Related papers: Large optical nonlinearity enhancement under elect…
We consider how nonlinear interaction effects can manifest themselves and even be enhanced in a strongly driven optomechanical system. Using a Keldysh Green's function approach, we calculate modifications to the cavity density of states due…
Strongly correlated solids are extremely complex and fascinating quantum systems, where new states continue to emerge, especially when interaction with light triggers interplay between them. In this interplay, sub-laser-cycle electron…
State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…
Optical information processing and computing can potentially offer enhanced performance, scalability and energy efficiency. However, achieving nonlinearity-a critical component of computation-remains challenging in the optical domain. Here…
Coherent nonlinear optical micro-spectroscopy is a frequently used tool in modern material science, as it is sensitive to many different local observables, which comprise, among others, crystal symmetry and vibrational properties. The…
Nonlinear interactions between x-rays and long wavelengths can be used as a powerful atomic scale probe for light-matter interactions and for properties of valence electrons. This probe can provide novel microscopic information in solids…
Silicon photonics has attracted significant interest in recent years due to its potential in integrated photonics components (1,2) as well as all-dielectric meta-optics elements.(3) Strong photon-photon interactions, aka optical…
We fabricate and characterize a microscale silicon electro-opto-mechanical system whose mechanical motion is coupled capacitively to an electrical circuit and optically via radiation pressure to a photonic crystal cavity. To achieve large…
Nonlinear optical phenomena play important roles in the vast emerging fields of micro- and nano-technology. This paper describes the general characteristics of nonlinear optical materials and systems, with a focus on parametric…
The extraordinary properties of resonant four-wave mixing of backward waves in doped negative-index materials are investigated. The feasibility of independent engineering of negative refractive index and nonlinear optical response as well…
Ultracompact nonlinear optical devices utilizing two-dimensional (2D) materials and nanostructures are emerging as important elements of photonic circuits. Integration of the nonlinear material into a subwavelength cavity or waveguide leads…
We investigate the collective optomechanics of an ensemble of scatterers inside a Fabry-Perot resonator and identify an optimized configuration where the ensemble is transmissive, in contrast with the usual reflective optomechanics…
We predict a resonant enhancement of the nonlinear optical response of an interacting Rydberg gas under conditions of electromagnetically induced transparency. The enhancement originates from a two-photon process which resonantly couples…
We describe an all-fiber nonlinear interferometer based on four-wave mixing in highly nonlinear fiber. Our configuration realizes phase-sensitive interference with 97% peak visibility and >90% visibility over a broad 554 GHz optical band.…
High peak power ultrafast lasers are widely used in nonlinear spectroscopy but often limit its spectral resolution because of the broad frequency bandwidth of ultrashort laser pulses. Improving the resolution by achieving spectrally narrow…
We investigate, theoretically and numerically, the dependence of a material's nonlinear-optical response on the linear relative electric permittivity $\epsilon$ and magnetic permeability $\mu$. The conversion efficiency of low-order…
In the last two decades, non-equilibrium spectroscopies have evolved from avant-garde studies to crucial tools for expanding our understanding of the physics of strongly correlated materials. The possibility of obtaining simultaneously…
Controlling chemical and material properties through strong light-matter coupling in optical cavities has gained considerable attention over the past decade. However, the underlying mechanisms remain insufficiently understood, and a…
Large exciton-polariton optical nonlinearities present a key mechanism for photonics-based communication, ultimately in the quantum regime. Enhanced nonlinear response from various materials hosting excitons and allowing for their strong…
We employ a quantum theory of the nonlinear optical response from an actual solid-state material possessing an intrinsic bulk contribution to the third-order nonlinear susceptibility (Kerr-type nonlinearity), which can be arbitrarily…