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The coherent-state initial-value representation (IVR) for the semi-classical real-time propagator of a quantum system, developed by Herman and Kluk (HK), is widely used in computational studies of chemical dynamics. On the other hand, the…

Chemical Physics · Physics 2025-12-22 Binhao Wang , Fan Yang , Chen Xu , Peng Zhang

We present an Initial Value Representation for the semiclassical coherent state propagator based on complex trajectories. We map the complex phase space into a real phase space with twice as many dimensions and use a simple procedure to…

Quantum Physics · Physics 2009-08-14 Marcus A. M. de Aguiar , Silvio A. Vitiello , Adriano Grigolo

We assess the suitability of quantum and semiclassical initial value representations, exemplified by the coupled coherent states (CCS) method and the Herman Kluk (HK) propagator, respectively, for modeling the dynamics of an electronic wave…

Atomic Physics · Physics 2015-06-19 C. Zagoya , J. Wu , M. Ronto , D. V. Shalashilin , C. Figueira de Morisson Faria

We present a comprehensive study of semiclassical phase-space propagation in the Wigner representation, emphasizing numerical applications, in particular as an initial-value representation. Two semiclassical approximation schemes are…

Chemical Physics · Physics 2010-07-01 Thomas Dittrich , Edgar A. Gomez , Leonardo A. Pachon

Propagation of the Wigner function is studied on two levels of semiclassical propagation, one based on the van-Vleck propagator, the other on phase-space path integration. Leading quantum corrections to the classical Liouville propagator…

Quantum Physics · Physics 2007-05-23 Thomas Dittrich , Luis Sandoval , Carlos Viviescas

We present a complete derivation of the semiclassical limit of the coherent state propagator in one dimension, starting from path integrals in phase space. We show that the arbitrariness in the path integral representation, which follows…

Quantum Physics · Physics 2009-11-07 M. Baranger , M. A. M. de Aguiar , F. Keck , H. J. Korsch , B. Schellhaass

A unified viewpoint on the van Vleck and Herman-Kluk propagators in Hilbert space and their recently developed counterparts in Wigner representation is presented. It is shown that the numerical protocol for the Herman-Kluk propagator, which…

Chemical Physics · Physics 2018-03-14 Fabian Gottwald , Sergei D. Ivanov

In this work, we derived a semiclassical approximation for the matrix elements of a quantum propagator in coherent states (CS) basis that avoids complex trajectories, it only involves real ones. For that propose, we used the, symplectically…

Quantum Physics · Physics 2015-06-05 Alejandro M. F Rivas

Recent experimental progress using ultracold gases in optical lattices necessitates a quantitative theoretical description for a significant number of bosons. In the present paper, we investigate if time-dependent semiclassical initial…

Quantum Physics · Physics 2016-03-14 Shouryya Ray , Paula Ostmann , Lena Simon , Frank Großmann , Walter T. Strunz

A mixed semiclassical initial value representation expression for spectroscopic calculations is derived. The formulation takes advantage of the time-averaging filtering and the hierarchical properties of different trajectory based…

Quantum Physics · Physics 2016-05-27 Max Buchholz , Frank Grossmann , Michele Ceotto

The semiclassical propagator in the representation of SU(n) coherent states is characterized by isolated classical trajectories subjected to boundary conditions in a doubled phase space. In this paper we recast this expression in terms of…

Quantum Physics · Physics 2011-07-05 Thiago F. Viscondi , Marcus A. M. de Aguiar

The semiclassical Double Herman-Kluk Initial Value Representation is an accurate approach to computing quantum real time correlation functions, but its applications are limited by the need to evaluate an oscillatory integral. In previous…

Chemical Physics · Physics 2019-10-23 Matthew S. Church , Nandini Ananth

The Herman--Kluk propagator is a popular semi-classical approximation of the unitary evolution operator in quantum molecular dynamics. In this paper we formulate the Herman--Kluk propagator as a phase space integral and discretise it by…

Numerical Analysis · Mathematics 2016-05-03 Caroline Lasser , David Sattlegger

By using the overcompleteness of coherent states we find an alternative form of the unit operator for which the ket and the bra appearing under the integration sign do not refer to the same phase-space point. This defines a new quantum…

Quantum Physics · Physics 2015-03-13 Fernando Parisio

The semiclassical formula for the quantum propagator in the coherent state representation $<\mathbf{z}'' | e^{-i\hat{H}T/\hbar} | \mathbf{z}'>$ is not free from the problem of caustics. These are singular points along the complex classical…

Quantum Physics · Physics 2008-03-03 A. D. Ribeiro , M. A. M. de Aguiar

Complex-valued semiclassical methods hold out the promise of treating classically allowed and classically forbidden processes on the same footing. In addition, they provide a natural way to describe optical excitation with complex fields…

Quantum Physics · Physics 2017-08-23 Werner Koch , David J. Tannor

The Gaussian Wave-Packet phase-space representation is used to show that the expansion in powers of $\hbar$ of the quantum Liouville propagator leads, in the zeroth order term, to results close to those obtained in the statistical…

Atomic Physics · Physics 2009-10-30 G. W. Bund , S. S. Mizrahi , M. C. Tijero

The Van Vleck formula is a semiclassical approximation to the integral kernel of the propagator associated to a time-dependent Schr\"odinger equation. Under suitable hypotheses, we present a rigorous treatment of this approximation which is…

Analysis of PDEs · Mathematics 2021-12-06 Matthew D. Blair

We study the phase-space representation of dynamics of bosons in the semiclassical regime where the occupation number of the modes is large. To this end, we employ the van Vleck-Gutzwiller propagator to obtain an approximation for the…

Quantum Gases · Physics 2019-09-04 Ranchu Mathew , Eite Tiesinga

For a subquadratic symbol $H$ on $\R^d\times\R^d = T^*(\R^d)$, the quantum propagator of the time dependent Schr\"odinger equation $i\hbar\frac{\partial\psi}{\partial t} = \hat H\psi$ is a Semiclassical Fourier-Integral Operator when $\hat…

Mathematical Physics · Physics 2015-05-13 Didier Robert
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