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The atomistic mechanisms occurring during the processes of aging and rejuvenation in glassy materials involve very small structural rearrangements that are extremely difficult to capture experimentally. Here we use in-situ X-ray diffraction…

Density functional theory (DFT) was employed to study the stress-strain behavior, elastic instabilities, and metallization during a solid-solid phase transformation (PT) between semiconducting Si I (cubic A4) and metallic Si II (tetragonal…

Materials Science · Physics 2018-10-24 Nikolai A. Zarkevich , Hao Chen , Valery I. Levitas , Duane D. Johnson

Pressure-induced phase transitions in orthovanadates have led to interesting physical phenomena. The observed transitions usually involve large volume collapses and drastic changes in the electronic and vibrational properties of the…

Materials Science · Physics 2020-07-30 Daniel Errandonea

High pressure behavior of potassium chlorate (KClO$_3$) has been investigated from 0-10 GPa by means of first principles density functional theory (DFT) calculations. The calculated ground state parameters, transition pressure and phonon…

Materials Science · Physics 2015-06-17 N. Yedukondalu , Vikas D. Ghule , G. Vaitheeswaran

The superconducting transition in the layered organic compound \alpha-(BEDT-TTF)_2KHg(SCN)_4 has been studied in the two hydrostatic pressure regimes where a charge-density wave is either present or completely suppressed. Within the…

Superconductivity · Physics 2016-08-31 D. Andres , M. V. Kartsovnik , W. Biberacher , K. Neumaier , E. Schuberth , H. Mueller

As a new class of two-dimensional (2D) materials, 2D covalent organic frameworks (COFs) are proven to possess remarkable electronic and magnetic properties. However, their mechanical behaviours remain almost unexplored. In this work, taking…

Mesoscale and Nanoscale Physics · Physics 2018-12-26 Jin Zhang

We examine the phase behavior of a quasi-one-dimensional system of hard squares with side-length $\sigma$, where the particles are confined between two parallel walls and only nearest neighbor interactions occur. As in our previous work…

Statistical Mechanics · Physics 2017-05-03 Peter Gurin , Gerardo Odriozola , Szabolcs Varga

The compression of arsenolite (cubic As2O3) has been studied from a joint experimental and theoretical point of view. Experimental X-ray diffraction and Raman scattering measurements of this molecular solid at high pressures with different…

In this work we describe the thermodynamics and mechanism of CO$_2$ polymorphic transitions under pressure from form I to form III combining standard molecular dynamics, well-tempered metadynamics and committor analysis. We find that the…

Materials Science · Physics 2017-10-11 Ilaria Gimondi , Matteo Salvalaglio

a-Quartz surfaces functionalized with hydroxyl and methyl groups provide a versatile platform for controlling interfacial properties critical to applications such as catalysis, protective coatings, and energy conversion. The arrangement of…

Silicate frameworks exhibit diverse structural responses under extreme conditions, which are strongly influenced by hydration. Here, we present a comparative high-pressure synchrotron X-ray diffraction study of Na2ZrSi2O7 and its hydrated…

First-principles calculations have been carried out to study the InVO4 compound under pressure. In this work, total energy calculations were performed in order to analyze the structural behavior of the experimentally known polymorphs of…

At high pressure, the typical behavior of elements dictated by the periodic table - including oxidation numbers, stoichiometries in compounds, and reactivity, to name but a few - is altered dramatically. As pressure is applied, the…

Materials Science · Physics 2022-05-11 Katerina P. Hilleke , Tiange Bi , Eva Zurek

The physicochemical behavior of elements and compounds is heavily altered by high pressure. The occurrence of pressure-induced reactions and phase transitions can be revealed by crystal structure prediction approaches. In this work, we…

Materials Science · Physics 2016-03-09 Gabriele Saleh , Artem R. Oganov

Carbon at extreme conditions is the focus of intensive scientific inquiry due to its importance for applications in inertial confinement fusion experiments and for understanding the interior structure of carbon-rich exoplanets. The extreme…

Materials Science · Physics 2022-11-21 Ashley S. Williams , Kien Nguyen-Cong , Jonathan T. Willman , Ivan I. Oleynik

Structural phase transitions accompanied by incommensurate and commensurate charge density wave (CDW) modulations of unconventional nature have been reported in BaNi$_2$As$_2$, a nonmagnetic cousin of the parent compound of Fe-based…

We have studied the structural behavior of bismuth phosphate under compression. We performed x-ray powder diffraction measurements up to 31.5 GPa and ab initio calculations. Experiments were carried out on different polymorphs; trigonal…

We report the experimental study of the structural transition of a stable complex plasma crystal to a solid-liquid phase coexistence by the controlled adjustment of the confinement potential, while keeping all other parameters constant. The…

Plasma Physics · Physics 2023-10-06 S. Jaiswal , Connor Belt , Anton Kananovich , E. M. Aguirre

We develop a statistical physics theory for solid-solid phase transitions in which a metamaterial undergoes longitudinal contraction in response to increase in external tension. Such transitions, which are forbidden in thermodynamic…

Statistical Mechanics · Physics 2013-05-16 Zachary G. Nicolaou , Adilson E. Motter

Disorder-induced ordering and unprecedentedly high radiation tolerance in $\gamma$-phase of gallium oxide is a recent spectacular discovery at the intersection of the fundamental physics and electronic applications. Importantly, by far,…

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