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Chromium (II) fluoroperovskites $A\mathrm{CrF_3}(A\mathrm{=Na^+,K^+})$ are strongly correlated Jahn-Teller active materials at low temperatures. In this paper, we examine the role that the $A$-site ion plays in this family of…

Materials Science · Physics 2021-07-07 F. L. M. Bernal , F. Lundvall , S. Kumar , P-A. Hansen , D. S. Wragg , O. M. Løvvik , H. Fjellvåg

The Jahn-Teller distortion and the resulting orbital order usually cause some fascinating correlated electronic behaviors, and generally lead to antiferromagnetism in perovskite bulks. Here we demonstrate that the Jahn-Teller distortion…

Materials Science · Physics 2023-05-03 Ke Ji , Zongshuo Wu , Xiaofan Shen , Jianli Wang , Junting Zhang

KCrF3 represents another prototypical orbital-ordered perovskite, where Cr2+ possesses the same electronic configuration of 3d4 as that of strongly Jahn-Teller distorted Mn3+ in many CMR manganites. The crystal and magnetic structures of…

Strongly Correlated Electrons · Physics 2013-09-30 Y. Xiao , Y. Su , H. -F. Li , C. M. N. Kumar , R. Mittal , J. Persson , A. Senyshyn , K. Gross , Th. Brueckel

There is great interest in hybrid organic-inorganic materials such as metal-organic frameworks (MOFs). The compounds [C(NH$_{2}$)$_{3}$]M(HCOO)$_{3}$, where M=Cu$^{2+}$ or Cr$^{2+}$ are Jahn-Teller (JT) active ions, are MOF with perovskite…

Materials Science · Physics 2014-03-27 Alessandro Stroppa , Paolo Barone , Prashant Jain , Jean Manuel Perez-Mato , Silvia Picozzi

The electronic structure and magnetic properties of the Jahn-Teller-distorted perovskite KAgF3 have been investigated using the full-potential linerized aug- mented plane-wave method. It is found that KAgF3 exhibits significant quasi-one-…

Strongly Correlated Electrons · Physics 2015-05-19 Xiaoli Zhang , Guoren Zhang , Ting Jia , Ying Guo , Zhi Zeng , H. Q. Lin

We investigate the origin of the orbital ordering in the paramagnetic phase of KCrF$_3$. All previous studies described structural parameters of the paramagnetic phase using a magnetic ordering in the compound. Our simulations of real…

Strongly Correlated Electrons · Physics 2016-08-24 D. Novoselov , Dm. M. Korotin , V. I. Anisimov

In this work we study the complex entanglement between spin interactions, electron correlation and Janh-Teller structural instabilities in the 5d$^1$ $J_{eff}=\frac{3}{2}$ spin-orbit coupled double perovskite $\rm Ba_2NaOsO_6$ using first…

Perovskite oxides are already widely used in industry and have huge potential for novel device applications thanks to the rich physical behaviour displayed in these materials. The key to the functional electronic properties exhibited by…

Materials Science · Physics 2017-05-08 Julien Varignon , Nicholas C. Bristowe , Eric Bousquet , Philippe Ghosez

We introduce an effective model for $e_g$ electrons to describe three-dimensional perovskite (La$_{1-x}$Sr$_{x}$MnO$_3$ and La$_{1-x}$Ca$_{x}$MnO$_3$) manganites and study the magnetic and orbital order on $4\times 4\times 4$ cluster using…

Strongly Correlated Electrons · Physics 2010-10-26 Krzysztof Rościszewski , Andrzej M. Oleś

The silver fluoride Ag$_3$F$_5$ consists structurally of square-planar units formed by four fluoride ions coordinated to a central silver ion, which possesses a partially filled $d$-subshell and the formal valence of +5/3. In this study, we…

Strongly Correlated Electrons · Physics 2025-04-07 Dmitry M. Korotin , Dmitry Y. Novoselov , Yaroslav M. Plotnikov , Vladimir I. Anisimov

Single crystalline (Bi,Ca)MnO3 (74< %Ca <82) were studied with neutron scattering, electron diffraction and bulk magnetic measurement. We discovered dynamic ferromagnetic spin correlations at high temperatures, which are replaced by…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , J. D. Axe , C. H. Chen , S-W. Cheong

The orbital, lattice, and spin ordering phenomena in KCuF3 are investigated by means of LDA+U calculations, based on ab-initio pseudopotentials.We examine the Cu-3d orbital ordering and the associated Jahn-Teller distortion in several…

Strongly Correlated Electrons · Physics 2009-11-10 N. Binggeli , M. Altarelli

Motivated by recent experiments, we present a comprehensive theoretical study of the geometrically frustrated strongly correlated magnetic insulator Mn$_3$O$_4$ spinel oxide based on a microscopic Hamiltonian involving lattice, spin and…

Strongly Correlated Electrons · Physics 2017-08-23 Santanu Pal , Siddhartha Lal

A detailed high-resolution, variable temperature powder diffraction study of the fluoro-perovskites NaFeF$_3$ and NaCoF$_3$ is performed to probe their orbital ordering transitions. Through analysis of the symmetry adapted macrostrains and…

Strongly Correlated Electrons · Physics 2025-04-07 C. A. Crawford , C. I. Hiley , J. Gainza , C. Ritter , R. I. Walton , Mark S. Senn

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

Strongly Correlated Electrons · Physics 2021-03-30 J. Khatua , T. Arh , Shashi B. Mishra , H. Luetkens , A. Zorko , B. Sana , M. S. Ramachandra Rao , B. R. K. Nanda , P. Khuntia

The electronic structure and magnetism in the sodium nickelate NaNiO_2 in the low-temperature phase is studied from density-functional calculations using the linear muffin-tin orbitals method. An antiferromagnetic solution with a magnetic…

Strongly Correlated Electrons · Physics 2009-11-10 H. Meskine , S. Satpathy

Exotic quantum phases, arising from a complex interplay of charge, spin, lattice and orbital degrees of freedom, are of immense interest to a wide research community. A well-known example of such an entangled behavior is the Jahn-Teller…

The Jahn-Teller distortion, by its very nature, is often at the heart of the various electronic properties displayed by perovskites and related materials. Despite the Jahn-Teller mode being non- polar in nature, we devise and demonstrate in…

Materials Science · Physics 2016-02-10 Julien Varignon , Nicholas C. Bristowe , Philippe Ghosez

The Jahn-Teller effect is a fascinating and ubiquitous phenomenon in modern quantum physics and chemistry. We propose a class of oxides with melilite structure Ba$_2$TGe$_2$O$_7$ (T=V,Ni) where Jahn-Teller distortions are the main…

Materials Science · Physics 2015-08-03 Paolo Barone , Kunihiko Yamauchi , Silvia Picozzi

We investigate the halide perovskite TiF$_3$, renowned for its intricate interplay between structure, electronic correlations, magnetism, and thermal expansion. Despite its simple structure, understanding its low-temperature magnetic…

Strongly Correlated Electrons · Physics 2023-11-23 Gayanath W. Fernando , Donal Sheets , Jason Hancock , Arthur Ernst , R. Matthias Geilhufe
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