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We describe how a local non-equilibrium nuclear polarisation can be generated and detected by electrical means in a semiconductor quantum point contact device. We show that measurements of the nuclear spin relaxation rate will provide clear…

Mesoscale and Nanoscale Physics · Physics 2008-06-26 N. R. Cooper , V. Tripathi

While the breakdown of the perturbation expansion for the many-electron problem has several formal consequences, here we unveil its physical effect: Flipping the sign of the effective electronic interaction in specific scattering channels.…

Strongly Correlated Electrons · Physics 2020-11-06 M. Reitner , P. Chalupa , L. Del Re , D. Springer , S. Ciuchi , G. Sangiovanni , A. Toschi

We calculate the non-linear tunneling current through a molecule with two electron-accepting orbitals which interact with an intramolecular vibration. We investigate the interplay between Coulomb blockade and non-equilibrium…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Katja C. Nowack , Maarten R. Wegewijs

As promising quantum sensors, nitrogen-vacancy (NV) centers in diamond have been widely used in frontier studies in condensed matter physics, material sciences, and life sciences. In practical applications, weak laser excitation is…

We report on the observation of coherent molecular vibrations launched by the breaking of a molecular bond. The methyl radical, which is produced by $267\,\mathrm{nm}$ photodissociation of methyl iodide, is excited to high levels in its…

Vibrational nonequilibrium effects in charge transport through single-molecule junctions are investigated. Focusing on molecular bridges with multiple electronic states, it is shown that electronic-vibrational coupling triggers a variety of…

Mesoscale and Nanoscale Physics · Physics 2011-03-15 R. Härtle , C. Benesch , M. Thoss

We investigate vibrational properties and lattice distortion of negatively charged nitrogen-vacancy (NV) center in diamond. Using the first-principles electronic structure calculations, we show that the presence of NV center leads to…

Materials Science · Physics 2015-05-27 Jianhua Zhang , Cai-Zhuang Wang , Z. Z. Zhu , V. V. Dobrovitski

The "atomic saw method" uses the passage of dislocations in two-dimensional (2D) quantum-well superlattices to create periodic slipping layers and one-dimensional (1D) quantum wire superlattices. The effects of this space structuring of the…

Disordered Systems and Neural Networks · Physics 2007-08-14 T. Ferrus , B. Goutiers , L. Ressier , J. P. Peyrade , J. A. Porto , J. Sanchez-dehesa

We study theoretically the effects of heating on the magnetic flux moving in superconductors with a periodic array of pinning sites (PAPS). The voltage-current characteristic (VI-curve) of superconductors with a PAPS includes a region with…

Superconductivity · Physics 2008-04-14 V. R. Misko , S. Savel'ev , A. L. Rakhmanov , Franco Nori

Carbon nanotube junctions are predicted to exhibit negative differential resistance, with very high peak-to-valley current ratios even at room temperature. We treat both nanotube p-n junctions and undoped metal-nanotube-metal junctions,…

Condensed Matter · Physics 2009-10-31 F. Leonard , J. Tersoff

Ultrafast laser excitation can trigger multiplex coherent dynamics in molecules. Here, we report attosecond transient absorption experiments addressing simultaneous probing of electronic and vibrational dynamics in a prototype molecule,…

Strong light-matter interaction in cavity environments is emerging as a promising approach to control chemical reactions in a non-intrusive and efficient manner. The underlying mechanism that distinguishes between steering, accelerating, or…

Quantum Physics · Physics 2022-12-20 Christian Schäfer , Johannes Flick , Enrico Ronca , Prineha Narang , Angel Rubio

The quantum nonlinear dimer consisting of an electron shuttling between the two sites and in weak interaction with vibrations, is studied numerically under the application of a DC electric field. A field-induced resonance phenomenon between…

Other Condensed Matter · Physics 2011-11-04 M. Tiwari , D. V. Seletskiy , V. M. Kenkre

We present a perturbation approach rooted in time-dependent density-functional theory to calculate electron hole (eh)-pair excitation spectra during the non-adiabatic vibrational damping of adsorbates on metal surfaces. Our analysis for the…

Chemical Physics · Physics 2017-11-22 Simon P. Rittmeyer , Jörg Meyer , Karsten Reuter

Gunn (or Gunn-Hilsum) Effect and its associated negative differential resistivity (NDR) emanates from transfer of electrons between two different energy bands in a semiconductor. If applying a voltage (electric field) transfers electrons…

Mesoscale and Nanoscale Physics · Physics 2018-05-01 Daryoush Shiri , Amit Verma , Reza Nekovei , Andreas Isacsson , C. R. Selvakumar , M. P. Anantram

The interplay between uniaxial strain and charging effects in zigzag graphene nanoribbons (ZGNR) is investigated by using non-equilibrium Green's function formalism. The I-V characteristic curves and especially negative differential…

Mesoscale and Nanoscale Physics · Physics 2019-12-05 Maliheh Azadparvar , Hosein Cheraghchi

Optically active quantum defects in solids, such as the nitrogen vacancy (NV) center in diamond, are a leading modality for micron-scale and nanoscale (ultralow-mass) nuclear magnetic resonance (NMR) spectroscopy and imaging under ambient…

We investigate chemical bond formation and conductance in a molecular C60-junction under finite bias voltage using first-principles calculations based on density functional theory and nonequilibrium Green's functions (DFT-NEGF). At the…

Mesoscale and Nanoscale Physics · Physics 2013-02-04 Søren Ulstrup , Thomas Frederiksen , Mads Brandbyge

We present a qualitative model for a fundamental process in molecular electronics: the change in conductance upon bond breaking. In our model a diatomic molecule is attached to spin-polarized contacts. Employing a Hubbard Hamiltonian,…

Materials Science · Physics 2008-06-24 Ali Goker , Francois Goyer , Matthias Ernzerhof

Two dimensional electron gases in narrow GaAs quantum wells show huge longitudinal resistance (HLR) values at certain fractional filling factors. Applying an RF field with frequencies corresponding to the nuclear spin splittings of {69}Ga,…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 S. Kronmueller , W. Dietsche , K. v. Klitzing , G. Denninger , W. Wegscheider , M. Bichler