlated Electrons · Physics 2020-05-29 Kunliang Bu , Wenhao Zhang , Ying Fei , Zongxiu Wu , Yuan Zheng , Jingjing Gao , Xuan Luo , Yu-Ping Sun , Yi Yin

In condensed matter physics, various mechanisms give rise to distinct insulating phases. The competition and interplay between these phases remain elusive, even for the seemingly most distinguishable band and Mott insulators. In multilayer…

Materials Science · Physics 2025-02-14 Zijian Lin , Jie Li , Xiaodong Cao , Jingjing Gao , Xuan Luo , Yuping Sun , Yi Lu , Nanlin Wang , Jiandong Guo , Xuetao Zhu

We investigate the interplay of the electron-electron and electron-phonon interactions in the electronic structure of an exotic insulating state in the layered dichalcogenide 1T-TaS2, where the charge-density-wave (CDW) order coexists with…

Materials Science · Physics 2017-07-12 Doohee Cho , Yong-Heum Cho , Sang-Wook Cheong , Ki-Seok Kim , Han Woong Yeom

Studying the atomic structure of intrinsic defects in two-dimensional transition metal dichalcogenides is difficult since they damage quickly under the intense electron irradiation in transmission electron microscopy (TEM). However, this…

Monolayers of two-dimensional van der Waals materials exhibit novel electronic phases distinct from their bulk due to the symmetry breaking and reduced screening in the absence of the interlayer coupling. In this work, we combine…

Mott insulator plays a central role in strongly correlated physics, where the repulsive Coulomb interaction dominates over the electron kinetic energy and leads to insulating states with one electron occupying each unit cell. Doped Mott…

Molybdenum disulfide (MoS2) is a layered semiconductor which has become very important recently as an emerging electronic device material. Being an intrinsic semiconductor the two-dimensional MoS2 has major advantages as the channel…

Mesoscale and Nanoscale Physics · Physics 2013-04-02 Ferdows Zahid , Lei Liu , Yu Zhu , Jian Wang , Hong Guo

Twisted bilayer MoTe2 is a prototypical moire material in which long-wavelength superlattices amplify electron correlations, enabling a wealth of emergent quantum phases. To date, experimental efforts have focused primarily on small twist…

1$T$-TaSe$_2$ is widely believed to host a Mott metal-insulator transition in the charge density wave (CDW) phase according to the spectroscopic observation of a band gap that extends across all momentum space. Previous investigations…

Strongly Correlated Electrons · Physics 2023-04-17 C. J. Sayers , G. Cerullo , Y. Zhang , C. E. Sanders , R. T. Chapman , A. S. Wyatt , G. Chatterjee , E. Springate , D. Wolverson , E. Da Como , E. Carpene

Mott insulators form because of strong electron repulsions, being at the heart of strongly correlated electron physics. Conventionally these are understood as classical "traffic jams" of electrons described by a short-ranged entangled…

High Energy Physics - Theory · Physics 2018-08-03 Tomas Andrade , Alexander Krikun , Koenraad Schalm , Jan Zaanen

Either in bulk form, or when exfoliated into atomically thin crystals, layered transition metal dichalcogenides are continuously leading to the discovery of new phenomena. The latest example is provided by 1T'-WTe$_2$, a semimetal recently…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Lin Wang , Ignacio Gutiérrez-Lezama , Céline Barreteau , Nicolas Ubrig , Enrico Giannini , A. F. Morpurgo

In a certain regime of low carrier densities and strong correlations, electrons can crystallize into a periodic arrangement of charge known as Wigner crystal. Such phases are particularly interesting in one dimension (1D) as they display a…

Strongly Correlated Electrons · Physics 2021-11-01 Anuva Aishwarya , Sean Howard , Bikash Padhi , Lihai Wang , Sang-Wook Cheong , Philip W. Phillips , Vidya Madhavan

The electronic structure of Mott insulators continues to be a major unsolved problem in physics despite more than half-century of intense research efforts. Well-developed momentum-resolved spectroscopies such as photoemission or neutron…

Strongly Correlated Electrons · Physics 2009-11-07 M. Z. Hasan , E. D. Isaacs , Z-X. Shen , L. L. Miller , K. Tsutsui , T. Tohyama , S. Maekawa

The electronic structures and topological properties of the orthorhombic and monoclinic phases of the quasi-one-dimensional excitonic insulator Ta2NiSe5 are investigated based on density functional theory. In contrast to a single parity or…

Materials Science · Physics 2022-02-02 Xiaobo Ma , Guangwei Wang , Huican Mao , Zhihong Yuan , Tianye Yu , Rui Liu , Yiran Peng , Pengyu Zheng , Zhiping Yin

Moir\'e superlattices in van der Waals heterostructures have emerged as a powerful tool for engineering novel quantum phenomena. Here we report the observation of a correlated interlayer exciton insulator in a double-layer heterostructure…

1T-transition metal dichalcogenides (TMD) have been an exciting platform for exploring the intertwinement of charge density waves and strong correlation phenomena. While the David star structure has been conventionally considered as the…

Strongly Correlated Electrons · Physics 2024-06-17 Cheong-Eung Ahn , Kyung-Hwan Jin , Young-Jae Choi , Jae Whan Park , Han Woong Yeom , Ara Go , Yong Baek Kim , Gil Young Cho

We present a combined experimental and theoretical study of monolayer VTe2 grown on highly oriented pyrolytic graphite by molecular-beam epitaxy. Using various in-situ microscopic and spectroscopic techniques, including scanning tunneling…

We compute the correlated electronic structure of stacked $1T$-TaS$_2$ bilayers using the $GW$ + EDMFT method. Depending on the surface termination, the semi-infinite uncorrelated system is either band-insulating or exhibits a metallic…