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In the quantum sensing context most of the efforts to design novel quantum techniques of sensing have been constrained to idealized, noise-free scenarios, in which effects of environmental disturbances could be neglected. In this work, we…
We propose a new technique for comparing two Raman active samples. The method employs optical interference of the signals generated via coherent anti-Stokes Raman scattering (CARS) of broadband laser pulses with noisy spectra. It does not…
Triple sum-frequency (TSF) spectroscopy measures multidimensional spectra by resonantly exciting multiple quantum coherences of vibrational and electronic states. In this work we demonstrate pump-TSF-probe spectroscopy in which a pump…
Vibrational spectroscopy, comprised of infrared absorption and Raman scattering spectroscopy, is widely used for label-free optical sensing and imaging in various scientific and industrial fields. The group theory states that the two…
We discuss layout and performance of a high-resolution Stimulated Raman Loss spectrometer that has been newly developed for accurate studies of spectral lineshapes and line center frequencies of hydrogen isotopologues and in general of…
Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…
The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. For addressing systems with underlying bosonic structure, it is advantageous to utilize a naturally bosonic platform.…
Quantum squeezed states enable precision measurements beyond the standard quantum limit, but conventional solid-state media fundamentally limit pump intensities to the ionization threshold. We demonstrate that plasma waves can mediate…
Stimulated Raman scattering (SRS) microscopy has emerged as a powerful technique for probing the spatiotemporal dynamics of molecular bonds with exceptional sensitivity, resolution, and speed. However, classically, its performance remains…
Microresonators are powerful tools to enhance the efficiency of second-order nonlinear optical processes, such as second-harmonic generation, which can coherently bridge octave-spaced spectral bands. However, dispersion constraints such as…
Raman spectroscopy has attracted interest as a non-invasive optical technique to study the composition and structure of a wide range of materials at the microscopic level. The intrinsic fluorescence background can be orders of magnitude…
In this work, a microwave photonic prototype for concurrent radar detection and spectrum sensing is proposed, designed, built, and investigated. A direct digital synthesizer and an analog electronic circuit are integrated to generate an…
Resonant optical excitation of few-level quantum systems enables coherent quantum control, resonance fluorescence, and direct characterization of dephasing mechanisms. Experimental demonstrations have been achieved in a variety of atomic…
Chemical imaging enabled by Raman processes is crucial to investigating biological and chemical samples in a label-free manner. Stimulated Raman spectroscopy (SRS) overcomes the key limitation associated with low signal levels in…
Phase-sensitive optical parametric amplification of squeezed states helps to overcome detection loss and noise and thus increase the robustness of sub-shot-noise sensing. Because such techniques, e.g., imaging and spectroscopy, operate with…
For more than 20 years, optical microresonators have served as the backbone of integrated nonlinear photonics, exploiting Kerr nonlinearity to generate octave-spanning frequency combs, enable quantum effects, and drive optical parametric…
Dual-comb interferometry utilizes two optical frequency combs to map the optical field's spectrum to a radio-frequency signal without using moving parts, allowing improved speed and accuracy. However, the method is compounded by the…
Generation of laser-like narrow bandwidth emissions from nitrogen molecular ions generated in intense near- and mid-infrared femtosecond laser fields has aroused much interest because of the mysterious physics underlying such a phenomenon…
The bosonisation technique is used to calculate the resonant Raman spectrum of a quantum wire with two electronic sub-bands occupied. Close to resonance, the cross section at frequencies in the region of the inter sub-band transitions shows…
Observing few-photon optomechanical effects remains a significant challenge in optomechanical systems. To investigate intrinsic radiation-pressure-induced nonlinear effects in the few-photon regime, it is essential to strengthen the…