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Entangled photon pairs are predicted to linearize and increase the efficiency of two-photon absorption, allowing continuous wave laser diodes to drive ultrafast time-resolved spectroscopy and nonlinear processes. Despite a range of…

Quantum Physics · Physics 2022-05-31 Bryce P. Hickam , Manni He , Nathan Harper , Szilard Szoke , Scott Cushing

The use of entangled photons in an imaging system can exhibit effects that cannot be mimicked by any other two-photon source, whatever the strength of the correlations between the two photons. We consider a two-photon imaging system in…

Quantum Physics · Physics 2009-11-07 Ayman F. Abouraddy , Bahaa E. A. Saleh , Alexander V. Sergienko , Malvin C. Teich

Entangled photons, generated by spontaneous parametric down-conversion from a second-order nonlinear crystal, present a rich potential for imaging and image-processing applications. Since this source is an example of a three-wave mixing…

Quantum Physics · Physics 2015-06-26 Ayman F. Abouraddy , Bahaa E. A. Saleh , Alexander V. Sergienko , Malvin C. Teich

Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that…

Quantum Physics · Physics 2021-08-25 Stefan Lerch , André Stefanov

Two-photon absorption (TPA) and other nonlinear interactions of molecules with time-frequency-entangled photon pairs (EPP) has been predicted to display a variety of fascinating effects. Therefore, their potential use in practical…

Quantum Physics · Physics 2021-09-15 Michael G. Raymer , Tiemo Landes , Andrew H. Marcus

Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

Most experimental demonstrations of entanglement require nonclassical states and correlated measurements of single-photon detection events. It is shown here that entanglement can produce a large decrease in the rate of two-photon absorption…

Quantum Physics · Physics 2009-11-11 J. D. Franson

Over the last 50 years entangled photon pairs have received attention for use in lowering the flux in two-photon absorption imaging and spectroscopy. Despite this, evidence for entangled two-photon absorption (ETPA) effects remain highly…

Quantum light is increasingly recognized as a promising resource for developing optical measurement techniques. Particular attention has been paid to enhancing the precision of the measurements beyond classical techniques by using…

Chemical Physics · Physics 2023-10-03 Yuta Fujihashi , Kuniyuki Miwa , Masahiro Higashi , Akihito Ishizaki

Correlations between entangled photons are a key ingredient for testing fundamental aspects of quantum mechanics and an invaluable resource for quantum technologies. However, scattering from a dynamic medium typically scrambles and averages…

Quantum Physics · Physics 2024-06-05 Mamoon Safadi , Ohad Lib , Ho-Chun Lin , Chia Wei Hsu , Arthur Goetschy , Yaron Bromberg

Entanglement can modify light-matter interaction effects and, conversely, these interactions can change the non-classical correlations present in the system. We present an example where these mutual connections can be discussed in a simple…

Quantum Physics · Physics 2018-12-26 Pedro Sancho

The study of entangled states has greatly improved the basic understanding about two-photon interferometry. Two-photon interference is not the interference of two photons but the result of superposition among indistinguishable two-photon…

Quantum Physics · Physics 2009-11-10 Giuliano Scarcelli , Alejandra Valencia , Yanhua Shih

Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…

Optics · Physics 2021-07-07 Szilard Szoke , Manni He , Bryce P. Hickam , Scott K. Cushing

We consider a photonic crystal (PC) doped with four-level atoms whose intermediate transition is coupled near-resonantly with a photonic band-gap edge. We show that two photons, each coupled to a different atomic transition in such atoms,…

Quantum Physics · Physics 2009-11-06 David Petrosyan , Gershon Kurizki

The non-classical spectral and temporal features of entangled photons offer new possibilities to investigate the interactions of excitons in photosynthetic complexes, and to target the excitation of specific states. Simulations of…

Quantum Physics · Physics 2012-11-05 Frank Schlawin , Konstantin Dorfman , Benjamin P. Fingerhut , Shaul Mukamel

Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

Two-photon processes are crucial in applications like microscopy and microfabrication, but their low cross-section requires intense illumination and limits, e.g., the penetration depth in nonlinear microscopy. Entangled states have been…

Entangled two-photon absorption (ETPA) could form the basis of nonlinear quantum spectroscopy at very low photon fluxes, since, at sufficiently low photon fluxes, ETPA scales linearly with the photon flux. When different pairs start to…

Quantum Physics · Physics 2023-12-04 Frank Schlawin

Quantum information science is driving progress in a vast number of scientific and technological areas that cover molecular spectroscopy and matter-light interactions in general. In these fields, the ability to generate quantum…

Quantum Physics · Physics 2023-03-02 M Wittkop , Juan M. Marmolejo-Tejada , Martín A. Mosquera

Entangled photon pairs -- discrete light quanta that exhibit non-classical correlations -- play a crucial role in quantum information science (for example in demonstrations of quantum non-locality and quantum cryptography). At the…

Quantum Physics · Physics 2009-11-07 Antia Lamas-Linares , John C. Howell , Dik Bouwmeester
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