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Superionic conductors, or solid-state ion-conductors surpassing 0.01 S/cm in conductivity, can enable more energy dense batteries, robust artificial ion pumps, and optimized fuel cells. However, tailoring superionic conductors require…

Instrumentation and Detectors · Physics 2024-07-23 Kim H. Pham , Scott K. Cushing

The processes of ionization and energy transfer in a quantum system composed of two distant H atoms with an initial internuclear separation of 100 atomic units (5.29 nm) have been studied by the numerical solution of the time-dependent…

Quantum Physics · Physics 2017-09-13 Guennaddi K. Paramonov , Andre D. Bandrauk , Oliver Kühn

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…

We propose a theory of optically-induced currents in dielectrics and wide-gap semiconductors exposed to a non-resonant ultrashort laser pulse with a stabilized carrier-envelope phase. In order to describe strong-field electron dynamics,…

Materials Science · Physics 2016-08-05 Stanislav Yu. Kruchinin , Michael Korbman , Vladislav S. Yakovlev

Technological advancements in generation of ultrafast and intense laser pulses have enabled the real-time observation and control of charge migration in molecules on their natural timescale, which ranges from few femtoseconds to several…

Optics · Physics 2025-02-25 Sucharita Giri

Theoretical study on H$_2^+$ in an intense infrared laser field on the attosecond time-scale reveals that the molecular ion shows multiple bursts of ionization within a half-cycle of the laser field oscillation, in contrast to the widely…

Chemical Physics · Physics 2010-12-10 Norio Takemoto , Andreas Becker

Electromagnetically induced transparency in an optically thick, cold medium creates a unique system where pulse-propagation velocities may be orders of magnitude less than $c$ and optical nonlinearities become exceedingly large. As a…

Quantum Physics · Physics 2009-11-10 Danielle A. Braje , Vlatko Balic , G. Y. Yin , S. E. Harris

The quantum tunneling time remains the subject of heated debate, and one of its most curious features is faster-than-light or superluminal tunneling. Our tunnel-ionization model of the time-delay, presented in previous work, shows good…

Quantum Physics · Physics 2026-02-24 Ossama Kullie , Igor A. Ivanov

Superluminal tunneling of light through a barrier has attracted broad interest in the last several decades. Despite the observation of such phenomena in various systems, it has been under intensive debate whether the transmitted light truly…

Optics · Physics 2021-04-06 Liang Wu , Zhiyong Wang , Kai Kang1 , Yi Fu , Chuanwei Li1 , Weili Zhang , Shuang Zhang

Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…

Optics · Physics 2018-03-21 Yuya Morimoto , Peter Baum

Quantum calculations of a 1+1-dimensional model for double ionization in strong laser fields are used to trace the time evolution from the ground state through ionization and rescattering to the two electron escape. The subspace of…

Atomic Physics · Physics 2009-11-13 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

We report on the non-adiabatic offset of the initial electron momentum distribution in the plane of polarization upon single ionization of argon by strong field tunneling and show how to experimentally control the degree of…

Ionization of hydrogen-like ions by intense, circularly polarized laser pulses is analyzed under the scope of the relativistic strong-field approximation. We show that, for specific parameters of the laser field, the energy spectra of…

Atomic Physics · Physics 2016-12-30 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

Using a three-dimensional quasiclassical technique we explore molecular double ionization by a linearly polarized, infrared (800~nm) 27~fs laser pulse. For intensities ranging from the tunneling to the over-the-barrier regime, we identify…

Atomic Physics · Physics 2011-01-27 A. Emmanouilidou , D. S. Tchitchekova

We study strong-field molecular ionization as a function of pulse duration. Experimental measurements of the photoelectron yield for a number of molecules reveal competition between different ionization continua (cationic states) which…

The absorption of a single photon that excites a quantum system from a low to a high energy level is an elementary process of light-matter interaction, and a route towards realizing pure single-photon absorption has both fundamental and…

Quantum Physics · Physics 2017-05-08 Chuan-Cun Shu , Daoyi Dong , Ian R. Petersen , Niels E. Henriksen

We propose a method for slowing particles by laser fields that potentially has the ability to generate large forces without the associated momentum diffusion that results from the random directions of spontaneously scattered photons. In…

Atomic Physics · Physics 2020-10-21 John P. Bartolotta , Jarrod T. Reilly , Murray J. Holland

Resonant Raman excitation by ultrafast vacuum ultraviolet laser pulses is a powerful means to study electron dynamics in molecules, but experiments must contend with linear background ionization: frequencies high enough to reach resonant…

Chemical Physics · Physics 2015-06-23 S. Miyabe , P. Bucksbaum

The response time of the electron to light in photoemission is difficult to define and measure. Tunneling ionization of atoms, a strong-laser-induced photoemission process, provides a semiclassical case for visiting the problem. Here, we…

Atomic Physics · Physics 2022-12-20 C. Chen , J. Y. Che , W. Y. Li , S. Wang , X. J. Xie , J. Y. Huang , Y. G. Peng , G. G. Xin , Y. J. Chen

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…