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Two-dimensional group-VI transition metal dichalcogenide semiconductors, such as MoS2, WSe2 and others, exhibit strong light-matter coupling and possess direct band gaps in the infrared and visible spectral regimes, making them potentially…

Mesoscale and Nanoscale Physics · Physics 2020-03-03 Thomas Mueller , Ermin Malic

Lead halide perovskites show remarkable performance when used in photovoltaic and optoelectronic devices. However, the peculiarities of light-matter interactions in these materials in general are far from being fully explored experimentally…

Other Condensed Matter · Physics 2022-02-24 A. V. Trifonov , S. Grisard , A. N. Kosarev , I. A. Akimov , D. R. Yakovlev , J. Höcker , V. Dyakonov , M. Bayer

Excitons -- quasiparticles formed by the binding of an electron and a hole through electrostatic attraction -- hold promise in the fields of quantum light confinement and optoelectronic sensing. Atomically thin transition metal…

The equilibrium and non-equilibrium optical properties of single-layer transition metal dichalcogenides (TMDs) are determined by strongly bound excitons. Exciton relaxation dynamics in TMDs have been extensively studied by time-domain…

Layered 2D organic-inorganic perovskite semiconductors support strongly confined excitons that offer significant potential for ultrathin polaritonic devices due to their tunability and huge oscillator strength. The application of a magnetic…

Mesoscale and Nanoscale Physics · Physics 2025-02-26 Jonas K. König , Jamie M. Fitzgerald , Ermin Malic

The study of two-dimensional (2D) van der Waals materials has been an active field of research in the development of new optoelectronics and photonic applications over the last decade. Organic-inorganic layered perovskites are currently…

The coherent manipulation of excitons in bulk semiconductors via the lattice degrees of freedom is key to the development of acousto-optic and acousto-excitonic devices. Wide-bandgap transition metal oxides exhibit strongly bound excitons…

Exciton-polaritons are mixed light-matter excitations that result from the strong coupling regime between an active excitonic material and photonic resonances. Harnessing these hybrid excitations provides a rich playground to explore…

We show that a quasi-two dimensional condensate of optically active excitons emits coherent light even in the absence of population inversion. This allows an unambiguous and clear experimental detection of the condensed phase. We prove…

Condensed Matter · Physics 2015-06-25 J. Fernandez-Rossier , C. Tejedor , R. Merlin

Excitons, bound electron-hole pairs, in Two-Dimensional Hybrid Organic Inorganic Perovskites (2D HOIPs) are capable of forming hybrid light-matter states known as exciton-polaritons (E-Ps) when the excitonic medium is confined in an optical…

We demonstrate room temperature optical trapping and generation of high-order angular harmonics in exciton-polariton condensates in a monocrystalline CsPbBr$_3$ perovskite-filled microcavity. Using an annular nonresonant excitation profile…

The microscopic origin of slow carrier cooling in lead-halide perovskites remains debated, and has direct implications for applications. Slow carrier cooling has been attributed to either polaron formation or a hot-phonon bottleneck effect…

The use of semiconductor nanocrystals in scalable quantum technologies requires characterization of the exciton coherence dynamics in an \emph{ensemble} of electronically isolated crystals in which system-bath interactions are nevertheless…

Fully-inorganic cesium lead halide perovskite nanocrystals (NCs) have shown to exhibit outstanding optical properties such as wide spectral tunability, high quantum yield, high oscillator strength as well as blinking-free single photon…

Metal-halide perovskites are a versatile material platform for light-harvesting and light-emitting applications as their variable chemical composition allows the optoelectronic properties to be tailored to specific applications. Halide…

Integrated electro-optical switches are essential as one of the fundamental elements in the development of modern optoelectronics. As an architecture for photonic systems, exciton polaritons, that are hybrid bosonic quasiparticles that…

Exciton-polaritons offer a versatile platform for realization of all-optical integrated logic gates due to the strong effective optical nonlinearity resulting from the exciton-exciton interactions. In most of the current excitonic materials…

Atomistically detailed computational studies of nanocrystals, such as those derived from the promising lead-halide perovskites, are challenging due to the large number of atoms and lack of symmetries to exploit. Here, focusing on…

Materials Science · Physics 2022-10-05 Giulia Biffi , Yeongsu Cho , Roman Krahne , Timothy C. Berkelbach

Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical…

Excitons and their correlated complexes underpin the rich photophysics of quantum-confined semiconductors. Among these, biexcitons -- bound states of two electrons and two holes -- provide a sensitive probe of Coulomb correlations,…

Materials Science · Physics 2026-01-23 Katherine A. Koch , Carlos Silva-Acuña , Ajay Ram Srimath Kandada
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