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In the search for materials for quantum information science applications, colloidal semiconductor nanoplatelets (NPLs) have emerged as a highly promising new class of materials due to their interesting optical properties, such as narrow…

Lead halide perovskite nanocrystals are promising materials for classical and quantum light emission. To understand these outstanding properties, a thorough analysis of the band-edge exciton emission is needed which is not reachable in…

Mesoscale and Nanoscale Physics · Physics 2023-04-07 Mohamed-Raouf Amara , Zakaria Said , Caixia Huo , Aurélie Pierret , Christophe Voisin , Weibo Gao , Qihua Xiong , Carole Diederichs

Colloidal 2D semiconductor nanoplatelets are highly efficient light emitters, which exhibit large absorption and emission cross sections, and constitute promising laser gain media. However, if dispersed in solutions, such nanoplatelets lack…

Colloidal nanocrystals are unique optical gain materials due to their high intrinsic absorption, excellent quantum yield, and tunable emission. However, integration of colloidal nanocrystal solutions into photonic systems for lasing…

Using an approximate time-dependent density functional theory method, we calculate the absorption and luminescence spectra for hydrogen passivated silicon nanoscale structures with large aspect ratio. The effect of electron confinement in…

Materials Science · Physics 2009-09-27 Y. Wang , R. Q. Zhang , Th. Frauenheim , T. A. Niehaus

The in-plane coefficient of thermal expansion (CTE) for CdSe nanoplatelets with the zinc-blende structure containing from two to five monolayers is calculated from first principles within the quasiharmonic approximation. A comparison of the…

Materials Science · Physics 2019-08-14 Alexander I. Lebedev

Excitons -- quasiparticles formed by the binding of an electron and a hole through electrostatic attraction -- hold promise in the fields of quantum light confinement and optoelectronic sensing. Atomically thin transition metal…

Charge carrier dynamics essentially determine the performance of various optoelectronic applications of colloidal semiconductor nanocrystals. Among them, two-dimensional nanoplatelets provide new adjustment freedom for their unique…

Mesoscale and Nanoscale Physics · Physics 2023-02-20 Yige Yao , Xiaotian Bao , Yunke Zhu , Xinyu Sui , An Hu , Peng Bai , Shufeng Wang , Hong Yang , Xinfeng Liu , Yunan Gao

The electronic structure of CdSe/CdS core/shell seeded nanorods of experimentally relevant size is studied using a combination of molecular dynamics and semiempirical pseudopotential techniques, with the aim to address the transition from…

Materials Science · Physics 2015-06-16 Hagai Eshet , Michael Grunwald , Eran Rabani

2D magnetic semiconductor CrSBr exhibits unique magneto-optical properties, yet its electronic structure and photophysical mechanisms remain unclear at high magnetic field and low temperature. Through comprehensive spectroscopic…

Materials Science · Physics 2024-11-28 Xiaodong Shen , Jiajun Cao , Weizheng Liang , Borong Cong , Bao Ke , Jialong Zhao , Bingsuo Zou

We study the low-temperature magneto-photoluminescence (PL) from individual CdSe nanocrystals. Nanocrystals having a small "bright" exciton fine structure splitting ($<$0.5 meV) exhibit a conventional left- and right-circularly polarized…

Mesoscale and Nanoscale Physics · Physics 2009-03-04 H. Htoon , S. A. Crooker , M. Furis , S. Jeong , Al. L. Efros , V. I. Klimov

Surface traps and associated emission in quantum dots (QDs) sought a lot of research attention because of the fundamental interests apart from their influence on the emission characteristics. In ref [Acc. Chem. Res. Vol 43 (2) pp 190, 2010]…

Materials Science · Physics 2014-10-20 Sesha Vempati

Quantum dots acting as single photon emitters in the blue-green range are fabricated and characterized at cryogenic temperature. They consist in CdSe dots inserted in (Zn,Mg)Se nanowires with a thick shell. Photoluminescence spectra, decay…

A brief review is given of recent positron studies of metal and semiconductor nanocrystals. The prospects offered by positron annihilation as a sensitive method to access nanocrystal (NC) properties are described and compared with other…

Materials Science · Physics 2007-10-11 S. W. H. Eijt , B. Barbiellini , A. J. Houtepen , D. Vanmaekelbergh , P. E. Mijnarends , A. Bansil

Seeded CdSe/CdS nanorods exhibit intense polarized emission along the rod main axis. The degree of linear polarization cannot be explained by dielectric effects alone, an additional electronic contribution is present whose nature has not…

Mesoscale and Nanoscale Physics · Physics 2016-11-28 Josep Planelles , Fernando Rajadell , Juan I. Climente

We present an experimental demonstration of strong coupling between a surface plasmon propagating on a planar silver substrate, and the lowest excited state of CdSe nanocrystals. Variable-angle spectroscopic ellipsometry measurements…

Materials Science · Physics 2009-12-16 D. E. Gómez , K. C. Vernon , T. J. Davis , T. L. Nguyen , P. Mulvaney

The energy levels and optical transitions of tetrahedral core/shell InP/ZnSe quantum dots (QDs) are investigated by means of multi-band k$\cdot$p theory. Despite the $\overline{T}_d$ symmetry relaxing spherical selection rules, the…

Mesoscale and Nanoscale Physics · Physics 2026-04-06 Josep Planelles , Juan I. Climente

Time-resolved photoluminescence (PL) and micro-PL imaging were used to study single CdS nanowires at 10 K. The low-temperature PL of all CdS nanowires exhibit spectral features near energies associated with free and bound exciton…

It is widely accepted that the properties of most semiconductor nanocrystals can be tuned by their core size, shape and material. In covalent semiconductor nanocrystal materials, such as silicon, germanium or carbon, certain degree of…

Mesoscale and Nanoscale Physics · Physics 2019-05-30 Katerina Dohnalova Newell , Prokop Hapala , Katerina Kusova , Ivan Infante

Due to the spatial confinement, two-dimensional metal chalcogenides display an extraordinary optical re-sponse and carrier transport ability. Solution-based synthesis techniques such as colloidal hot injection and ion exchange provide a…

Materials Science · Physics 2021-10-25 Ziyi Hu , Ryan O'Neill , Rostyslav Lesyuk , Christian Klinke
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