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Using a three-dimensional quasiclassical technique we explore the double ionization pathways of a diatomic molecule driven by an intense infrared (800nm) ultrashort laser pulse. For intensities corresponding to the tunneling regime, we find…

Atomic Physics · Physics 2009-02-26 Agapi Emmanouilidou

The development of high-intensity ultrashort laser pulses unlocks the potential of pump-probe spectroscopy in sub-femtosecond timescale. Notably, subcycle pump pulses can generate electronic states unreachable by conventional multicycle…

Strongly Correlated Electrons · Physics 2025-06-17 Kazuya Shinjo , Shigetoshi Sota , Seiji Yunoki , Takami Tohyama

Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Ofer Neufeld , Nicolas Tancogne-Dejean , Umberto De Giovannini , Hannes Hübener , Angel Rubio

We report the breakdown of the electric dipole approximation in the long-wavelength limit in strong-field ionization with linearly polarized few-cycle mid-infrared laser pulses at intensities on the order of 10$^{13}$ W/cm$^2$.…

Atomic Physics · Physics 2014-12-16 A. Ludwig , J. Maurer , B. W. Mayer , C. R. Phillips , L. Gallmann , U. Keller

The strong-field control of plasmonic nanosystems opens up new perspectives for nonlinear plasmonic spectroscopy and petahertz electronics. Questions, however, remain regarding the nature of nonlinear light-matter interactions at…

We present a detailed comparison of strong-field ionization of diatomic molecules and their companion atoms with nearly equal ionization potentials. We perform calculations in the length and velocity gauge formulations of the molecular…

Atomic Physics · Physics 2009-11-10 Thomas Kim Kjeldsen , Lars Bojer Madsen

A mechanism of light transmission through metallic films is proposed, assisted by tunnelling between resonating buried dielectric inclusions. This is illustrated by arrays of Si spheres embedded in Ag. Strong transmission peaks are observed…

Other Condensed Matter · Physics 2009-11-13 F. J. Garcia de Abajo , G. Gomez-Santos , L. A. Blanco , A. G. Borisov , S. V. Shabanov

We report on the unambiguous observation of the sub-cycle ionization bursts in sequential strong-field double ionization of H$_2$ and their disentanglement in molecular frame photoelectron angular distributions. This observation was made…

Quantized nano-objects offer a myriad of exciting possibilities for manipulating electrons and light that impact photonics, nanoelectronics, and quantum information. In this context, ultrashort laser pulses combined with nanotips and field…

This work models the propagation of an optical pulse in a 4-level atomic system in the electromagnetic induced transparency regime. By demonstrating that linear and nonlinear optical properties can be externally controlled and tailored by a…

Optics · Physics 2018-10-11 Nuno A. Silva , André L. Almeida , A. Guerreiro

We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show…

We measure the emission of energetic electrons from the interaction between ultrashort laser pulses and a solid density plasma in the relativistic regime. We detect an electron beam that only appears with few-cycle pulses (< 10 fs) and…

Plasma Physics · Physics 2018-06-04 N. Zaïm , F. Böhle , M. Bocoum , A. Vernier , S. Haessler , X. Davoine , L. Videau , J. Faure , R. Lopez-Martens

The dynamic processes in the surface layers of metals subjected activity of a pulsing laser irradiation, which destroyed not the crystalline structure in details surveyed. The procedure of calculation of a dislocation density generated in…

Materials Science · Physics 2009-11-07 A. E. Pogorelov , K. P. Ryaboshapka , A. F. Zhuravlyov

The interaction of metal-molecule-metal junctions with light is considered within a simple generic model. We show, for the first time, that light induced current in unbiased junctions can take place when the bridging molecule is…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan

Using extreme-ultraviolet attosecond-pulse-trains, we investigate the photoionization dynamics of a Helium atom in the presence of moderately-strong (~10^12 W/cm^2) femtosecond laser pulses. The electronic structure of a laser-dressed atom…

Atomic Physics · Physics 2011-08-02 Niranjan Shivaram , Henry Timmers , Xiao-Min Tong , Arvinder S. Sandhu

We report on the development of an ultrafast Transmission Electron Microscope based on a laser-driven cold-field emission source. We first describe the instrument before reporting on numerical simulations of the laser-driven electron…

Optics · Physics 2019-11-27 G. M. Caruso , F. Houdellier , S. Weber , M. Kociak , A. Arbouet

We investigate laser induced nonsequential multiple ionization using a simple statistical model in which an electron recollides inelastically with its parent ion. In this collision, it thermalizes with the remaining $N-1$ bound electrons…

Atomic Physics · Physics 2007-05-23 C. Figueira de Morisson Faria , X. Liu

We report on the observation of subcycle interferences of electron wave packets released during the strong field ionization of H$_2$ with cycle-shaped two-color laser fields. With a reaction microscope, channel-resolved photoelectron…

Chemical Physics · Physics 2016-12-08 Xinhua Xie , Stefan Roither , Daniil Kartashov , Li Zhang , Andrius Baltuška , Markus Kitzler

We demonstrate that strong-field ionization of atoms driven by circularly polarized light becomes an adiabatic process when described in the frame rotating with the laser field. As a direct consequence, a conservation law emerges: in the…

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen