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Yb-based magnets, with a perfect triangular lattice of pseudospin-$1/2$ Yb$^{3+}$ ions, have emerged as candidates for realizing a quantum spin-liquid state, with NaYbS$_2$ being a prominent example. Here we present the solid-solution…

Strongly Correlated Electrons · Physics 2022-06-09 Ellen Häußler , Jörg Sichelschmidt , Michael Baenitz , Eric C. Andrade , Matthias Vojta , Thomas Doert

We introduce the rare-earth delafossite compound TlYbSe$_2$ -- extending the search for quantum spin liquids in frustrated triangular lattice magnets. While the DC magnetisation suggests magnetic exchange interactions in the order of…

Strongly Correlated Electrons · Physics 2025-09-16 Bishnu P. Belbase , Arjun Unnikrishnan , Shi Feng , Eun Sang Choi , Johannes Knolle , Arnab Banerjee

Quantum spin liquids~(QSLs) represent a unique quantum disordered state of matter that hosts long-range quantum entanglement and fractional excitations. However, structural disorder resulting from site mixing between different types of ions…

We study fermionic quantum spin liquids (QSLs) on the three-dimensonal trillium lattice of corner-sharing triangles. We are motivated by recent experimental and theoretical investigations that have explored various classical and quantum…

Strongly Correlated Electrons · Physics 2024-09-05 Ming-Hao Li , Sounak Biswas , S. A. Parameswaran

High-quality single crystals of NaYbSe$_2$, which resembles a perfect triangular-lattice antiferromagnet without the intrinsic disorder, are investigated by magnetization and specific heat, as well as the local probe techniques nuclear…

A quantum spin liquid (QSL) is an exotic quantum state of matter characterized by fluctuating spins which may exhibit long-range entanglement. Among the possible host candidates for a QSL ground state, the $S$=1/2 kagome lattice…

The quantum spin liquid (QSL) is an exotic phase of magnetic materials where the spins continue to fluctuate without any symmetry breaking down to zero temperature. Among the handful reports of QSL with spin $S\ge$1, examples with magnetic…

YbMgGaO$_{4}$, a structurally perfect two-dimensional triangular lattice with odd number of electrons per unit cell and spin-orbit entangled effective spin-1/2 local moments of Yb$^{3+}$ ions, is likely to experimentally realize the quantum…

Strongly Correlated Electrons · Physics 2015-10-20 Yuesheng Li , Gang Chen , Wei Tong , Li Pi , Juanjuan Liu , Zhaorong Yang , Xiaoqun Wang , Qingming Zhang

We investigated the spin dynamics by electron spin resonance (ESR) of the Yb-based, effective spin-1/2 delafossites NaYbO$_{2}$, AgYbO$_{2}$, LiYbS$_{2}$, NaYbS$_{2}$, and NaYbSe$_{2}$ which all show an absence of magnetic order down to…

Strongly Correlated Electrons · Physics 2020-11-17 Jörg Sichelschmidt , Burkhard Schmidt , Philipp Schlender , Seunghyun Khim , Thomas Doert , Michael Baenitz

Quantum spin liquid (QSL) represents a new class of condensed matter states characterized by the long-range many-body entanglement of topological orders. The most prominent feature of the elusive QSL state is the existence of fractionalized…

Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS$_2$. At low temperatures, it features an effective spin-$\frac{1}{2}$ state due to the combined effect of crystal electric field and spin…

Strongly Correlated Electrons · Physics 2020-04-22 K. M. Ranjith , Ph. Schlender , Th. Doert , M. Baenitz

Recent experiments indicate that Na$_4$Ir$_3$O$_8$, a material in which s=1/2 iridium local moments form a three dimensional network of corner-sharing triangles, may have a quantum spin liquid ground state with gapless spin excitations.…

Strongly Correlated Electrons · Physics 2009-11-13 Michael Lawler , Arun Paramekanti , Yong Baek Kim , Leon Balents

Quantum spin liquids (QSLs) host emergent, fractionalized fermionic excitations that are charge-neutral. Identifying clear experimental signatures of these excitations remains a central challenge in the field of strongly correlated systems,…

Strongly Correlated Electrons · Physics 2025-12-04 Penghao Zhu , Archisman Panigrahi , Leonid Levitov , Nandini Trivedi

The most fascinating feature of certain two-dimensional (2D) gapless quantum spin liquid (QSL) is that their spinon excitations behave like the fermionic carriers of a paramagnetic metal. The spinon Fermi surface is then expected to produce…

Strongly Correlated Electrons · Physics 2020-09-17 N. Li , Q. Huang , X. Y. Yue , W. J. Chu , Q. Chen , E. S. Choi , X. Zhao , H. D. Zhou , X. F. Sun

The search for quantum spin liquids (QSL) and chemical doping in such materials to explore superconductivity have continuously attracted intense interest. Here, we report the discovery of a potential QSL candidate, pyrochlore-lattice…

Yb- and Ce-based delafossites were recently identified as effective spin-1/2 antiferromagnets on the triangular lattice. Several Yb-based systems, such as NaYbO2, NaYbS2, and NaYbSe2, exhibit no long-range order down to the lowest measured…

The delafossite-like compound NaYbO$_2$ hosts a triangular lattice of Yb$^{3+}$ moments and is a promising candidate for the realization of a quantum spin liquid ground state -- an exotic, quantum-disordered magnetic phase featuring…

Polycrystalline samples of NaYbO$_2$ are investigated by bulk magnetization and specific-heat measurements, as well as by nuclear magnetic resonance (NMR) and electron spin resonance (ESR) as local probes. No signatures of long-range…

Strongly Correlated Electrons · Physics 2019-05-08 K. M. Ranjith , D. Dmytriieva , S. Khim , J. Sichelschmidt , S. Luther , D. Ehlers , H. Yasuoka , J. Wosnitza , A. A. Tsirlin , H. Kühne , M. Baenitz

Platelike high-quality NaYbS$_{2}$ rhombohedral single crystals with lateral dimensions of a few mm have been grown and investigated in great detail by bulk methods like magnetization and specific heat, but also by local probes like nuclear…

The rare-earth-based geometrically frustrated triangular magnets have attracted considerable attention due to the intricate interplay between strong spin-orbit coupling and the crystal electric field (CEF), which often leads to effective…