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An efficient all-electron G$^0$W$^0$ method and a quasiparticle selfconsistent GW (QSGW) method for molecules are proposed in the molecular orbital space with the full random phase approximation. The convergence with basis set is examined.…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 San-Huang Ke

We present a tight-binding based GW approach for the calculation of quasiparticle energy levels in confined systems such as molecules. Key quantities in the GW formalism like the microscopic dielectric function or the screened Coulomb…

Materials Science · Physics 2009-11-10 T. A. Niehaus , M. Rohlfing , F. Della Sala , A. Di Carlo , Th. Frauenheim

Electronic level alignment at the interface between an adsorbed molecular layer and a semiconducting substrate determines the activity and efficiency of many photocatalytic materials. Standard density functional theory (DFT) based methods…

Materials Science · Physics 2014-08-28 Annapaoala Migani , Duncan J. Mowbray , Jin Zhao , Hrvoje Petek , Angel Rubio

We present theoretical calculations of quasiparticle energies in closed-shell molecules using the GW method. We compare three different approaches: a full-frequency $G_0W_0$ (FF-$G_0W_0$) method with density functional theory (DFT-PBE) used…

Materials Science · Physics 2015-06-22 Johannes Lischner , Sahar Sharifzadeh , Jack Deslippe , Jeffrey B. Neaton , Steven G. Louie

We calculate the quasiparticle defect states and charge transition levels of oxygen vacancies in monoclinic hafnia. The charge transition levels, although they are thermodynamic quantities, can be critically dependent on the band gap owing…

Materials Science · Physics 2011-11-29 Manish Jain , James R. Chelikowsky , Steven G. Louie

We present a method for obtaining outer valence quasiparticle excitation energies from a DFT-based calculation, with accuracy that is comparable to that of many-body perturbation theory within the GW approximation. The approach uses a…

Strongly Correlated Electrons · Physics 2015-06-04 Sivan Refaely-Abramson , Sahar Sharifzadeh , Niranjan Govind , Jochen Autschbach , Jeffrey B. Neaton , Roi Baer , Leeor Kronik

In this review, we shortly summarize the basic theoretical milestones achieved in the mean-field theory of room temperature ionic liquids (RTILs) on charged electrodes since the publication of Kornyshev's seminal paper in 2007. We pay…

Soft Condensed Matter · Physics 2021-12-28 Yury A. Budkov , Andrei L. Kolesnikov

Quasiparticle excitation energies and optical properties of TiO$_{2}$ in the rutile and anatase structures are calculated using many-body perturbation theory methods. Calculations are performed for a frozen crystal lattice; electron-phonon…

Materials Science · Physics 2010-08-16 Wei Kang , Mark S. Hybertsen

Many-body perturbation theory within the G$_0$W$_0$ approximation is used to determine molecular orbital level alignment at a liquid water/Pt(111) interface generated through $ab~ initio$ molecular dynamics. Molecular orbital energy levels…

Mesoscale and Nanoscale Physics · Physics 2014-07-31 Isaac Tamblyn

The numerous combinations of cations and anions turn out possible to produce ionic liquids with fine-tuned properties once the correlation with the molecular structure is known. In this sense, computer simulations are useful tools to…

Quasielectrons and quasiholes in the fractional quantum Hall liquids obey fractional (including nontrivial mutual) exclusion statistics. Their statistics matrix can be determined from several possible state-counting scheme, involving…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 Y. S. Wu , Y. Yu , Y. Hatsugai , M. Kohmoto

Quasiparticle (QP) wave functions, also known as Dyson orbitals, extend the concept of single-particle states to interacting electron systems. Here we employ many-body perturbation theory in the GW approximation to calculate the QP wave…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 M. Strange , K. S. Thygesen

Quasiparticle - a key concept to describe interacting particles - characterizes electron-electron interaction in metals (Fermi liquid) and electron pairing in superconductors. While this concept essentially relies on the simplification of…

Mesoscale and Nanoscale Physics · Physics 2021-07-30 Satoru Tokuda , Seigo Souma , Kouji Segawa , Takashi Takahashi , Yoichi Ando , Takeshi Nakanishi , Takafumi Sato

The $GW$ approximation is a widely used method for computing electron addition and removal energies of molecules and solids. The computational effort of conventional $GW$ algorithms increases as $O(N^4)$ with the system size $N$, hindering…

Chemical Physics · Physics 2024-09-12 Mia Schambeck , Dorothea Golze , Jan Wilhelm

Correlations and the formation of bound states (nuclei) are essential for the properties of nuclear matter in equilibrium as well as in nonequilibrium. In a quantum statistical approach, quasiparticle energies are obtained for the light…

Nuclear Theory · Physics 2015-05-27 G. Röpke

The movement of ionic solutions is an essential part of biology and technology. Fluidics, from nano- to micro- to microfluidics, is a burgeoning area of technology which is all about the movement of ionic solutions, on various scales. Many…

Quantitative Methods · Quantitative Biology 2018-06-08 Shixin Xu , Bob Eisenberg , Zilong Song , Huaxiong Huang

In collisionless astrophysical plasmas, turbulence mediates the partitioning of free energy among cascade channels and its dissipation into ion and electron heat. The resulting ion heating is often anisotropic, with ions observed to be…

Solar and Stellar Astrophysics · Physics 2025-12-04 Zade Johnston , Jonathan Squire

The concept of the partial osmotic pressure of ions in an electrolyte solution is critically examined. In principle these can be defined by introducing a solvent-permeable wall and measuring the force per unit area which can certainly be…

Soft Condensed Matter · Physics 2022-12-09 Patrick B. Warren

A many-body wave function is approximated by a product of two functions: the wave function $\phi$ depending on the particle coordinates and the function $\chi$ depending only on the value of interparticle interaction potential. For the…

Quantum Physics · Physics 2008-09-10 V. M. Tapilin

We develop a flexible quasiparticle theory of transport coefficients of hot hadronic matter at finite baryon density. We begin with a hadronic quasiparticle model which includes a scalar and a vector mean field. Quasiparticle energies and…

Nuclear Theory · Physics 2016-01-20 M. Albright , J. I. Kapusta
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