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We present time-resolved X-ray diffraction measurements using advanced timing schemes that provide high temporal resolution while also maintaining a high flux in the X-ray probe beam. The method employs patterned probe pulse sequences that…

Dynamical diffraction effects in single crystals produce highly monochromatic parallel X-ray beams with a mutual separation of a few micrometer and a time-delay of a few fs -the so-called echoes. This ultrafast diffraction effect is used at…

Dispersive Fourier transformation is a powerful technique in which the spectrum of an optical pulse is mapped into a time-domain waveform using chromatic dispersion. It replaces a diffraction grating and detector array with a dispersive…

Optics · Physics 2009-11-13 Keisuke Goda , Kevin K. Tsia , Bahram Jalali

This paper describes the demonstration of linearly polarized picosecond pulse shaping with variable profiles including symmetric and non-symmetric intensity distributions. Important characteristics such as stability and transmission were…

Optics · Physics 2019-01-21 Fangming Liu , Senlin Huang , Kexin Liu , Shukui Zhang

Time-dependent diffusion behavior is probed over sub-millisecond timescales in a single shot using an NMR static gradient, time-incremented echo train acquisition (SG-TIETA) framework. The method extends the Carr-Purcell-Meiboom-Gill (CPMG)…

Quantitative Methods · Quantitative Biology 2021-03-18 Teddy X. Cai , Nathan H. Williamson , Velencia J. Witherspoon , Rea Ravin , Peter J. Basser

We present a method for a complete characterization of a femtosecond ultraviolet pulse when a fundamental near-infrared beam is also available. Our approach relies on generation of second harmonic from the pre-characterized fundamental,…

Optics · Physics 2009-07-09 Marcin Kacprowicz , Wojciech Wasilewski , Konrad Banaszek

Instruments to visualize transient structural changes of inhomogeneous materials on the nanometer scale with atomic spatial and temporal resolution are demanded to advance materials science, bioscience, and fusion sciences. One such…

Accelerator Physics · Physics 2017-03-20 X. Shen , R. K. Li , U. Lundström , T. J. Lane , A. H. Reid , S. P. Weathersby , X. J. Wang

Ultrashort burst laser pulses serve as powerful tools for precise laser processing, broadband ultrafast spectroscopy, and high-speed laser-scanning microscopy. However, the performance of conventional burst pulse generators is limited by…

We introduce a new method for generation of the phase screen samples with arbitrary spatial spectrum: Sparse Spectrum with uniform wave vectors (SU). Similar to the known Sparse Spectrum (SS) technique, it uses trigonometric series with…

Image and Video Processing · Electrical Eng. & Systems 2019-12-03 Mikhail Charnotskii

We exploit a slightly noncollinear second-harmonic cross-correlation scheme to map the 3D space-time intensity distribution of an unknown complex-shaped ultrashort optical pulse. We show the capability of the technique to reconstruct both…

The temporal characterization of ultrafast laser pulses has become a cornerstone capability of ultrafast optics laboratories and is routine both for optimizing laser pulse duration and designing custom fields. Beyond pure temporal…

Optics · Physics 2020-10-28 Spencer W. Jolly , Olivier Gobert , Fabien Quéré

Microspectrometer features remarkable portability and integration, and is prospected to provide quick detection tools to daily life and revolutionary techniques to researchers. For the extremely finite footprint, microspectrometer can…

"Single-shot" ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics using chirped probe pulses is analyzed theoretically. FDSS has an advantage over pump-probe spectroscopy in a situation where the "noise"…

Optics · Physics 2007-05-23 Ilya A. Shkrob , Stanislas Pommeret

The recently developed information-theoretic approach to crystallographic symmetry classifications and quantifications in two dimensions (2D) from digital transmission electron and scanning probe microscope images is adapted for the…

Materials Science · Physics 2022-08-10 Peter Moeck , Lukas von Koch

Ultrafast single-shot imaging techniques now reach frame rates of tens of tera-frame-per-second (Tfps) and long sequence depths but are often too complex for large-scale use, both in terms of image acquisition and reconstruction. We propose…

We demonstrate a dispersive measurement pulse shaping technique that allows for arbitrarily fast quantum non-demolition, single-quadrature measurements of non-linear systems and unconditionally leaves the measurement resonator empty. For…

Quantum Physics · Physics 2018-09-13 Felix Motzoi , Lukas Buchmann , Christian DIckel

The low repetition rates and possible shot-to-shot variations in laser-plasma studies place a high value on single-shot diagnostics. For example, white-beam scattering methods based on broadband backlighter x-ray sources are used to…

Plasma Physics · Physics 2014-03-04 O. R. Hoidn , G. T. Seidler

Single-shot supercontinuum spectral interferometry (SSSI) is an optical technique that can measure ultrafast transients in the complex index of refraction. This method uses chirped supercontinuum reference/probe pulses that need to be…

Instrumentation and Detectors · Physics 2018-06-05 DinhDuy Tran Vu , Dogeun Jang , Ki-Yong Kim

Four-dimensional scanning transmission electron microscopy (4D-STEM) enables mapping of diffraction information with nanometer-scale spatial resolution, offering detailed insight into local structure, orientation, and strain. However, as…

X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…