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Electronic structure calculation of atoms and molecules, in the past few decades has largely been dominated by density functional methods. This is primarily due to the fact that this can account for electron correlation effects in a…

Chemical Physics · Physics 2013-07-12 Amlan K. Roy

Efficient hybrid DFT simulations of solid state materials would be extremely beneficial for computational chemistry and materials science, but is presently bottlenecked by difficulties in computing Hartree-Fock (HF) exchange with plane wave…

Chemical Physics · Physics 2024-10-30 Yuanheng Wang , Diptarka Hait , Pablo A. Unzueta , Juncheng Harry Zhang , Todd J. Martínez

In this paper, we present a spectral method based on Radial Basis Functions (RBFs) for numerically solving the fully nonlinear 1D Serre Green-Naghdi equations. The approximation uses an RBF discretization in space and finite differences in…

Fluid Dynamics · Physics 2014-07-17 Maurice S. Fabien

We present a new method to solve the nuclear density functional theory (DFT) equations using a two-center harmonic oscillator for Skyrme-like functionals, incorporating pairing and Coulomb interactions. The goal is to efficiently determine…

Nuclear Theory · Physics 2025-07-08 Adrián Sánchez-Fernández , Jacek Dobaczewski , Xuwei Sun , Herlik Wibowo

Spectral methods for solving partial differential equations (PDEs) and stochastic partial differential equations (SPDEs) often use Fourier or polynomial spectral expansions on either uniform and non-uniform grids. However, while very widely…

Numerical Analysis · Mathematics 2025-07-30 Channa Hatharasinghe , Run Yan Teh , Jesse van Rhijn , Peter D. Drummond , Margaret D. Reid

The ground state energy of a many-electron system can be approximated by an variational approach in which the total energy of the system is minimized with respect to one and two-body reduced density matrices (RDM) instead of many-electron…

Optimization and Control · Mathematics 2017-09-01 Yongfeng Li , Zaiwen Wen , Chao Yang , Yaxiang Yuan

Several applications of spectral methods to problems related to the relativistic astrophysics of compact objects are presented. Based on a proper definition of the analytical properties of regular tensorial functions we have developed a…

General Relativity and Quantum Cosmology · Physics 2007-05-23 S. Bonazzola , J. Frieben , E. Gourgoulhon , J. A. Marck

Vibrational properties of molecular crystals are constantly used as structural fingerprints, in order to identify both the chemical nature and the structural arrangement of molecules. The simulation of these properties is typically very…

Computational Physics · Physics 2019-10-09 Nathaniel Raimbault , Andrea Grisafi , Michele Ceriotti , Mariana Rossi

The self consistent version of the density functional theory (DFT) is presented, which allows to calculate the ground state and dynamic properties of finite multi-electron systems such as atoms, molecules and clusters. The exact functional…

Condensed Matter · Physics 2007-05-23 M. Ya. Amusia , V. R. Shaginyan

The Generalized Method of Moments (GMM) is a partition of unity based technique for solving electromagnetic and acoustic boundary integral equations. Past work on the GMM for electromagnetics was confined to geometries modeled by piecewise…

Computational Physics · Physics 2015-06-18 Daniel Dault , Naveen V. Nair , Jie Li , Balasubramaniam Shanker

We employ a fast and accurate algorithm to treat dielectric interfaces within molecular dynamics simulations and demonstrate the importance of dielectric boundary forces (DBFs) in two systems of interests in soft-condensed matter science.…

Soft Condensed Matter · Physics 2010-03-08 Stefan Kesselheim , Marcello Sega , Christian Holm

We introduce a fast Fourier spectral method for the multi-species Boltzmann collision operator. The method retains the riveting properties of the single-species fast spectral method (Gamba et al. SIAM J. Sci. Comput., 39 pp. B658--B674…

Computational Physics · Physics 2019-05-07 Shashank Jaiswal , Alina A. Alexeenko , Jingwei Hu

We introduce a general, variational scheme applied to Kohn-Sham density functional theory that allows for partitioning of the ground-state density matrix into distinct spectral domains, each of which spanned by an independent diagonal…

Plasma Physics · Physics 2023-08-29 Babak Sadigh , Daniel Aberg , John Pask

An analytical representation for the potential energy curve for the ground state $X^1\Sigma^+$ of the hydrogen fluoride molecule (HF) is presented in the frame of the Born-Oppenheimer approximation. The analytical expression for the…

Chemical Physics · Physics 2021-10-29 Laura E. Angeles Gantes , Horacio Olivares-Pilón

The subject of this paper is the design of efficient and stable spectral methods for time-dependent partial differential equations in unit balls. We commence by sketching the desired features of a spectral method, which is defined by a…

Numerical Analysis · Mathematics 2023-12-21 Jing Gao , Arieh Iserles

A new (algebraic) approximation scheme to find {\sl global} solutions of two point boundary value problems of ordinary differential equations (ODE's) is presented. The method is applicable for both linear and nonlinear (coupled) ODE's whose…

High Energy Physics - Theory · Physics 2008-11-26 Bruno Boisseau , Peter Forgacs , Hector Giacomini

We proposed a distributed approximating functional method for efficiently describing the electronic dynamics in atoms and molecules in the presence of the Coulomb singularities, using the kernel of a grid representation derived by using the…

Computational Physics · Physics 2016-04-05 Zhigang Sun

Extracting relevant information from atomistic simulations relies on a complete and accurate characterization of atomistic configurations. We present a framework for characterizing atomistic configurations in terms of a complete and…

Applied Physics · Physics 2024-02-07 Edward M. Kober , Jacob P. Tavenner , Colin M. Adams , Nithin Mathew

Stochastic and mixed stochastic-deterministic density functional theory (DFT) are promising new approaches for the calculation of the equation-of-state and transport properties in materials under extreme conditions. In the intermediate warm…

Computational Physics · Physics 2023-09-27 Vidushi Sharma , Lee A. Collins , Alexander J. White

Gaussian fields (GFs) are frequently used in spatial statistics for their versatility. The associated computational cost can be a bottleneck, especially in realistic applications. It has been shown that computational efficiency can be…

Computation · Statistics 2015-03-13 Xiaoyu Liu , Serge Guillas , Ming-Jun Lai