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We present general expressions for the magnetic transition rates in beam Electron Paramagnetic Resonance (EPR) experiments of anisotropic spin systems in the solid state. The expressions apply to general spin centers and arbitrary…

Mesoscale and Nanoscale Physics · Physics 2015-01-14 Joscha Nehrkorn , Alexander Schnegg , Karsten Holldack , Stefan Stoll

Electron-spin resonance carried out with scanning tunneling microscopes (ESR-STM) is a recently developed experimental technique that is attracting enormous interest on account of its potential to carry out single-spin on-surface resonance…

Mesoscale and Nanoscale Physics · Physics 2023-04-19 Santiago A. Rodríguez , Sergio S. Gómez , Joaquín Fernández-Rossier , Alejandro Ferrón

W-band ({\nu} ca. 94 GHz) electron paramagnetic resonance (EPR) spectroscopy was used for a single-crystal study of a star-shaped Fe3Cr single-molecule magnet (SMM) with crystallographically imposed trigonal symmetry. The high resolution…

Mesoscale and Nanoscale Physics · Physics 2013-09-13 L. Sorace , M. -E. Boulon , P. Totaro , A. Cornia , J. Fernandes-Soares , R. Sessoli

Electron spin resonance scanning tunneling microscopy (ESR-STM) has become a powerful tool for probing spin dynamics and coherence of individual atoms and molecules on surfaces. In this work, we perform Rabi oscillation and Hahn echo pulse…

Mesoscale and Nanoscale Physics · Physics 2026-03-30 Paul Greule , Wantong Huang , Máté Stark , Kwan Ho Au-Yeung , Christoph Wolf , Soo-hyon Phark , Andreas J. Heinrich , Philip Willke

The recent development of all-electrical electron spin resonance (ESR) in a scanning tunneling microscope (STM) setup has opened the door to vast applications. Despite the fast growing number of experimental works on STM-ESR, the…

Mesoscale and Nanoscale Physics · Physics 2019-07-17 J. Reina Gálvez , C. Wolf , F. Delgado , N. Lorente

Lattices of odd-layered two-dimensional (2D) transition metal dichalcogenides (TMDs) such as WSe2 are non-centrosymmetric, and thus could possess linear piezoelectricity that is attractive for applications such as nanoelectromechanical…

Materials Science · Physics 2018-08-10 Ehsan Nasr Esfahani , Terrance Li , Bevin Huang , Xiaodong Xu , Jiangyu Li

Electron paramagnetic resonance (EPR) spectroscopy interrogates unpaired electron spins in solids and liquids to reveal local structure and dynamics; for example, EPR has elucidated parts of the structure of protein complexes that have…

Other Condensed Matter · Physics 2012-05-08 S. Takahashi , L. -C. Brunel , D. T. Edwards , J. van Tol , G. Ramian , S. Han , M. S. Sherwin

We report the detection of electron spin resonance (ESR) in individual dimers of the stable free radical 2,2,6,6-tetramethyl-piperidine-1-oxyl (TEMPO). ESR is measured by the current fluctuations in a scanning tunnelling microscope (ESR-STM…

Mesoscale and Nanoscale Physics · Physics 2023-05-25 Yishay Manassen , Moamen Jbara , Michael Averbukh , Zion Hazan , Carsten Henkel , Baruch Horovitz

Coherent spin resonance methods such as nuclear magnetic resonance (NMR) and electron spin resonance (ESR) spectroscopy have led to spectrally highly sensitive, non-invasive quantum imaging techniques with groundbreaking applications in…

We address the problem of electronic and nuclear spin resonance of an individual atom on a surface driven by a scanning tunnelling microscope. Several mechanisms have been proposed so far, some of them based on the modulation of exchange…

Mesoscale and Nanoscale Physics · Physics 2019-12-25 Alejandro Ferrón , Santiago A. Rodríguez , Sergio S. Gómez , Jose L. Lado , Joaquín Fernández-Rossier

We present a state interaction spin-orbit coupling method to calculate electron paramagnetic resonance (EPR) $g$-tensors from density matrix renormalization group wavefunctions. We apply the technique to compute $g$-tensors for the…

Chemical Physics · Physics 2018-07-17 Elvira R. Sayfutyarova , Garnet K. -L. Chan

Recent radio frequency scanning tunneling spectroscopy (rf-STS) experiments have demonstrated nuclear and electron spin excitations up to $\pm12\hbar$ in a single molecular spin quantum dot (qudot). Despite the profound experimental…

We study theoretically Electron Paramagentic Resonance (EPR) linewidths for single crystals of the molecular magnets Fe$_8$ and Mn$_{12}$ as functions of energy eigenstates $M_s$, frequency, and temperature when a magnetic field along the…

Condensed Matter · Physics 2009-11-07 Kyungwha Park , M. A. Novotny , N. S. Dalal , S. Hill , P. A. Rikvold

Electrically detected electron spin resonance (ESR) is used to study the hyperfine interaction of the two-dimensional electrons and the nuclei of the host lattice in a GaAs/AlGaAs heterostructure. Under the microwave and radio- frequency…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Chris Hillman , H. W. Jiang

Integrated magnetic sensors that allow simultaneous EPR and magnetization measurements have been developed to study single molecule magnets. A high frequency microstrip resonator has been integrated with a micro-Hall effect magnetometer.…

Materials Science · Physics 2009-11-11 G. de Loubens , G. D. Chaves , A. D. Kent , C. Ramsey , E. del Barco , C. Beedle , D. N. Hendrickson

The electron paramagnetic resonance (EPR) linewidths of B acceptors in Si are found to reduce dramatically in isotopically purified 28Si single crystals. Moreover, extremely narrow substructures in the EPR spectra are visible corresponding…

Localized surface plasmon resonance (LSPR) excitation of nanostructures and charge transfer in plasmonic nanocavities plays a central role in nanoscale optoelectronics and in applications for plasmonic devices. However, the direct…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Shuyi Liu , Martin Wolf , Takashi Kumagai

Paramagnetic magnetic resonance, a powerful technique for characterizing and identifying chemical targets, is increasingly used for imaging; however, low spin polarization at room temperature and moderate magnetic fields poses challenges…

Mesoscale and Nanoscale Physics · Physics 2019-09-04 C. M. Purser , V. P. Bhallamudi , C. S. Wolfe , H. Yusuf , B. A. McCullian , C. Jayaprakash , M. E. Flatté , P. C. Hammel

Spin-valve based nanojunctions incorporating Co|Ni multilayers with perpendicular anisotropy were used to study spin-torque driven ferromagnetic resonance (ST-FMR) in a nonlinear regime. Perpendicular field swept resonance lines were…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 W. Chen , G. de Loubens , J-M. L. Beaujour , J. Z. Sun , A. D. Kent

Recent advances in increasing the spectroscopic energy resolution in scanning tunneling microscopy (STM) have been achieved by integrating electron spin resonance (ESR) with STM. Here, we demonstrate the design and performance of a…