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Optical binding is a form of light-mediated forces between elements of matter which emerge in response to the collective scattering of light. Such phenomenon has been studied mainly in the context of equilibrium stability of dielectric…
Single atoms coupled to a cavity offer unique opportunities as quantum optomechanical devices because of their small mass and strong interaction with light. A particular regime of interest in optomechanics is that of "single-photon strong…
The interaction of atoms with higher-order Poincar\'e optical vortex modes of order $m\geq 0$ is explored for light close to resonance with atomic dipole transitions. It is well-known that atoms subject to optical vortex modes experience…
Photonic molecules, i.e. artificial structures composed of coherently coupled optical cavities, are paradigmatic systems for investigating fundamental phenomena across photonics, quantum optics and topological physics. In recent years,…
Ultracold collisions of the polyatomic species CaOH are considered, in internal states where the collisions should be dominated by long-range dipole-dipole interactions. The computed rate constants suggest that evaporative cooling can be…
The rovibrational spectrum of the molecular ion H$_2$CCCH$^+$ was investigated in a 4~K cryogenic ion trap instrument employing the leak-out spectroscopy method. Transitions within the fundamental $\nu_1$ (C-H stretch) and the combination…
Polyatomic molecules have rich structural features that make them uniquely suited to applications in quantum information science, quantum simulation, ultracold chemistry, and searches for physics beyond the Standard Model. However, a key…
Recent years have seen significant developments in the study of strong light-matter coupling including the control of chemical reactions by altering the vibrational normal modes of molecules. In the vibrational strong coupling regime the…
Nonadiabatic phenomena are investigated in the rovibrational motion of molecules confined in an infrared cavity. Conical intersections (CIs) between vibrational polaritons, similar to CIs between electronic polaritonic surfaces, are found.…
We study the motion of an undamped single-ion harmonic oscillator, resonantly driven with a pulsed radiation pressure force. We demonstrate that a barium ion, initially cooled to the Doppler limit, quickly phase locks to the drive and…
Doppler cooling of calcium ions has been experimentally demonstrated using the S1/2 to D5/2 dipole-forbidden transition. Scattering forces and fluorescence levels a factor of 5 smaller than for usual Doppler cooling on the dipole allowed…
In the last decade, hybrid organic-inorganic halide perovskites have emerged as a new type of semiconductor for photovoltaics and other optoelectronic applications. Unlike standard, tetrahedrally bonded semiconductors (e.g. Si and GaAs),…
We demonstrate the ability to load, cool and detect singly-charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using…
A theoretical study of the low-energy scattering properties of two aligned identical bosonic and fermionic dipoles in the presence of isotropic spin-orbit coupling (SOC) is presented. A general treatment of particles with arbitrary…
We propose a novel cooling scheme for realising single photon sideband cooling on particles trapped in a state-dependent optical potential. We develop a master rate equation from an ab-initio model and find that in experimentally feasible…
We present a new method for the generation of rotationally and vibrationally state-selected, translationally cold molecular ions in ion traps. Our technique is based on the state-selective threshold photoionization of neutral molecules…
We demonstrate direct cooling of gaseous formaldehyde (H2CO) to the microkelvin regime. Our approach, optoelectrical Sisyphus cooling, provides a simple dissipative cooling method applicable to electrically trapped dipolar molecules. By…
The absorption spectra of the cold Na2 molecule dressed by a linearly polarized standing laser wave is investigated. In the studied scenario the rotational motion of the molecules is frozen while the vibrational and translational degrees of…
Recent experiments involving the interaction of optical vortices with atoms in quadrupole transitions have been shown to be accompanied by the exchange of orbital angular momentum (OAM) between the electronic states of the atom and the…
We demonstrate several building blocks for an ion-photon interface based on a trapped Ca ion in an optical cavity. We identify a favorable experimental configuration and measure system parameters, including relative motion of the trapped…