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Possible strain induced Mott gap collapse in 1T-TaS$_2$

Strongly Correlated Electrons 2020-05-29 v2 Materials Science

Abstract

Tuning the electronic properties of a matter is of fundamental interest in scientific research as well as in applications. Recently, the Mott insulator-metal transition has been reported in a pristine layered transition metal dichalcogenides 1T-TaS2_2, with the transition triggered by an optical excitation, a gate controlled intercalation, or a voltage pulse. However, the sudden insulator-metal transition hinders an exploration of how the transition evolves. Here, we report the strain as a possible new tuning parameter to induce Mott gap collapse in 1T-TaS2_2. In a strain-rich area, we find a mosaic state with distinct electronic density of states within different domains. In a corrugated surface, we further observe and analyze a smooth evolution from a Mott gap state to a metallic state. Our results shed new lights on the understanding of the insulator-metal transition and promote a controllable strain engineering on the design of switching devices in the future.

Keywords

Cite

@article{arxiv.2005.13311,
  title  = {Possible strain induced Mott gap collapse in 1T-TaS$_2$},
  author = {Kunliang Bu and Wenhao Zhang and Ying Fei and Zongxiu Wu and Yuan Zheng and Jingjing Gao and Xuan Luo and Yu-Ping Sun and Yi Yin},
  journal= {arXiv preprint arXiv:2005.13311},
  year   = {2020}
}

Comments

16 pages, 4 figures

R2 v1 2026-06-23T15:51:03.007Z