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Simulating strongly correlated systems in two dimensions is notoriously challenging due to rapid entanglement growth and frustration. Here, we introduce the adaptive projected-purified pseudoboson density-matrix renormalization group…

Strongly Correlated Electrons · Physics 2026-02-17 Fabian J. Pauw , Thomas Köhler , Ulrich Schollwöck , Sebastian Paeckel

We reveal limitations of several standard coupled-cluster (CC) methods with perturbation-theorybased noniterative or approximate iterative treatments of triple excitations when applied to thedetermination of highly accurate potential energy…

Chemical Physics · Physics 2021-10-04 Jan Schnabel , Lan Cheng , Andreas Köhn

A new method that accurately describes strongly correlated states and captures dynamical correlation is presented. It is derived as a modification of coupled-cluster theory with single and double excitations (CCSD) through consideration of…

Chemical Physics · Physics 2013-07-15 Daniel Kats , Frederick R. Manby

The similarity renormalization group (SRG) has been successfully applied to soften interactions for ab initio nuclear calculations. In almost all practical applications in nuclear physics, an SRG generator with the kinetic energy operator…

Nuclear Theory · Physics 2014-09-10 Nuiok M. Dicaire , Conor Omand , Petr Navratil

Introducing low-energy effective Hamiltonians is usual to grasp most correlations in quantum many-body problems. For instance, such effective Hamiltonians can be treated at the mean-field level to reproduce some physical properties of…

Quantum Gases · Physics 2025-01-09 Raphaël Photopoulos , Antoine Boulet

The (T) and [T] perturbative corrections are derived for multicomponent coupled-cluster theory with single and double excitations (CCSD). Benchmarking shows that multicomponent CCSD methods that include the perturbative corrections are more…

Chemical Physics · Physics 2022-07-01 Dylan Fowler , Kurt R. Brorsen

A practical high-accuracy relativistic method of atomic structure calculations for univalent atoms is presented. The method is rooted in the coupled-cluster formalism and includes non-perturbative treatment of single and double excitations…

Atomic Physics · Physics 2009-11-11 Sergey G. Porsev , Andrei Derevianko

We present an alternative approach to decompose non-negative tensors, called many-body approximation. Traditional decomposition methods assume low-rankness in the representation, resulting in difficulties in global optimization and target…

Machine Learning · Statistics 2023-10-31 Kazu Ghalamkari , Mahito Sugiyama , Yoshinobu Kawahara

Many binary systems of interest for gravitational-wave astronomy are orbited by a third distant body, which can considerably alter their relativistic dynamics. Precision computations are needed to understand the interplay between…

General Relativity and Quantum Cosmology · Physics 2023-02-22 Adrien Kuntz , Francesco Serra , Enrico Trincherini

We present an efficient implementation of a one-step relativistic second-order multireference perturbation theory based on the multireference driven similarity renormalization group (MR-DSRG) using the exact two-component (X2C) Hamiltonian,…

Chemical Physics · Physics 2026-05-13 Zijun Zhao , Francesco A. Evangelista

We extend the self-consistent Green's functions formalism to take into account three-body interactions. We analyze the perturbative expansion in terms of Feynman diagrams and define effective one- and two-body interactions, which allows for…

Nuclear Theory · Physics 2013-12-03 Arianna Carbone , Andrea Cipollone , Carlo Barbieri , Arnau Rios , Artur Polls

We discuss renormalization of the non-relativistic three-body problem with short-range forces. The problem becomes non-perturbative at momenta of the order of the inverse of the two-body scattering length, and an infinite number of graphs…

Nuclear Theory · Physics 2009-10-31 P. F. Bedaque , H. -W. Hammer , U. van Kolck

We apply degenerate many-body perturbation theory at high orders for the ab-initio description of ground states and excitation spectra of open-shell nuclei using soft realistic nucleon-nucleon interactions. We derive a recursive formulation…

Nuclear Theory · Physics 2012-11-30 Joachim Langhammer , Robert Roth , Christina Stumpf

We introduce a non-iterative energy correction, added on top of the rank-reduced coupled-cluster method with single, double, and triple substitutions, that accounts for excitations excluded from the parent triple excitation subspace. The…

Chemical Physics · Physics 2022-01-06 Michał Lesiuk

We employ correlated realistic nucleon-nucleon interactions for the description of nuclear ground states throughout the nuclear chart within the Hartree-Fock approximation. The crucial short-range central and tensor correlations, which are…

Nuclear Theory · Physics 2007-05-23 R. Roth , P. Papakonstantinou , N. Paar , H. Hergert , T. Neff , H. Feldmeier

The accuracy at which total energies of open-shell atoms and organic radicals may be calculated is assessed for selected coupled cluster perturbative triples expansions, all of which augment the coupled cluster singles and doubles (CCSD)…

Chemical Physics · Physics 2016-05-17 Janus Juul Eriksen , Devin A. Matthews , Poul Jørgensen , Jürgen Gauss

Coupled-cluster theories can be used to compute ab initio electronic correlation energies of real materials with systematically improvable accuracy. However, the widely-used coupled cluster singles and doubles plus perturbative triples…

Materials Science · Physics 2024-03-01 Nikolaos Masios , Andreas Irmler , Tobias Schäfer , Andreas Grüneis

Correlations play a crucial role in the nuclear many-body problem. We give an overview of recent developments in nuclear structure theory aiming at the description of these interaction-induced correlations by unitary transformations. We…

Nuclear Theory · Physics 2010-06-08 Robert Roth , Thomas Neff , Hans Feldmeier

A reliable and efficient computation of the entire single-particle spectrum of correlated molecules is an outstanding challenge in the field of quantum chemistry, with standard density functional theory approaches often giving an inadequate…

Chemical Physics · Physics 2021-10-08 Oliver J. Backhouse , Alejandro Santana-Bonilla , George H. Booth

In the last decade, the quantum chemical version of the density matrix renormalization group (DMRG) method has established itself as the method of choice for calculations of strongly correlated molecular systems. Despite its favourable…

Chemical Physics · Physics 2016-11-15 Libor Veis , Andrej Antalík , Jiří Brabec , Frank Neese , Örs Legeza , Jiří Pittner