Related papers: Singlet fission for quantum information and quantu…
We construct and analyze a two-dimensional frustrated quantum spin model with plaquette order, in which the low-energy dynamics is controlled by spin singlets. At a critical value of frustration the singlet spectrum becomes gapless,…
We apply an elementary measurement scheme to calculate the electronic triplet-singlet transition mediated by hyperfine interaction in a double quantum dot. We show how the local character of the hyperfine interaction and the nuclear…
We investigate theoretically the influence of strong light-matter coupling on the initial steps of the photo-triggered singlet-fission process. In particular we focus on intra-molecular singlet fission in a TIPS-pentacene dimer derivative…
Singlet fission, an exciton multiplication process in organic semiconductors which converts one singlet exciton into two triplet excitons is a promising way to reduce thermalization losses in conventional solar cells. One way to harvest…
Entangled photon pairs are key to many novel applications in quantum technologies. Semiconductor quantum dots can be used as sources of on-demand, highly entangled photons. The fidelity to a fixed maximally entangled state is limited by the…
For the theoretical screening of Singlet Fission (SF) rates in molecular aggregates, commonly dimer model systems are employed. However, there is experimental evidence, that the SF process proceeds from the $^{1}$(TT) state via an…
We show that spin-orbit coupling in a quantum dot molecule allows for coherent manipulation of two electron spin states using Raman transitions. Such two-electron spin states defined by the singlet and triplet states of two exchange coupled…
Singlet fission (SF) is an electronic transition that in the last decade has been under the spotlight for its applications in optoelectronics, from photovoltaics to spintronics. Despite considerable experimental and theoretical…
The mechanisms underlying coherent and thermally activated singlet exciton fission in pi-stacked acene crystals are clarified based on quantum dynamics simulations parameterized against a highly correlated description of the electronic…
Coupled pairs of nuclear spins-1/2 support one singlet state and three triplet states. Transitions between the singlet state and one of the triplet states may be driven by an oscillating low-frequency magnetic field, in the presence of…
We show that a singlet of many multi-level quantum systems arises naturally as the ground state of a physically-motivated Hamiltonian. The Hamiltonian simply exchanges the states of nearest-neighbours in some network of qudits (d-level…
We investigate theoretically the hyperfine-induced dephasing of two-electron-spin states in a double quantum dot with a finite singlet-triplet splitting J. In particular, we derive an effective pure dephasing Hamiltonian, which is valid…
Entanglement is the quintessential quantum phenomenon and a necessary ingredient in most emerging quantum technologies, including quantum repeaters, quantum information processing (QIP) and the strongest forms of quantum cryptography. Spin…
We present studies of thermal entanglement of a three-spin system in triangular symmetry. Spin correlations are described within an effective Heisenberg Hamiltonian, derived from the Hubbard Hamiltonian, with super-exchange couplings…
We describe our dynamical simulations of the excited states of the carotenoid, neurosporene, following its photoexcitation into the 'bright' (nominally $1^1B_u^+$) state. We employ the adaptive tDMRG method on the UV model of…
A holy grail of photonics research is the realization of a laser that uses a single quantum emitter as the gain medium. Such a device would exhibit a plethora of new features, including lasing without a well-defined threshold and output…
Quantum computing applications in diverse domains are emerging rapidly. Given the limitations of classical computing techniques, the peculiarity of quantum circuits, which can observe quantum phenomena such as superposition, entanglement,…
We study the low energy states of finite spin chains with isotropic (Heisenberg) and anisotropic (XY and Ising-like) exchange interaction with uniform and non-uniform coupling constants. We show that for an odd number of sites a spin…
We develop a powerful tree tensor network states method that is capable of simulating exciton-phonon quantum dynamics of larger molecular complexes and open quantum systems with multiple bosonic environments. We interface this method with…
We show how the spin independent scattering between two identical flying qubits can be used to implement an entangling quantum gate between them. We consider one dimensional models with a delta interaction in which the qubits undergoing the…