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The spin waves in single crystals of the layered van der Waals antiferromagnet CoPS$_3$ have been measured using inelastic neutron scattering. The data show four distinct spin wave branches with large ($\gtrsim 14$ meV) energy gaps at the…

Materials Science · Physics 2023-03-08 A. R. Wildes , B. Fåk , U. B. Hansen , M. Enderle , J. R. Stewart , L. Testa , H. M. Rønnow , C. Kim , Je-Geun Park

Two-dimensional van der Waals compounds with magnetic ions on a honeycomb lattice are hosts to a variety of exotic behavior. The magnetic interactions in one such compound, MnPSe$_3$, are investigated with elastic and inelastic neutron…

Strongly Correlated Electrons · Physics 2021-01-20 S. Calder , A. V. Haglund , A. I. Kolesnikov , D. Mandrus

We report a comprehensive spin wave analysis of the semiconducting honeycomb van der Waal antiferromagnet NiPS$_3$. Using single crystal inelastic neutron scattering, we map out the full Brillouin zone and fit the observed modes to a spin…

Neutron inelastic scattering has been used to measure the magnetic excitations in powdered NiPS$_3$, a quasi-two dimensional antiferromagnet with spin $S = 1$ on a honeycomb lattice. The spectra show clear, dispersive magnons with a $\sim…

Materials Science · Physics 2018-10-17 D. Lançon , R. A. Ewings , T. Guidi , F. Formisano , A. R. Wildes

Antiferromagnetic van der Waals family $\rm \textit{M}P\textit{X}_{3}\ (M=Fe,\ Mn,\ Co,\text{ and}\ Ni; X=S\text{ and}\ Se)$ have attracted significant research attention due to the possibility of realizing long-range magnetic order down to…

Strongly Correlated Electrons · Physics 2024-06-11 Junbo Liao , Zhentao Huang , Yanyan Shangguan , Bo Zhang , Shufan Cheng , Hao Xu , Ryoichi Kajimoto , Kazuya Kamazawa , Song Bao , Jinsheng Wen

Neutron spectroscopy measurements have been performed on single crystals of the antiferromagnetic van der Waals compound NiPS$_3$. Linear spin wave theory using a Heisenberg Hamiltonian with single-ion anisotropies has been applied to…

Strongly Correlated Electrons · Physics 2022-12-19 A. R. Wildes , J. R. Stewart , M. D. Le , R. A. Ewings , K. C. Rule , G. Deng , K. Anand

In the Van der Waal material $\rm NiPS_3$, Ni atoms have spin S=1 and realize a honeycomb lattice. Six sulfur atoms surround each Ni and split their d manifold into three filled and two unfilled bands. Aimed to determine the spin…

Strongly Correlated Electrons · Physics 2023-12-14 Paula Mellado

VI$_{3}$ is a ferromagnet with planar honeycomb sheets of bonded V$^{3+}$ ions held together by van der Waals forces. We apply neutron spectroscopy to measure the two dimensional ($J/J_{c} \approx 17$) magnetic excitations in the…

Strongly Correlated Electrons · Physics 2021-07-23 H. Lane , E. Pachoud , J. A. Rodriguez-Rivera , M. Songvilay , G. Xu , P. M. Gehring , J. P. Attfield , R. A. Ewings , C. Stock

Cu2(pymca)3(ClO4) (pymca: pyrimidine-2-carboxylate) consists of a slightly distorted honeycomb lattice of Cu2+ spins, which shows no long-range magnetic order down to 0.6 K. A magnetization study revealed 1/3 and 2/3 plateau phases [A.…

Strongly Correlated Electrons · Physics 2025-08-11 Masaaki Matsuda , Alexander I. Kolesnikov , Zentaro Honda , Tokuro Shimokawa , Sho Inoue , Yasuo Narumi , Masayuki Hagiwara

We present inelastic neutron scattering measurements of the antiferromagnetic insulator CaMn$_2$Sb$_2$, which consists of corrugated honeycomb layers of Mn. The dispersion of magnetic excitations has been measured along the H and L…

The magnetic properties of the two-dimensional, S=1 honeycomb antiferromagnet BaNi$_2$V$_2$O$_8$ have been comprehensively studied using DC susceptibility measurements and inelastic neutron scattering techniques. The magnetic excitation…

Strongly Correlated Electrons · Physics 2018-01-04 E. S. Klyushina , B. Lake , A. T. M. N. Islam , J. T. Park , A. Schneidewind , T. Guidi , E. A. Goremychkin , B. Klemke , M. Månsson

FePS3 is a layered van der Waals (vdW) Ising antiferromagnet that has recently been studied in the context of true 2D magnetism, and emerged as an ideal material platform for investigating strong spin-phonon coupling, and non-linear…

Strongly Correlated Electrons · Physics 2024-06-25 Ramesh Dhakal , Samuel Griffith , Stephen M. Winter

Altermagnets provide promising platforms for unconventional magnetism, whose controllability would enable a whole new generation of spintronic devices. While a variety of bulk altermagnets have been discovered, altermagnetism in…

Materials Science · Physics 2025-08-22 Luigi Camerano , Adolfo O. Fumega , Jose L. Lado , Alessandro Stroppa , Gianni Profeta

Van der Waals materials hosting Kitaev interactions are promising platforms for exploring exotic quantum phenomena. Here, we report inelastic neutron scattering investigations of the van der Waals antiferromagnet VBr3, which forms a…

Strongly Correlated Electrons · Physics 2026-03-03 Zeyu Kao , Yimeng Gu , Yiqing Gu , Hao Zhang , Shiyi Zheng , Naoki Murai , Seiko Ohira-Kawamura , Jun Zhao

The search for topological spin excitations in recently discovered two-dimensional (2D) van der Waals (vdW) magnetic materials is important because of their potential applications in dissipation-less spintronics. In the 2D vdW ferromagnetic…

Quantum magnets based on honeycomb lattices with low-coordination number offer a viable ground to realize exotic emergent quantum excitations and phenomena arising from the interplay between competing magnetic interactions, spin…

Strongly Correlated Electrons · Physics 2024-11-14 J. Khatua , M. Gomilsek , Kwang-Yong Choi , P. Khuntia

We report the revised crystal structure, static and dynamic magnetic properties of quasi-two dimensional honeycomb-lattice silver delafossite Ag3Co2SbO6. The magnetic susceptibility and specific heat data are consistent with the onset of…

FePS$_3$ is a van der Waals compound with a honeycomb lattice that is a good example of a two-dimensional antiferromagnet with Ising-like anisotropy. Neutron spectroscopy data from FePS3 were previously analysed using a straight-forward…

Materials Science · Physics 2020-07-15 A. R. Wildes , M. E. Zhitomirsky , T. Ziman , D. Lançon , H. C. Walker

We combine polarized infrared magneto-transmission and Faraday angle rotation measurements to map the collective excitations of the van der Waals antiferromagnet FePS$_3$. Below the N\'{e}el temperature ($T_\mathrm{N} \approx 118$ K), the…

Strongly Correlated Electrons · Physics 2025-08-21 Kartik Panda , Itzik Kapon , Dumitru Dumcenco , Dirk van der Marel , Alexey Kuzmenko , Nimrod Bachar

Strong interactions between different degrees of freedom lead to exotic phases of matter with complex order parameters and emergent collective excitations. Conventional techniques, such as scattering and transport, probe the amplitudes of…

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