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Photoabsorption spectra of N$_2$ and CO were recorded at 900K, using the vacuum-ultraviolet Fourier-transform spectrometer at the DESIRS beamline of synchrotron SOLEIL. These high-temperature and high-resolution measurements allow for…

Using the Tunable Diode Laser Absorption Spectroscopy (TDLAS) 82 CH$_3$I ro-vibrational overtone absorption were detected for the first time between 11660 and 11840 cm$^{-1}$ (844 -- 857 nm), with strengths estimated to be around $10^{-27}$…

Chemical Physics · Physics 2023-04-14 Alessandro Lucchesini

We present the first precise frequency measurement of the 2$^{1}$S$_{0}$-3$^{1}$D$_{2}$ two-photon transition in $^{4}$He at 1009 nm. The laser source at 1009 nm is stabilized on an optical frequency comb to perform the absolute frequency…

Positronium and muonium, as purely leptonic atoms without internal structure, provide ideal systems for high-precision tests of quantum electrodynamics (QED) and measurements of fundamental constants. However, the high velocities of these…

We report the absolute frequency measurements of rubidium 5S-7S two-photon transitions with a cw laser digitally locked to an atomic transition and referenced to an optical frequency comb. The narrow, two-photon transition, 5S-7S (760 nm)…

We demonstrate a dual wavelength acousto-optic deflector (AOD) designed to deflect two wavelengths to the same angles by driving with two RF frequencies. The AOD is designed as a beam scanner to address two-photon transitions in a…

Quantum Physics · Physics 2012-06-05 Sangtaek Kim , Robert R. Mcleod , Mark Saffman , Kelvin H. Wagner

Vacuum-ultraviolet (VUV) photoabsorption spectra were recorded of the $A\,{}^2\Sigma^+(v'=0)\leftarrow{}X\,{}^2\Pi(v''=0)$, $D\,{}^2\Sigma^-(v'=0)\leftarrow{}X\,{}^2\Pi(v''=0)$ and $D\,{}^2\Sigma^-(v'=1)\leftarrow{}X\,{}^2\Pi(v''=0)$ bands…

In this paper, we introduce an all-fibered dual-comb spectrometer based on a new design of highly nonlinear fiber to efficiently convert frequency combs from 1.55 micron to 2 micron We show that our spectrometer can be used to measure…

The technique of dual modulation Faraday rotation spectroscopy has been applied for near shot-noise limited detection of HO2 at the exit of an atmospheric pressure flow reactor. This was achieved by combining direct current modulation at 51…

Optics · Physics 2015-06-17 Brian Brumfield , Wenting Sun , Yiguang Ju , Gerard Wysocki

We present absolute frequency measurement of the unperturbed P7 P7 O$_2$ B-band transition with relative standard uncertainty of $2\times10^{-11}$. We reached the level of accuracy typical for Doppler-free techniques, with Doppler-limited…

We demonstrate an efficient high-precision optical spectroscopy technique for single trapped ions with non-closed transitions. In a double-shelving technique, the absorption of a single photon is first amplified to several phonons of a…

The $3p^{4}$ $^{3}$P$_{J}$ - $3p^{3}4p$ $^{3}$P$_{J}$ transition in the sulphur atom is investigated in a precision two-photon excitation scheme under Doppler-free and collision-free circumstances yielding an absolute accuracy of 0.0009…

Atomic Physics · Physics 2020-06-23 K. -F. Lai , E. J. Salumbides , W. Ubachs

A novel mid-infrared/near-infrared double resonant absorption setup for studying infrared-inactive vibrational states is presented. A strong vibrational transition in the mid-infrared region is excited using an idler beam from a singly…

Chemical Physics · Physics 2016-07-21 J. Karhu , J. Nauta , M. Vainio , M. Metsälä , S. Hoekstra , L. Halonen

The nonlinear (NL) optical response of bulk lithium niobate (LiNbO$_3$) was investigated at 532 nm using the second harmonic of a Nd:YAG laser delivering pulses of 12 ps. The experiments were performed using the D4$\sigma$ method combined…

Optics · Physics 2023-11-30 Hongzhen Wang , Georges Boudebs , Cid de Araújo

We demonstrated the observation of Rb two-photon absorption directly excided by an optical frequency comb at fiber communication bands. A chain of comb spectral control is elaborately implemented to increase the power of the second harmonic…

Optics · Physics 2015-06-16 Jiutao Wu , Dong Hou , Xiaoliang Dai , Zhengyu Qin , Zhigang Zhang , Jianye Zhao

We report the observation and characterization of a high-contrast dual-frequency Doppler-free ground-state crossover resonance in the D1 line of 87Rb.The crossover appears at a two-photon detuning exceeding the natural linewidth of the…

A tunable far-infrared laser sideband spectrometer was used to investigate a nitric oxide sample enriched in 18O between 0.99 and 4.75 THz. Regular, electric dipole transitions were recorded between 0.99 and 2.52 THz, while magnetic dipole…

Astrophysics of Galaxies · Physics 2015-04-21 Holger S. P. Müller , Kaori Kobayashi , Kazumasa Takahashi , Kazuko Tomaru , Fusakazu Matsushima

We theoretically investigate the two-photon absorption spectrum of conventional s-wave superconductors. The calculation is carried out in the local limit at absolute zero. The direct excitation of quasiparticles is excluded under the…

Superconductivity · Physics 2015-10-26 Takanobu Jujo

Precise molecular transition frequencies are of great interest in the test of fundamental physics and also in various applications. Two well isolated ro-vibrational transitions of $^{12}$C$^{16}$O at 1.57 $\mu$m, R(9) and R(10) in the…

Atomic Physics · Physics 2017-10-11 Jin Wang , Yu R. Sun , Lei-Gang Tao , An-Wen Liu , Shui-Ming Hu

We have performed for the first time direct laser spectroscopy of the 1S0-3P0 optical clock transition at 265.6 nm in fermionic isotopes of neutral mercury laser-cooled in a magneto-optical trap. Spectroscopy is performed by measuring the…

Atomic Physics · Physics 2009-11-13 M. Petersen , R. Chicireanu , S. T. Dawkins , D. V. Magalhães , C. Mandache , Y. Lecoq , A. Clairon , S. Bize