Related papers: Entangled light-matter interactions and spectrosco…
Plasmonics and metamaterials have recently been shown to allow the control and interaction with non-classical states of light, a rather counterintuitive finding given the high losses typically encountered in these systems. Here, we…
Nonlinear spectroscopy and microscopy techniques are ubiquitous in a wide range of applications across physics and biology. However, these usually rely on high-powered pulsed laser systems. A promising alternative is to exploit entangled…
Quantum light spectroscopy, providing novel molecular information non-accessible by classical light, necessitates new computational tools when applied for complex molecular systems. We introduce two computational protocols for the molecular…
We describe two-photon absorption processes excited by entangled pairs, but not by non-entangled pairs of the same energy and polarization. Photon states are selected for destructive interference in the non-entangled process between…
Entangled photons can be used to make measurements with an accuracy beyond that possible with classical light. While most implementations of quantum metrology have used states made up of a single colour of photons, we show that entangled…
Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…
Optical signals obtained by the material response to classical laser fields are given by nonlinear response functions which can be expressed by sums over various quantum pathways of matter. We show that some pathways can be selected by…
Recent investigations suggest that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of…
Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…
Multiparticle entangled states generated via interaction between narrow-band light and an ensemble of identical two-level atoms are considered. Depending on the initial photon statistics, correlation between atoms and photons can give rise…
Quantum entangled photons provide a sensitive probe of many-body interactions and offer an unique experimental portal for quantifying many-body correlations in a material system. In this paper, we present a theoretical demonstration of how…
Quantum mechanics predicts microscopic phenomena with undeniable success. Nevertheless, current theoretical and experimental efforts still do not yield conclusive evidence that there is, or not, a fundamental limitation on the possibility…
Recent theoretical and experiments have explored the use of entangled photons as a spectroscopic probe of material systems. We develop here a theoretical description for entropy production in the scattering of an entangled biphoton state…
Energy-time entangled photon holes are shown to be relatively insensitive to photon loss due to absorption by atoms whose coherence times are longer than the time delays typically employed in nonlocal interferometry (a fraction of a…
Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…
We study the dynamics of quantum matter interacting with time-energy entangled photons. We consider the stimulation of a collective mode of a two-dimensional material by means of one of the two partners of a time-energy entangled pair of…
Single--photon which is initially uncorrelated with atom, will evolve to be entangled with the atom on their continuous kinetic variables in the process of resonant scattering. We find the relations between the entanglement and their…
High-dimensional quantum entanglement is an important resource for emerging quantum technologies such as quantum communication and quantum computation. The scalability of metres-long experimental setups limits high-dimensional entanglement…
The ability to detect the interaction of light and matter at the single-particle level is becoming increasingly important for many areas of science and technology. The absorption or emission of a photon on a narrow transition of a trapped…
In this paper the coherence and crossing symmetry of the electromagnetic interaction of photons involved in the spontaneous parametric down conversion (SPDC) phenomena in nonlinear crystals, are investigated. On this basis a new…