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Two techniques that employ equally spaced trains of optical pulses to map an optical high frequency into a low frequency modulation of the signal that can be detected in real time are compared. The development of phase-stable optical…

Quantum Physics · Physics 2017-08-22 Kochise Bennett , Jeremy Rouxel , Shaul Mukamel

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

Optics · Physics 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

Terahertz (THz) frequency combs (TFCs) are promising for numerous applications in spectroscopy, metrology, sensing, and wireless communications. However, the practical applications of TFCs have been hindered thus far by the need for…

Applied Physics · Physics 2025-11-27 Feifan Han , Xiongbin Yu , Qun Zhang , Zebin Huang , Longhao Zou , Weichao Li , Jingpu Duan , Zhen Gao , Xiaofeng Tao

Quantum cascade lasers (QCLs) are high-power coherent light sources in the midinfrared and terahertz parts of the electromagnetic spectrum. They are devices in which the electronic and lattice systems are far from equilibrium, strongly…

Mesoscale and Nanoscale Physics · Physics 2021-06-16 Y. B. Shi , S. Mei , O. Jonasson , I. Knezevic

We demonstrate the performance of a dual frequency comb QCL spectrometer for the application of vibrational Stark spectroscopy. Measurements performed on fluorobenzene with the dual-comb spectrometer (DCS) were compared to results obtained…

Chemical Physics · Physics 2019-11-22 Urszula Szczepaniak , Samuel H. Schneider , Raphael Horvath , Jacek Kozuch , Markus Geiser

For the growing demand of frequency combs in mid-infrared (mid-IR), known as the "molecular fingerprint" region of the spectrum [1], down conversion of near-IR frequency combs through half- harmonic generation offers numerous benefits…

Optics · Physics 2015-10-14 Alireza Marandi , Kirk A. Ingold , Marc Jankowski , Robert L. Byer

Frequency combs based on nonlinear-optical phenomena in integrated photonics are a versatile light source that can explore new applications, including frequency metrology, optical communications, and sensing. We demonstrate robust…

Frequency combs, specialized laser sources emitting multiple equidistant frequency lines, have revolutionized science and technology with unprecedented precision and versatility. Recently, integrated frequency combs are emerging as scalable…

Dual comb spectroscopy allows for high-resolution spectra to be measured over broad bandwidths, but an essential requirement for coherent integration is the availability of a phase reference. Usually, this means that the combs' phase and…

Optics · Physics 2016-06-01 David Burghoff , Yang Yang , Qing Hu

Quantum frequency combs from chip-scale integrated sources are promising candidates for scalable and robust quantum information processing (QIP). However, to use these quantum combs for frequency domain QIP, demonstration of entanglement in…

Optical frequency comb, with precisely controlled spectral lines spanning a broad range, has been the key enabling technology for many scientific breakthroughs. In addition to the traditional implementation based on modelocked lasers,…

Optics · Physics 2023-01-02 Mingming Nie , Yijun Xie , Bowen Li , Shu-Wei Huang

Fourier-transform spectroscopy is an indispensable tool for analyzing chemical samples in scientific research as well as chemical and pharmaceutical industries. Recently, its measurement speed, sensitivity, and precision have been shown to…

Optics · Physics 2025-05-06 Takuro Ideguchi , Tasuku Nakamura , Yohei Kobayashi , Keisuke Goda

Fast (sub-second) spectroscopy with high spectral resolution is of vital importance for revealing quantum chemistry kinetics of complex chemical and biological reactions. Fourier transform (FT) spectrometers can achieve high spectral…

Integrated microresonator facilitates the realization of quantum frequency comb (QFC), which provides a large number of discrete frequency modes with broadband spectral range and narrow linewidth. However, all previous demonstrations have…

Quantum Physics · Physics 2024-04-19 Wenjun Wen , Wenhan Yan , Chi Lu , Liangliang Lu , Xiaoyu Wu , Yanqing Lu , Shining Zhu , Xiao-song Ma

Optical frequency combs based on mode-locked lasers have revolutionised the field of metrology and precision spectroscopy by providing precisely calibrated optical frequencies and coherent pulse trains. Amplification of the pulsed output…

Atomic Physics · Physics 2014-01-17 Jonas Morgenweg , Itan Barmes , Kjeld S. E. Eikema

We report on the operation of a 50 mW continuous wave quantum cascade laser (QCL) in the 9.2 micrometer range, phase locked to a single mode CO2 laser with a tunable frequency offset. The wide free running emission spectrum of the QCL (3-5…

Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously…

We report the first experimental demonstration of frequency-locking of an extended-cavity quantum-cascade-laser (EC-QCL) to a near-infrared frequency comb. The locking scheme is applied to carry out absolute spectroscopy of N2O lines near…

Instrumentation and Detectors · Physics 2018-11-29 Marco Lamperti , Bidoor Alsaif , Davide Gatti , Martin Fermann , Paolo Laporta , Aamir Farooq , Marco Marangoni

We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an…

Dual-comb spectroscopy (DCS) utilizes a pair of broadband mutually coherent laser frequency combs to enable high-resolution, high-accuracy spectroscopic measurements with atomic-clock-level frequency referencing, and rapid, multiplexed…

Optics · Physics 2025-10-01 D. Konnov , A. Muraviev , K. L. Vodopyanov