Related papers: Transition strength measurements to guide magic wa…
Motivated by compelling advances in manipulating cold Rydberg (Ry) atoms in optical traps, we consider the effect of large extent of Ry electron wave function on trapping potentials. We find that when the Ry orbit lies outside inflection…
Molecular excited vibrational states are metastable states and we incorporate their finite lifetimes into the theory of vibrational energy transfer between weakly interacting molecules, i.e., at internuclear distances at which they do not…
We demonstrate $|W\rangle$ state encoding of multi-atom ensemble qubits. Using optically trapped Rb atoms the $T_2$ coherence time is 2.6(3) ms for $\bar N=7.6$ atoms and scales approximately inversely with the number of atoms. Strong…
Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit…
Optical skyrmions are topological structures of light whose defining property, the skyrmion number, is robust against perturbations. This makes them attractive for applications in quantum information storage, where resilience to decoherence…
Direct evidence of quantum coherence in a single-molecule magnet in frozen solution is reported with coherence times as long as T2 = 630 ns. We can strongly increase the coherence time by modifying the matrix in which the single-molecule…
A long-lived coherent state and non-linear interaction have been experimentally demonstrated for the vibrational mode of a trapped ion. We propose an implementation of quantum computation using coherent states of the vibrational modes of…
Using first-principles calculations, we identify magic wavelengths for the 2s-2p and 2s-3p transitions in lithium. The ns and np atomic levels have the same ac Stark shifts at the corresponding magic wavelength, which facilitates…
Several years ago, it was shown that strong coupling between an electronic transition in organic molecules and a resonant photonic structure can modify the electronic landscape of the molecules and affect their chemical behavior. Since…
Selection of "magic" trapping conditions with ultracold atoms or molecules, where pairs of internal states experience identical trapping potentials, brings substantial benefits to precision measurements and quantum computing schemes.…
The quantum Rabi model, involving a two-level system and a bosonic field mode, is arguably the simplest and most fundamental model describing quantum light-matter interactions. Historically, due to the restricted parameter regimes of…
The act of measurement bridges the quantum and classical worlds by projecting a superposition of possible states into a single, albeit probabilistic, outcome. The time-scale of this "instantaneous" process can be stretched using weak…
Using numerical simulations of two-photon electronic absorption with femtosecond pulses in Na$_2$ we show that: i) it is possible to avoid the characteristic saturation or dumped Rabi oscillations in the yield of absorption by time-delaying…
Rabi measurements in atomic vapor cells are of current interest in a range of microwave imaging and sensing experiments, but are increasingly in a parameter space outside of theoretical studies of coherence defined by spin-exchange…
The absorption spectra of the cold Na2 molecule dressed by a linearly polarized standing laser wave is investigated. In the studied scenario the rotational motion of the molecules is frozen while the vibrational and translational degrees of…
We demonstrate the coherent creation of a single NaCs molecule in its rotational, vibrational, and electronic (rovibronic) ground state in an optical tweezer. Starting with a weakly bound Feshbach molecule, we locate a two-photon transition…
We show how one can measure the signal from slow jumps of a single molecule between metastable positions using a setup where the molecule is fixed to one lead, and one of the coupling strengths is controlled externally. Such a measurement…
Continuous weak or fuzzy measurement of the Rabi oscillation of a two level atom subjected to a $\pi-$pulse of a resonant light field is simulated numerically. We thereby address the question whether it is possible to measure characteristic…
We investigate the influence of atomic motion on precision Rabi spectroscopy of ultracold fermionic atoms confined in a deep, one dimensional (1D) optical lattice. We analyze the spectral components of longitudinal sideband spectra and…
We study the internal state dynamics of optically trapped polyatomic molecules subject to room temperature blackbody radiation. Using rate equations that account for radiative decay and blackbody excitation between rovibrational levels of…