Related papers: Plasmonic Purcell Effect in Organic Molecules
We theoretically explore the notion of nonreciprocal near-zone manipulation of electromagnetic fields within subwavelength plasmonic nanostructures embedded in magneto-optical materials. We derive an analytical model predicting a strong,…
A surrounding electromagnetic environment can engineer spontaneous emissions from quantum emitters through the Purcell effect. For instance, a plasmonic antenna can efficiently confine an electromagnetic field and enhance the fluorescent…
Strong optical nonreciprocity at the nanoscale, relying on extreme one-way modes and backscattering suppression, can enable fundamentally new approaches in optoelectronics and plasmonics. Of special interest is achieving nonreciprocity in…
In the regime of strong coupling between molecular excitons and confined optical modes, the intra-molecular degrees of freedom are profoundly affected, leading to a reduced vibrational dressing of polaritons compared to bare electronically…
In this work, we introduce an elastic analog of the Purcell effect and show theoretically that spherical nanoparticles can serve as tunable and robust antennas for modifying the emission from localized elastic sources. This effect can be…
The Purcell effect - the modification of the spontaneous emission rate in presence of resonant cavities or other resonant objects - is a fundamental effect of quantum electrodynamics. However, a change of the emission rate caused by…
We show a break down of the conventional partition of optical states into its radiative and non-radiative parts. Large divergence of experimental observations from current theory in the case of emitters interacting with fully absorbing…
Ultrafast pump-probe measurements of plasmonic nanostructures probe the non-equilibrium behavior of excited carriers, which involves several competing effects obscured in typical empirical analyses. Here we present pump-probe measurements…
We study the effect of the electromagnetic environment on the resonance frequency of plasmonic excitations in dimers of interacting metallic nanoparticles. The coupling between plasmons and vacuum electromagnetic fluctuations induces a…
The vast majority of proteins are intrinsically fluorescent in the ultraviolet, thanks to the emission from their tryptophan and tyrosine amino-acid constituents. However, the protein autofluorescence quantum yields are generally very low…
Strong coupling between molecules and quantized fields has emerged as an effective methodology to engineer molecular properties. New hybrid states are formed when molecules interact with quantized fields. Since the properties of these…
Since Purcell's seminal report 75 years ago, electromagnetic resonators have been used to control light-matter interactions to make brighter radiation sources and unleash unprecedented control over quantum states of light and matter.…
X-ray scattering at the carbon absorption edge is uniquely sensitive to local molecular bond identity and orientation in organic nanostructures, encoded as a function of photon energy and polarization. However, quantitative analysis is…
Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is…
We derive a new expression for the two-photon spontaneous emission (TPSE) rate of an excited quantum emitter in the presence of arbitrary bodies in its vicinities. After investigating the influence of a perfectly conducting plate on the…
Electrically connected and plasmonically enhanced molecular junctions combine the optical functionalities of high field confinement and enhancement (cavity function), and of high radiative efficiency (antenna function) with the electrical…
Surface waves on a thin metal filament are described in terms of quantum electrodynamics. The interaction of surface waves with a quantum oscillator is discussed in the dipole approximation. The increase in the spontaneous emission rate of…
We describe the possibility of drastically boosting the spontaneous emission of a collection of two-level quantum emitters by embedding them in an epsilon-near-zero (ENZ) environment, consisting of a plasmonic waveguide operated at cut-off.…
Nanoplasmonics exploits the coupling between light and collective electron density oscillations (plasmons) to bypass the stringent limits imposed by diffraction. This coupling enables confinement of light to sub-wavelength volumes and is…
Plasmonic nanoparticles resonantly couple to and confine light below the diffraction limit. This mechanism has enabled a modern renaissance in optical materials, with potential applications ranging from sensing and circuitry to renewable…