Related papers: Singlet fission for quantum information and quantu…
In this work we study singlet fission in tetracene para-dimers, covalently linked by a phenyl group. In contrast to most previous works, we account for the full quantum dynamics of the combined excitonic and vibrational system. For our…
Two electrons in a quantum dot (QD) can form triplet states. We analyze the exchange coupling of the triplet states of the negatively charged exciton in a QD (X$^-$, two electrons and one hole) with the spin of a magnetic atom (Mn). Two…
Photons are the ideal carriers of quantum information for communication. Each photon can have a single qubit or even multiple qubits encoded in its internal quantum state, as defined by optical degrees of freedom such as polarization,…
A photonic process named as "quantum state joining" has been recently experimentally demonstrated [C. Vitelli et al., Nature Photon. 7, 521 (2013)] that corresponds to the transfer of the internal two-dimensional quantum states of two input…
We report the first theoretical calculations of excited state absorptions (ESAs) from the singlet and triplet excitons, as well as the key intermediate in the singlet fission (SF) process, the spin singlet multiexciton triplet-triplet…
Manipulation of spin states at the single-atom scale underlies spin-based quantum information processing and spintronic devices. Such applications require protection of the spin states against quantum decoherence due to interactions with…
A spin qubit in semiconductor quantum dots holds promise for quantum information processing for scalability and long coherence time. An important semiconductor qubit system is a double quantum dot trapping two electrons or holes, whose spin…
Probing extended polyene systems with energy in excess of the bright state ($1^1B_u^+$/$S_2$) band edge generates triplets via singlet fission. This process is not thought to involve the $2^1A_g^-$/$S_1$ state, suggesting that other states…
The electronic interaction between an optically active singlet state ($S_1S_0$) and a dark state of singlet multiplicity, known as correlated triplet pair ($^1[TT]$), plays a crucial role in the effective transformation from $S_1S_0$ to…
We use tunneling spectroscopy to study the evolution of few-electron spin states in parallel InAs nanowire double quantum dots (QDs) as a function of level detuning and applied magnetic field. Compared to the much more studied serial…
A quantum dot interacting with two resonant cavity modes is described by a two-mode Jaynes-Cummings model. Depending on the quantum dot energy level scheme, the interaction of a singly doped quantum dot with a cavity photon generates…
Detailed analysis of behavior of spin-entangled particle pairs under arbitrary rotations in their Hilbert space has been performed. It shows a rich range of varieties (faces) of entanglement in different bases. Analytic criteria are…
Singlet Fission (SF) into two triplets offers exciting avenues for high-efficiency photovoltaics and optically initializable qubits. While the chemical space of SF chromophores is ever-expanding, the mechanistic details of…
We investigate theoretically the spin splitting of the exciton states in semiconductor coupled quantum dots (CQDs) containing a single magnetic ion. We find that the spin splitting can be switched on/off in the CQDs \textit{via} the…
Singlet-triplet states in double quantum dots are promising realizations of qubits, and capacitive coupling can be used to create entanglement between these qubits. We propose an entangling three-qubit gate of singlet-triplet qubits in a…
We engineer a system of two strongly confined quantum dots to gain reproducible electrostatic control of the spin at zero magnetic field. Coupling the dots in a tight ring-shaped potential with two tunnel barriers, we demonstrate that an…
The ``entanglement of formation'' of a mixed state of a bipartite quantum system can be defined in terms of the number of pure singlets needed to create the state with no further transfer of quantum information. We find an exact formula for…
Studying the excited states of doublets is challenging for their typically multiconfigurational character. We employ light-scanning-tunneling microscopy (light-STM) to investigate photon-induced currents on a single open-shell PTCDA anion…
The development of a working quantum computer utilizing electron spin states as qubits is a major goal for many theorists and experimentalists. The future applications of quantum information technology would also require a reliable method…
Dispersively coupled distant qubits in a shared cavity can become entangled through virtual photon exchange with energy-conserving phase evolution of their quantum states. This interaction can potentially be accelerated by operating on…