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Despite several different measures of efficiency that are applicable to the photosynthetic systems, a precise degree of efficiency of these systems is not completely determined. Introducing an efficient model for the dynamics of…

Chemical Physics · Physics 2020-06-24 Fatemeh Ghasemi , Afshin Shafiee

Coherent generation of indistinguishable single photons is crucial for many quantum communication and processing protocols. Solid-state realizations of two-level atomic transitions or three-level spin-$\Lambda$ systems offer significant…

Mesoscale and Nanoscale Physics · Physics 2019-12-03 Zhe-Xian Koong , Dale Scerri , Markus Rambach , Ted S. Santana , Suk-In Park , Jin D. Song , Erik M. Gauger , Brian D. Gerardot

Noise-assisted transport in quantum systems occurs when quantum time-evolution and decoherence conspire to produce a transport efficiency that is higher than what would be seen in either the purely quantum or purely classical cases. In…

Quantum Physics · Physics 2012-08-30 Ivan Kassal , Alán Aspuru-Guzik

Floquet engineering, while a powerful tool for ultrafast quantum-state manipulation, faces challenges under strong-field conditions, as recent high harmonic generation studies unveil exceptionally short dephasing times. In this study, using…

Charge separation in light-harvesting complexes occurs in a pair of tightly coupled chlorophylls at the heart of photosynthetic reaction centers of both plants and bacteria. Recently it has been shown that quantum coherence can, in…

Biological Physics · Physics 2016-11-28 M. Qin , H. Z Shen , X. X. Yi

We investigate the quantum dynamics of energy and charge transfer in a wheel-shaped artificial photosynthetic antenna-reaction center complex.This complex consists of six light-harvesting chromophores and an electron-acceptor fullerene. To…

Biological Physics · Physics 2015-05-28 Pulak Kumar Ghosh , Anatoly Yu. Smirnov , Franco Nori

We utilize the novel non-Markovian quantum jump (NMQJ) approach to stochastically simulate exciton dynamics derived from a time-convolutionless master equation. For relevant parameters and time scales, the time-dependent, oscillatory…

Quantum Physics · Physics 2009-12-07 Patrick Rebentrost , Rupak Chakraborty , Alan Aspuru-Guzik

Coherent transport of excitations along chains of coupled quantum systems represents an interesting problem with a number of applications ranging from quantum optics to solar cell technology. A convenient tool for studying such processes…

Quantum Physics · Physics 2016-02-16 Martin Stefanak , Jaroslav Novotny , Igor Jex

We present an approach using quantum walks (QWs) to redistribute ultracold atoms in an optical lattice. Different density profiles of atoms can be obtained by exploiting the controllable properties of QWs, such as the variance and the…

Quantum Physics · Physics 2008-08-13 C. M. Chandrashekar , Raymond Laflamme

The photosynthetic reaction center of plants and bacteria is an extremely efficient energy to charge conversion device. Solar photons create excitons in the pigment molecules. These excitons are then transferred to the reaction center where…

Biological Physics · Physics 2018-12-11 Vishvendra Singh Poonia

We study the evolution of quantum entanglement during exciton energy transfer (EET) in a network model of the Fenna-Matthews-Olson (FMO) complex, a biological pigment-protein complex involved in the early steps of photosynthesis in sulphur…

Quantum Physics · Physics 2010-06-29 Filippo Caruso , Alex W. Chin , Animesh Datta , Susana F. Huelga , Martin B. Plenio

Quantum coherence offers potential for energy conversion technologies. It influences light absorption and emission, affecting energy conversion limits and efficiency. As a result, quantum coherence is being harnessed to boost performance in…

Quantum Physics · Physics 2026-02-13 Ludovica Donati , Francesco Saverio Cataliotti , Stefano Gherardini

First-order perturbation theory and many-body Green function analysis are used to quantify the influence of size, surface reconstruction and surface treatment on exciton transport between small silicon quantum dots. Competing radiative…

Mesoscale and Nanoscale Physics · Physics 2011-11-01 Zhibin Lin , Huashan Li , Alberto Franceschetti , Mark T. Lusk

We investigate the role of quantum coherence in the efficiency of excitation transfer in a ring-hub arrangement of interacting two-level systems, mimicking a light-harvesting antenna connected to a reaction center as it is found in natural…

Quantum Physics · Physics 2009-11-13 Alexandra Olaya-Castro , Chiu Fan Lee , Francesca Fassioli Olsen , Neil F. Johnson

Coherent quantum phenomena can only emerge when decoherence is minimized, and mastery over decoherence is technologically crucial for designing and operating functional quantum devices. However, its microscopic mechanisms in…

Mesoscale and Nanoscale Physics · Physics 2026-04-01 Xian-Peng Zhang , Yan-Qing Feng , Haiwen Liu , Wanxiang Feng , Yugui Yao

The long-standing problem of nearly perfect photosynthetic yield in some types of bacteria and nearly all kinds of plants despite the interaction with a hot and noisy environment has witnessed quantum optical explanations in the last decade…

Quantum Physics · Physics 2022-08-24 Zibo Wang , Antonio V. Lim , Imran M. Mirza

Inspired by the classical phenomenon of random walk, the concept of quantum walk has emerged recently as a powerful platform for the dynamical simulation of complex quantum systems, entanglement production and universal quantum computation.…

We review recent theoretical calculations of quantum entanglement in photosynthetic light harvesting complexes. These works establish, for the first time, a manifestation of this characteristically quantum mechanical phenomenon in…

Quantum Physics · Physics 2010-12-21 K. Birgitta Whaley , Mohan Sarovar , Akihito Ishizaki

Phonon interactions in solid-state photonics systems cause intrinsic quantum decoherence and often present the limiting factor in emerging quantum technology. Due to recent developments in nanophotonics, exciton-cavity structures with very…

Quantum Physics · Physics 2021-01-04 Emil V. Denning , Matias Bundgaard-Nielsen , Jesper Mork

In this work we study the first step in photosynthesis for the limiting case of a single photon interacting with photosystem II (PSII). We model our system using quantum trajectory theory, which allows us to consider not only the average…

Biological Physics · Physics 2022-08-10 Robert L. Cook , Liwen Ko , K. Birgitta Whaley