Related papers: Low Frequency Collinear Pre-Resonant Impulsive Sti…
Measurements monitoring the inductive coupling between oscillating radio-frequency magnetic fields and objects of interest create versatile platforms for non-destructive testing. The benefits of ultra low frequency measurements, i.e., below…
We propose and demonstrate a versatile technique to measure the lifetime of the one-phonon Fock state using two-color pump-probe Raman scattering and spectrally-resolved, time-correlated photon counting. Following pulsed laser excitation,…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
We present a flexible and efficient ultrafast time-resolved spontaneous Raman spectroscopy setup to study collective excitation and quasi-particle dynamics in quantum matter. The setup has a broad energy tuning range extending from the…
A dual-excitation method for resonant-frequency tracking in scanning probe microscopy based on amplitude detection is developed. This method allows the cantilever to be operated at or near resonance for techniques where standard phase…
Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…
Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…
Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…
Phase-sensitive pump-probe hyperspectral imaging is a precise technique for absolute two-beam measurements of the optical Kerr coefficient ($n_2$). The irradiance profile is characterized and background effects are rejected by rastering the…
Raman spectroscopy is a label-free, chemically specific optical technique which provides detailed information about the chemical composition and structure of the excited analyte. Because of this, there is growing research interest in…
Coplanar waveguide resonators are central to the thriving field of circuit quantum electrodynamics. Recently, we have demonstrated the generation of a broadband microwave-frequency comb spectrum using a superconducting quantum interference…
Time-resolved femtosecond stimulated Raman spectroscopy (FSRS) is a powerful tool for investigating ultrafast structural and vibrational dynamics in light absorbing systems. However, the technique generally requires exposing a sample to…
We propose to amplify and compress an ultrashort Light Spring laser seed with a long Gaussian-shaped laser pump through Raman amplification. This Light Spring, which has a helical spatio-temporal intensity profile, can be built on the…
The velocity distribution of a hot ionic beam can be filtered with a narrow stimulated Raman process to prepare a colder subensemble, as substantiated in this theoretical analysis. Using two counter-propagating, far-detuned lasers, we can…
We introduce the concept of phase-synchronous undersampling in nonlinear spectroscopy. The respective theory is presented and validated experimentally in a phase-modulated quantum beat experiment by sampling high phase modulation…
We demonstrate a new technique for saturated-absorption spectroscopy using co-propagating beams that does not have the problem of crossover resonances. The pump beam is locked to a transition and its absorption signal is monitored while the…
We show that it is possible to realize simultaneous Raman lasing at two different frequencies using a double-$\Lambda$ system pumped by a bi-frequency field. The Raman lasers are phase-locked to one another, and the beat-frequency matches…
We use the phenomenon of electromagnetically-induced transparency in a three-level atomic system for hyperfine spectroscopy of upper states that are not directly coupled to the ground state. The three levels form a ladder system: the probe…
We have observed multi-photon resonances in a system with a spin 3/2 irradiated simultaneously by a multiple pulse radiofrequency sequence and a low frequency field swept in the range 0-80 kHz. The used excitation scheme allowed us to…
We demonstrate the acquisition of stimulated Raman scattering spectra with the use of a single femtosecond pulse. High resolution vibrational spectra are obtained by shifting the phase of a narrow band of frequencies in the broadband input…