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We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…

Quantum Physics · Physics 2009-11-05 Jan Roden , Alexander Eisfeld , Wolfgang Wolff , Walter T. Strunz

Several recent studies of energy transfer in photosynthetic light harvesting complexes have revealed a subtle interplay between coherent and decoherent dynamic contributions to the overall transfer efficiency in these open quantum systems.…

Quantum Physics · Physics 2015-05-14 Mohan Sarovar , Yuan-Chung Cheng , K. Birgitta Whaley

Coherent optical manipulation of electronic bandstructures via Floquet Engineering is a promising means to control quantum systems on an ultrafast timescale. However, the ultrafast switching on/off of the driving field comes with questions…

A vibronic exciton model is developed to investigate the origin of long lived coherences in light-harvesting complexes. Using experimentally determined parameters and uncorrelated site energy fluctuations, the model predicts oscillations in…

Biological Physics · Physics 2012-06-07 Niklas Christensson , Harald F. Kauffmann , Tonu Pullerits , Tomas Mancal

The light-harvesting is a problem of long interest. It becomes active again in recent years stimulated by suggestions of quantum effects in energy transport. Recent experiments found evidence that BChla 1 and BChla 6 are the first to be…

Biological Physics · Physics 2015-06-04 B. Cui , X. X. Yi , C. H. Oh

We have prepared and detected quantum coherences with long dephasing times at the level of single trapped cesium atoms. Controlled transport by an "optical conveyor belt" over macroscopic distances preserves the atomic coherence with slight…

We describe a method for simulating exciton dynamics in protein-pigment complexes, including effects from charge transfer as well as fluorescence. The method combines the hierarchical equations of motion, which are used to describe quantum…

Chemical Physics · Physics 2022-11-23 Thomas P. Fay , David T. Limmer

We propose an implementation of a quantum walk on a circle on an optomechanical system by encoding the walker on the phase space of a radiation field and the coin on a two-level state of a mechanical resonator. The dynamics of the system is…

Quantum Physics · Physics 2015-09-24 Jalil Khatibi Moqadam , Renato Portugal , Marcos Cesar de Oliveira

The resource theory of quantum thermodynamics has emerged as a powerful tool for exploring the out-of-equilibrium dynamics of microscopic and highly correlated systems. Recently, it has been employed in photoisomerization, a mechanism…

Quantum Physics · Physics 2024-12-19 Mattheus Burkhard , Onur Pusuluk , Tristan Farrow

Quantum walks in atomic systems, owing to their continuous nature, are especially well-suited for the simulation of many-body physics and can potentially offer an exponential speedup in solving certain black box problems. Photonics offers…

We investigate the lateral transport of excitons in ZnSe quantum wells by using time-resolved micro-photoluminescence enhanced by the introduction of a solid immersion lens. The spatial and temporal resolutions are 200 nm and 5 ps,…

Strongly Correlated Electrons · Physics 2009-11-07 Hui Zhao , B. Dal Don , S. Moehl , H. Kalt , K. Ohkawa , D. Hommel

Experimental/theoretical evidence for sustained vibration-assisted electronic (vibronic) coherence in the Photosystem II Reaction Center (PSII RC) indicates that photosynthetic solar-energy conversion might be optimized through the…

We derive transport equations for fermions and bosons in spatially or temporally varying backgrounds with special symmetries, by use of the Schwinger-Keldysh formalism. In a noninteracting theory the coherence information is shown to be…

High Energy Physics - Phenomenology · Physics 2014-11-18 Matti Herranen , Kimmo Kainulainen , Pyry M. Rahkila

Recent evidence of electronic coherence during energy transfer in photosynthetic antenna complexes has reinvigorated the discussion of whether coherence and/or entanglement has any practical functionality for these molecular systems. Here…

Quantum Physics · Physics 2015-03-13 Francesca Fassioli , Alexandra Olaya-Castro

A variety of open quantum networks are currently under intense examination to model energy transport in photosynthetic systems. Here we study the coherent transfer of a quantum excitation over a network incoherently coupled with a…

Quantum Physics · Physics 2015-03-18 Lorenzo Campos Venuti , Paolo Zanardi

Quantum walks are central to a wide range of applications such as quantum search, quantum information processing, and entanglement transport. Gaining control over the duration and the direction of quantum walks (QWs) is crucial to…

Understanding the pathways taken by a quantum particle during a transport process is an enormous challenge. There are broadly two different aspects of the problem that affect the route taken. First is obviously the couplings between the…

Chemical Physics · Physics 2023-08-25 Amartya Bose , Peter L. Walters

The objective of this paper is to describe a simple phenomenological approach for including incoherent dephasing processes in quantum transport models. The presented illustrative numerical results show this model provides the flexibility of…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Roksana Golizadeh-Mojarad , Supriyo Datta

We investigate the dynamical properties of the two-bosons quantum walk in system with different degrees of coherence, where the effect of the coherence on the two-bosons quantum walk can be naturally introduced. A general analytical…

Quantum Physics · Physics 2019-08-15 Li-Hua Lu , Shan Zhu , You-Quan Li

Quantum synchronisation has recently been proposed as a mechanism for electronic excitation energy transfer in light-harvesting complexes, yet its robustness in driven-dissipative settings remains under active investigation. Here, we…

Biological Physics · Physics 2026-01-30 Wenhao Xu