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In this work, control over the precise state emitted by quantum cascade laser frequency combs through strong radio-frequency current modulation close to their repetition frequency is demonstrated. In particular, broadening of the spectrum…

A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…

Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

We propose and characterize experimentally a new source of optical frequency combs for performing multi-heterodyne spectrometry. This comb modality is based on a frequency shifting loop seeded with a CW monochromatic laser. The comb lines…

Optics · Physics 2018-07-04 V. Duran , C. Schnebelin , H. Guillet De Chatellus

Infrared spectroscopy is a powerful tool for basic and applied science. The molecular spectral fingerprints in the 3 um to 20 um region provide a means to uniquely identify molecular structure for fundamental spectroscopy, atmospheric…

We demonstrate a two-photon interference experiment for phase coherent biphoton frequency combs (BFCs), created through spectral amplitude filtering of biphotons with a continuous broadband spectrum. By using an electro-optic phase…

In this work, we systematically investigate the optical feedback dynamics of terahertz (THz) frequency combs generated from quantum cascade lasers (QCLs) using the effective semiconductor Maxwell-Bloch equations (ESMBEs). Starting from a…

Optics · Physics 2025-12-04 Xiaoqiong Qi , Carlo Silvestri , Thomas Taimre , Aleksandar D. Rakic

Real-time measurement of the absolute frequency of continuous-wave terahertz (CW-THz) waves is required for characterization and frequency calibration of practical CW-THz sources. We proposed a method for real-time monitoring of the…

Optical frequency combs have emerged as a cornerstone for a wide range of areas, including spectroscopy, ranging, optical clocks, time and frequency transfer, waveform synthesis, and communications. However, quantum mechanical fluctuations…

Quantum Physics · Physics 2024-12-30 Abdulkarim Hariri , Shuai Liu , Haowei Shi , Quntao Zhuang , Xudong Fan , Zheshen Zhang

We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…

Instrumentation and Detectors · Physics 2024-12-03 Francis Hindle , Alexandra Khabbaz , Anthony Roucou , Jean-Francois Lampin , Gaël Mouret

Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…

Atomic Physics · Physics 2018-06-13 Bachana Lomsadze , Steven T. Cundiff

Mode-resolved dual-comb spectroscopy (DCS) is an emerging spectroscopic tool with the potential to simultaneously achieve a broad spectral coverage and ultrahigh spectral resolution in terahertz (THz) spectroscopy. However, the need for two…

Instrumentation and Detectors · Physics 2020-06-02 Jie Chen , Kazuki Nitta , Xin Zhao , Takahiko Mizuno , Takeo Minamikawa , Francis Hindle , Zheng Zheng , Takeshi Yasui

Mid-wave infrared (MIR, 3--5 $\mu$m) optical frequency combs (OFC) are of critical importance for spectroscopy of fundamental molecular absorption features in space and terrestrial applications. Although in this band OFCs can be obtained…

Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the…

The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…

Optics · Physics 2023-07-19 Vicente Duran , Santiago Tainta , Victor Torres-Company

Recently, there has been a growing interest in integrated THz photonics for various applications in communications, spectroscopy and sensing. We present a new integrated photonic platform based on active and passive elements integrated in a…

While being invented for precision measurement of single atomic transitions, frequency combs have also become a versatile tool for broadband spectroscopy in the last years. In this paper we present a novel and simple approach for broadband…

Harmonic frequency combs, in which the lasing modes are separated by a period of tens of free spectral ranges from each other, have been recently discovered in quantum cascade lasers (QCLs). There is an ongoing debate how the harmonic combs…

Optics · Physics 2020-08-05 Yongrui Wang , Alexey Belyanin

Hyperspectral imaging provides spatially resolved spectral information. Utilising dual frequency combs as active illumination sources, hyperspectral imaging with ultra-high spectral resolution can be implemented in a scan-free manner when a…

The mid-infrared spectral range (2 to 20 \mu m) is of particular importance for chemistry, biology and physics as many molecules exhibit strong ro-vibrational fingerprints. Frequency combs - broad spectral bandwidth coherent light sources…

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