Related papers: Transition strength measurements to guide magic wa…
Some of us have recently reported in Science 321 232 (2008) vibrational cooling of translationally cold Cs_2 molecules into the lowest vibrational level v=0 of the singlet X 1Sigma_g ground electronic state. Starting from a sample of cold…
The soft character of organic materials leads to strong coupling between molecular nuclear and electronic dynamics. This coupling opens the way to control charge transport in organic electronic devices by inducing molecular vibrational…
Europium-doped crystal $\mathrm{Y}_2\mathrm{SiO}_5$ is an interesting platform for optical quantum memories, due to its long optical and spin coherence times. In this work, we investigate…
Magneto-optically trapped atoms enable the determination of lifetimes of metastable states and higher lying excited states like the $\rm{5d^{2}~^{3}F_{2}}$ state in barium. The state is efficiently populated by driving strong transitions…
Quantum simulations provide means to probe challenging problems within controllable quantum systems. However, implementing or simulating deep-strong nonlinear couplings between bosonic oscillators on physical platforms remains a challenge.…
We present a joint experimental and theoretical study of spin coherence properties of 39K, 85Rb, 87Rb, and 133Cs atoms trapped in a solid parahydrogen matrix. We use optical pumping to prepare the spin states of the implanted atoms and…
A two-level quantum system coherently driven by a resonant electromagnetic field oscillates sinusoidally between the two levels at frequency $\Omega$ which is proportional to the field amplitude [1]. This phenomenon, known as the Rabi…
Molecular complexes are held together via a variety of bonds, but they all share the common feature that their individual entities are in contact. In this work, we introduce and demonstrate the concept of a \textit{molecular optical bond},…
Quantum process tomography is used to fully characterize the evolution of the quantum vibrational state of atoms. Rubidium atoms are trapped in a shallow optical lattice supporting only two vibrational states, which we charcterize by…
The hydrogen molecule has become a test ground for quantum electrodynamical calculations in molecules. Expanding beyond studies on stable hydrogenic species to the heavier radioactive tritium-bearing molecules, we report on a measurement of…
We argue that long optical storage times are required to establish entanglement at high rates over large distances using memory-based quantum repeaters. Triggered by this conclusion, we investigate the $^3$H$_6$ $\leftrightarrow$ $^3$H$_4$…
We show that the lifetime of ultracold ground-state $^{87}$Rb$^{133}$Cs molecules in an optical trap is limited by fast optical excitation of long-lived two-body collision complexes. We partially suppress this loss mechanism by applying…
Strong coupling between light and matter is possible with a variety of organic materials. In contrast to the simpler inorganic case, organic materials often have a complicated spectrum, with vibrationally dressed electronic transitions.…
Single molecules trapped in the solid state at liquid helium temperatures are promising quantum emitters for the development of quantum technologies owing to their remarkable photostability and their lifetime-limited optical coherence time…
Strong light-matter coupling to form exciton- and vibropolaritons is increasingly touted as a powerful tool to alter the fundamental properties of organic materials. It is proposed that these states and their facile tunability can be used…
In modern particle physics experiments wavelength-shifting and scintillating fibres based on plastic polymers are used for tracking and calorimetry. In this review the role of photon trapping efficiencies, transmission functions and signal…
Perfectly controlled molecules are at the forefront of the quest to explore chemical reactivity at ultra low temperatures. Here, we investigate for the first time the formation of the long-lived intermediates in the time-dependent…
Rare-earth ions are characterised by transitions with very narrow linewidths even in solid state crystals. Exceedingly long coherence times have been shown on both spin and optical transitions of rare-earth-ion doped crystals. A key factor,…
We have studied the temporal behavior of the atomic absorption signal under resonant excitation with a continuous-wave laser radiation. Measurements done for D2 line of 85Rb with ~ 1 ns temporal resolution have shown irregular oscillatory…
Optically trapped ensembles are of crucial importance for frequency measurements and quantum memories, but generally suffer from strong dephasing due to inhomogeneous density and light shifts. We demonstrate a drastic increase of the…